Solution processable and optically switchable 1D photonic structures

Abstract We report the first demonstration of a solution processable, optically switchable 1D photonic crystal which incorporates phototunable doped metal oxide nanocrystals. The resulting device structure shows a dual optical response with the photonic bandgap covering the visible spectral range an...

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Autores principales: Giuseppe M. Paternò, Chiara Iseppon, Alessia D’Altri, Carlo Fasanotti, Giulia Merati, Mattia Randi, Andrea Desii, Eva A. A. Pogna, Daniele Viola, Giulio Cerullo, Francesco Scotognella, Ilka Kriegel
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Lenguaje:EN
Publicado: Nature Portfolio 2018
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Acceso en línea:https://doaj.org/article/9a33d3f631b04b33838536afc0a89335
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spelling oai:doaj.org-article:9a33d3f631b04b33838536afc0a893352021-12-02T11:40:46ZSolution processable and optically switchable 1D photonic structures10.1038/s41598-018-21824-w2045-2322https://doaj.org/article/9a33d3f631b04b33838536afc0a893352018-02-01T00:00:00Zhttps://doi.org/10.1038/s41598-018-21824-whttps://doaj.org/toc/2045-2322Abstract We report the first demonstration of a solution processable, optically switchable 1D photonic crystal which incorporates phototunable doped metal oxide nanocrystals. The resulting device structure shows a dual optical response with the photonic bandgap covering the visible spectral range and the plasmon resonance of the doped metal oxide the near infrared. By means of a facile photodoping process, we tuned the plasmonic response and switched effectively the optical properties of the photonic crystal, translating the effect from the near infrared to the visible. The ultrafast bandgap pumping induces a signal change in the region of the photonic stopband, with recovery times of several picoseconds, providing a step toward the ultrafast optical switching. Optical modeling uncovers the importance of a complete modeling of the variations of the dielectric function of the photodoped material, including the high frequency region of the Drude response which is responsible for the strong switching in the visible after photodoping. Our device configuration offers unprecedented tunability due to flexibility in device design, covering a wavelength range from the visible to the near infrared. Our findings indicate a new protocol to modify the optical response of photonic devices by optical triggers only.Giuseppe M. PaternòChiara IsepponAlessia D’AltriCarlo FasanottiGiulia MeratiMattia RandiAndrea DesiiEva A. A. PognaDaniele ViolaGiulio CerulloFrancesco ScotognellaIlka KriegelNature PortfolioarticleMedicineRScienceQENScientific Reports, Vol 8, Iss 1, Pp 1-8 (2018)
institution DOAJ
collection DOAJ
language EN
topic Medicine
R
Science
Q
spellingShingle Medicine
R
Science
Q
Giuseppe M. Paternò
Chiara Iseppon
Alessia D’Altri
Carlo Fasanotti
Giulia Merati
Mattia Randi
Andrea Desii
Eva A. A. Pogna
Daniele Viola
Giulio Cerullo
Francesco Scotognella
Ilka Kriegel
Solution processable and optically switchable 1D photonic structures
description Abstract We report the first demonstration of a solution processable, optically switchable 1D photonic crystal which incorporates phototunable doped metal oxide nanocrystals. The resulting device structure shows a dual optical response with the photonic bandgap covering the visible spectral range and the plasmon resonance of the doped metal oxide the near infrared. By means of a facile photodoping process, we tuned the plasmonic response and switched effectively the optical properties of the photonic crystal, translating the effect from the near infrared to the visible. The ultrafast bandgap pumping induces a signal change in the region of the photonic stopband, with recovery times of several picoseconds, providing a step toward the ultrafast optical switching. Optical modeling uncovers the importance of a complete modeling of the variations of the dielectric function of the photodoped material, including the high frequency region of the Drude response which is responsible for the strong switching in the visible after photodoping. Our device configuration offers unprecedented tunability due to flexibility in device design, covering a wavelength range from the visible to the near infrared. Our findings indicate a new protocol to modify the optical response of photonic devices by optical triggers only.
format article
author Giuseppe M. Paternò
Chiara Iseppon
Alessia D’Altri
Carlo Fasanotti
Giulia Merati
Mattia Randi
Andrea Desii
Eva A. A. Pogna
Daniele Viola
Giulio Cerullo
Francesco Scotognella
Ilka Kriegel
author_facet Giuseppe M. Paternò
Chiara Iseppon
Alessia D’Altri
Carlo Fasanotti
Giulia Merati
Mattia Randi
Andrea Desii
Eva A. A. Pogna
Daniele Viola
Giulio Cerullo
Francesco Scotognella
Ilka Kriegel
author_sort Giuseppe M. Paternò
title Solution processable and optically switchable 1D photonic structures
title_short Solution processable and optically switchable 1D photonic structures
title_full Solution processable and optically switchable 1D photonic structures
title_fullStr Solution processable and optically switchable 1D photonic structures
title_full_unstemmed Solution processable and optically switchable 1D photonic structures
title_sort solution processable and optically switchable 1d photonic structures
publisher Nature Portfolio
publishDate 2018
url https://doaj.org/article/9a33d3f631b04b33838536afc0a89335
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