Room temperature ferroelectricity in fluoroperovskite thin films
Abstract The NaMnF3 fluoride-perovskite has been found, theoretically, to be ferroelectric under epitaxial strain becoming a promising alternative to conventional oxides for multiferroic applications. Nevertheless, this fluoroperovskite has not been experimentally verified to be ferroelectric so far...
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Nature Portfolio
2017
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oai:doaj.org-article:9b36e039cb684dd18977fcc700337d6f2021-12-02T12:32:04ZRoom temperature ferroelectricity in fluoroperovskite thin films10.1038/s41598-017-07834-02045-2322https://doaj.org/article/9b36e039cb684dd18977fcc700337d6f2017-08-01T00:00:00Zhttps://doi.org/10.1038/s41598-017-07834-0https://doaj.org/toc/2045-2322Abstract The NaMnF3 fluoride-perovskite has been found, theoretically, to be ferroelectric under epitaxial strain becoming a promising alternative to conventional oxides for multiferroic applications. Nevertheless, this fluoroperovskite has not been experimentally verified to be ferroelectric so far. Here we report signatures of room temperature ferroelectricity observed in perovskite NaMnF3 thin films grown on SrTiO3. Using piezoresponse force microscopy, we studied the evolution of ferroelectric polarization in response to external and built-in electric fields. Density functional theory calculations were also performed to help understand the strong competition between ferroelectric and paraelectric phases as well as the profound influences of strain. These results, together with the magnetic order previously reported in the same material, pave the way to future multiferroic and magnetoelectric investigations in fluoroperovskites.Ming YangAmit KCA. C. Garcia-CastroPavel BorisovE. BousquetDavid LedermanAldo H. RomeroCheng CenNature PortfolioarticleMedicineRScienceQENScientific Reports, Vol 7, Iss 1, Pp 1-9 (2017) |
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Medicine R Science Q Ming Yang Amit KC A. C. Garcia-Castro Pavel Borisov E. Bousquet David Lederman Aldo H. Romero Cheng Cen Room temperature ferroelectricity in fluoroperovskite thin films |
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Abstract The NaMnF3 fluoride-perovskite has been found, theoretically, to be ferroelectric under epitaxial strain becoming a promising alternative to conventional oxides for multiferroic applications. Nevertheless, this fluoroperovskite has not been experimentally verified to be ferroelectric so far. Here we report signatures of room temperature ferroelectricity observed in perovskite NaMnF3 thin films grown on SrTiO3. Using piezoresponse force microscopy, we studied the evolution of ferroelectric polarization in response to external and built-in electric fields. Density functional theory calculations were also performed to help understand the strong competition between ferroelectric and paraelectric phases as well as the profound influences of strain. These results, together with the magnetic order previously reported in the same material, pave the way to future multiferroic and magnetoelectric investigations in fluoroperovskites. |
format |
article |
author |
Ming Yang Amit KC A. C. Garcia-Castro Pavel Borisov E. Bousquet David Lederman Aldo H. Romero Cheng Cen |
author_facet |
Ming Yang Amit KC A. C. Garcia-Castro Pavel Borisov E. Bousquet David Lederman Aldo H. Romero Cheng Cen |
author_sort |
Ming Yang |
title |
Room temperature ferroelectricity in fluoroperovskite thin films |
title_short |
Room temperature ferroelectricity in fluoroperovskite thin films |
title_full |
Room temperature ferroelectricity in fluoroperovskite thin films |
title_fullStr |
Room temperature ferroelectricity in fluoroperovskite thin films |
title_full_unstemmed |
Room temperature ferroelectricity in fluoroperovskite thin films |
title_sort |
room temperature ferroelectricity in fluoroperovskite thin films |
publisher |
Nature Portfolio |
publishDate |
2017 |
url |
https://doaj.org/article/9b36e039cb684dd18977fcc700337d6f |
work_keys_str_mv |
AT mingyang roomtemperatureferroelectricityinfluoroperovskitethinfilms AT amitkc roomtemperatureferroelectricityinfluoroperovskitethinfilms AT acgarciacastro roomtemperatureferroelectricityinfluoroperovskitethinfilms AT pavelborisov roomtemperatureferroelectricityinfluoroperovskitethinfilms AT ebousquet roomtemperatureferroelectricityinfluoroperovskitethinfilms AT davidlederman roomtemperatureferroelectricityinfluoroperovskitethinfilms AT aldohromero roomtemperatureferroelectricityinfluoroperovskitethinfilms AT chengcen roomtemperatureferroelectricityinfluoroperovskitethinfilms |
_version_ |
1718394174382800896 |