Single-atom catalytic growth of crystals using graphene as a case study

Abstract Anchored Single-atom catalysts have emerged as a cutting-edge research field holding tremendous appeal for applications in the fields of chemicals, energy and the environment. However, single-atom-catalysts for crystal growth is a nascent field. Of the few studies available, all of them are...

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Autores principales:	Xiaoqin Yang, Yu Liu, Huy Q. Ta, Ehsan Rezvani, Yue Zhang, Mengqi Zeng, Lei Fu, Alicja Bachmatiuk, Jinping Luo, Lijun Liu, Mark H. Rümmeli
Formato:	article
Lenguaje:	EN
Publicado:	Nature Portfolio 2021
Materias:	Materials of engineering and construction. Mechanics of materials TA401-492 Chemistry QD1-999
Acceso en línea:	https://doaj.org/article/9ba8b0e3a4b14062a9166dab70351e4a
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spelling	oai:doaj.org-article:9ba8b0e3a4b14062a9166dab70351e4a2021-12-05T12:25:26ZSingle-atom catalytic growth of crystals using graphene as a case study10.1038/s41699-021-00267-42397-7132https://doaj.org/article/9ba8b0e3a4b14062a9166dab70351e4a2021-12-01T00:00:00Zhttps://doi.org/10.1038/s41699-021-00267-4https://doaj.org/toc/2397-7132Abstract Anchored Single-atom catalysts have emerged as a cutting-edge research field holding tremendous appeal for applications in the fields of chemicals, energy and the environment. However, single-atom-catalysts for crystal growth is a nascent field. Of the few studies available, all of them are based on state-of-the-art in situ microscopy investigations and computational studies, and they all look at the growth of monolayer graphene from a single-atom catalyst. Despite the limited number of studies, they do, collectively, represent a new sub-field of single-atom catalysis, namely single-atom catalytic growth of crystalline solids. In this review, we examine them on substrate-supported and as freestanding graphene fabrication, as well as rolled-up graphene, viz., single-walled carbon nanotubes (SWCNT), grown from a single atom. We also briefly discuss the catalytic etching of graphene and SWCNT’s and conclude by outlining the future directions we envision this nascent field to take.Xiaoqin YangYu LiuHuy Q. TaEhsan RezvaniYue ZhangMengqi ZengLei FuAlicja BachmatiukJinping LuoLijun LiuMark H. RümmeliNature PortfolioarticleMaterials of engineering and construction. Mechanics of materialsTA401-492ChemistryQD1-999ENnpj 2D Materials and Applications, Vol 5, Iss 1, Pp 1-13 (2021)
institution	DOAJ
collection	DOAJ
language	EN
topic	Materials of engineering and construction. Mechanics of materials TA401-492 Chemistry QD1-999
spellingShingle	Materials of engineering and construction. Mechanics of materials TA401-492 Chemistry QD1-999 Xiaoqin Yang Yu Liu Huy Q. Ta Ehsan Rezvani Yue Zhang Mengqi Zeng Lei Fu Alicja Bachmatiuk Jinping Luo Lijun Liu Mark H. Rümmeli Single-atom catalytic growth of crystals using graphene as a case study
description	Abstract Anchored Single-atom catalysts have emerged as a cutting-edge research field holding tremendous appeal for applications in the fields of chemicals, energy and the environment. However, single-atom-catalysts for crystal growth is a nascent field. Of the few studies available, all of them are based on state-of-the-art in situ microscopy investigations and computational studies, and they all look at the growth of monolayer graphene from a single-atom catalyst. Despite the limited number of studies, they do, collectively, represent a new sub-field of single-atom catalysis, namely single-atom catalytic growth of crystalline solids. In this review, we examine them on substrate-supported and as freestanding graphene fabrication, as well as rolled-up graphene, viz., single-walled carbon nanotubes (SWCNT), grown from a single atom. We also briefly discuss the catalytic etching of graphene and SWCNT’s and conclude by outlining the future directions we envision this nascent field to take.
format	article
author	Xiaoqin Yang Yu Liu Huy Q. Ta Ehsan Rezvani Yue Zhang Mengqi Zeng Lei Fu Alicja Bachmatiuk Jinping Luo Lijun Liu Mark H. Rümmeli
author_facet	Xiaoqin Yang Yu Liu Huy Q. Ta Ehsan Rezvani Yue Zhang Mengqi Zeng Lei Fu Alicja Bachmatiuk Jinping Luo Lijun Liu Mark H. Rümmeli
author_sort	Xiaoqin Yang
title	Single-atom catalytic growth of crystals using graphene as a case study
title_short	Single-atom catalytic growth of crystals using graphene as a case study
title_full	Single-atom catalytic growth of crystals using graphene as a case study
title_fullStr	Single-atom catalytic growth of crystals using graphene as a case study
title_full_unstemmed	Single-atom catalytic growth of crystals using graphene as a case study
title_sort	single-atom catalytic growth of crystals using graphene as a case study
publisher	Nature Portfolio
publishDate	2021
url	https://doaj.org/article/9ba8b0e3a4b14062a9166dab70351e4a
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Single-atom catalytic growth of crystals using graphene as a case study

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