Intermediate stages of electrochemical oxidation of single-crystalline platinum revealed by in situ Raman spectroscopy

Understanding degradation of platinum catalysts during oxygen reduction is vital for improving proton-exchange membrane fuel cells. Here, the authors identify intermediate stages in the oxidation of Pt(111) and Pt(100) in perchloric acid using in situshell-isolated nanoparticle-enhanced Raman spectr...

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Autores principales: Yi-Fan Huang, Patricia J. Kooyman, Marc T. M. Koper
Formato: article
Lenguaje:EN
Publicado: Nature Portfolio 2016
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Acceso en línea:https://doaj.org/article/9c443b6f23a9477cb83a1e8e23e62fde
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spelling oai:doaj.org-article:9c443b6f23a9477cb83a1e8e23e62fde2021-12-02T16:49:42ZIntermediate stages of electrochemical oxidation of single-crystalline platinum revealed by in situ Raman spectroscopy10.1038/ncomms124402041-1723https://doaj.org/article/9c443b6f23a9477cb83a1e8e23e62fde2016-08-01T00:00:00Zhttps://doi.org/10.1038/ncomms12440https://doaj.org/toc/2041-1723Understanding degradation of platinum catalysts during oxygen reduction is vital for improving proton-exchange membrane fuel cells. Here, the authors identify intermediate stages in the oxidation of Pt(111) and Pt(100) in perchloric acid using in situshell-isolated nanoparticle-enhanced Raman spectroscopy.Yi-Fan HuangPatricia J. KooymanMarc T. M. KoperNature PortfolioarticleScienceQENNature Communications, Vol 7, Iss 1, Pp 1-7 (2016)
institution DOAJ
collection DOAJ
language EN
topic Science
Q
spellingShingle Science
Q
Yi-Fan Huang
Patricia J. Kooyman
Marc T. M. Koper
Intermediate stages of electrochemical oxidation of single-crystalline platinum revealed by in situ Raman spectroscopy
description Understanding degradation of platinum catalysts during oxygen reduction is vital for improving proton-exchange membrane fuel cells. Here, the authors identify intermediate stages in the oxidation of Pt(111) and Pt(100) in perchloric acid using in situshell-isolated nanoparticle-enhanced Raman spectroscopy.
format article
author Yi-Fan Huang
Patricia J. Kooyman
Marc T. M. Koper
author_facet Yi-Fan Huang
Patricia J. Kooyman
Marc T. M. Koper
author_sort Yi-Fan Huang
title Intermediate stages of electrochemical oxidation of single-crystalline platinum revealed by in situ Raman spectroscopy
title_short Intermediate stages of electrochemical oxidation of single-crystalline platinum revealed by in situ Raman spectroscopy
title_full Intermediate stages of electrochemical oxidation of single-crystalline platinum revealed by in situ Raman spectroscopy
title_fullStr Intermediate stages of electrochemical oxidation of single-crystalline platinum revealed by in situ Raman spectroscopy
title_full_unstemmed Intermediate stages of electrochemical oxidation of single-crystalline platinum revealed by in situ Raman spectroscopy
title_sort intermediate stages of electrochemical oxidation of single-crystalline platinum revealed by in situ raman spectroscopy
publisher Nature Portfolio
publishDate 2016
url https://doaj.org/article/9c443b6f23a9477cb83a1e8e23e62fde
work_keys_str_mv AT yifanhuang intermediatestagesofelectrochemicaloxidationofsinglecrystallineplatinumrevealedbyinsituramanspectroscopy
AT patriciajkooyman intermediatestagesofelectrochemicaloxidationofsinglecrystallineplatinumrevealedbyinsituramanspectroscopy
AT marctmkoper intermediatestagesofelectrochemicaloxidationofsinglecrystallineplatinumrevealedbyinsituramanspectroscopy
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