Materializing efficient methanol oxidation via electron delocalization in nickel hydroxide nanoribbon

Development of suitable methanol oxidation reaction catalysts for direct methanol fuel cells is challenging due to sluggish kinetics. Herein, authors show that four-coordinate nickel atoms form charge-transfer orbitals near the Fermi energy level, leading to remarkable methanol oxidation activity.

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Autores principales:	Xiaopeng Wang, Shibo Xi, Wee Siang Vincent Lee, Pengru Huang, Peng Cui, Lei Zhao, Weichang Hao, Xinsheng Zhao, Zhenbo Wang, Haijun Wu, Hao Wang, Caozheng Diao, Armando Borgna, Yonghua Du, Zhi Gen Yu, Stephen Pennycook, Junmin Xue
Formato:	article
Lenguaje:	EN
Publicado:	Nature Portfolio 2020
Materias:	Science Q
Acceso en línea:	https://doaj.org/article/9f927ea6b1e14dd7aa94294106b4849e
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spelling	oai:doaj.org-article:9f927ea6b1e14dd7aa94294106b4849e2021-12-02T18:02:08ZMaterializing efficient methanol oxidation via electron delocalization in nickel hydroxide nanoribbon10.1038/s41467-020-18459-92041-1723https://doaj.org/article/9f927ea6b1e14dd7aa94294106b4849e2020-09-01T00:00:00Zhttps://doi.org/10.1038/s41467-020-18459-9https://doaj.org/toc/2041-1723Development of suitable methanol oxidation reaction catalysts for direct methanol fuel cells is challenging due to sluggish kinetics. Herein, authors show that four-coordinate nickel atoms form charge-transfer orbitals near the Fermi energy level, leading to remarkable methanol oxidation activity.Xiaopeng WangShibo XiWee Siang Vincent LeePengru HuangPeng CuiLei ZhaoWeichang HaoXinsheng ZhaoZhenbo WangHaijun WuHao WangCaozheng DiaoArmando BorgnaYonghua DuZhi Gen YuStephen PennycookJunmin XueNature PortfolioarticleScienceQENNature Communications, Vol 11, Iss 1, Pp 1-9 (2020)
institution	DOAJ
collection	DOAJ
language	EN
topic	Science Q
spellingShingle	Science Q Xiaopeng Wang Shibo Xi Wee Siang Vincent Lee Pengru Huang Peng Cui Lei Zhao Weichang Hao Xinsheng Zhao Zhenbo Wang Haijun Wu Hao Wang Caozheng Diao Armando Borgna Yonghua Du Zhi Gen Yu Stephen Pennycook Junmin Xue Materializing efficient methanol oxidation via electron delocalization in nickel hydroxide nanoribbon
description	Development of suitable methanol oxidation reaction catalysts for direct methanol fuel cells is challenging due to sluggish kinetics. Herein, authors show that four-coordinate nickel atoms form charge-transfer orbitals near the Fermi energy level, leading to remarkable methanol oxidation activity.
format	article
author	Xiaopeng Wang Shibo Xi Wee Siang Vincent Lee Pengru Huang Peng Cui Lei Zhao Weichang Hao Xinsheng Zhao Zhenbo Wang Haijun Wu Hao Wang Caozheng Diao Armando Borgna Yonghua Du Zhi Gen Yu Stephen Pennycook Junmin Xue
author_facet	Xiaopeng Wang Shibo Xi Wee Siang Vincent Lee Pengru Huang Peng Cui Lei Zhao Weichang Hao Xinsheng Zhao Zhenbo Wang Haijun Wu Hao Wang Caozheng Diao Armando Borgna Yonghua Du Zhi Gen Yu Stephen Pennycook Junmin Xue
author_sort	Xiaopeng Wang
title	Materializing efficient methanol oxidation via electron delocalization in nickel hydroxide nanoribbon
title_short	Materializing efficient methanol oxidation via electron delocalization in nickel hydroxide nanoribbon
title_full	Materializing efficient methanol oxidation via electron delocalization in nickel hydroxide nanoribbon
title_fullStr	Materializing efficient methanol oxidation via electron delocalization in nickel hydroxide nanoribbon
title_full_unstemmed	Materializing efficient methanol oxidation via electron delocalization in nickel hydroxide nanoribbon
title_sort	materializing efficient methanol oxidation via electron delocalization in nickel hydroxide nanoribbon
publisher	Nature Portfolio
publishDate	2020
url	https://doaj.org/article/9f927ea6b1e14dd7aa94294106b4849e
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Materializing efficient methanol oxidation via electron delocalization in nickel hydroxide nanoribbon

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