Dynamics from elastic neutron-scattering via direct measurement of the running time-integral of the van Hove distribution function

Abstract We present a new neutron-scattering approach to access the van Hove distribution function directly in the time domain, I(t), which reflects the system dynamics. Currently, I(t) is essentially determined from neutron energy-exchange. Our method consists of the straightforward measurement of...

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Autores principales: Antonio Benedetto, Gordon J. Kearley
Formato: article
Lenguaje:EN
Publicado: Nature Portfolio 2019
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Acceso en línea:https://doaj.org/article/a057147fc5bb41619e94e0176bc720bb
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spelling oai:doaj.org-article:a057147fc5bb41619e94e0176bc720bb2021-12-02T15:07:55ZDynamics from elastic neutron-scattering via direct measurement of the running time-integral of the van Hove distribution function10.1038/s41598-019-46835-z2045-2322https://doaj.org/article/a057147fc5bb41619e94e0176bc720bb2019-08-01T00:00:00Zhttps://doi.org/10.1038/s41598-019-46835-zhttps://doaj.org/toc/2045-2322Abstract We present a new neutron-scattering approach to access the van Hove distribution function directly in the time domain, I(t), which reflects the system dynamics. Currently, I(t) is essentially determined from neutron energy-exchange. Our method consists of the straightforward measurement of the running time-integral of I(t), by computing the portion of scattered neutrons corresponding to species at rest within a time t, (conceptually elastic scattering). Previous attempts failed to recognise this connection. Starting from a theoretical standpoint, a practical realisation is assessed via numerical methods and an instrument simulation.Antonio BenedettoGordon J. KearleyNature PortfolioarticleMedicineRScienceQENScientific Reports, Vol 9, Iss 1, Pp 1-6 (2019)
institution DOAJ
collection DOAJ
language EN
topic Medicine
R
Science
Q
spellingShingle Medicine
R
Science
Q
Antonio Benedetto
Gordon J. Kearley
Dynamics from elastic neutron-scattering via direct measurement of the running time-integral of the van Hove distribution function
description Abstract We present a new neutron-scattering approach to access the van Hove distribution function directly in the time domain, I(t), which reflects the system dynamics. Currently, I(t) is essentially determined from neutron energy-exchange. Our method consists of the straightforward measurement of the running time-integral of I(t), by computing the portion of scattered neutrons corresponding to species at rest within a time t, (conceptually elastic scattering). Previous attempts failed to recognise this connection. Starting from a theoretical standpoint, a practical realisation is assessed via numerical methods and an instrument simulation.
format article
author Antonio Benedetto
Gordon J. Kearley
author_facet Antonio Benedetto
Gordon J. Kearley
author_sort Antonio Benedetto
title Dynamics from elastic neutron-scattering via direct measurement of the running time-integral of the van Hove distribution function
title_short Dynamics from elastic neutron-scattering via direct measurement of the running time-integral of the van Hove distribution function
title_full Dynamics from elastic neutron-scattering via direct measurement of the running time-integral of the van Hove distribution function
title_fullStr Dynamics from elastic neutron-scattering via direct measurement of the running time-integral of the van Hove distribution function
title_full_unstemmed Dynamics from elastic neutron-scattering via direct measurement of the running time-integral of the van Hove distribution function
title_sort dynamics from elastic neutron-scattering via direct measurement of the running time-integral of the van hove distribution function
publisher Nature Portfolio
publishDate 2019
url https://doaj.org/article/a057147fc5bb41619e94e0176bc720bb
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AT gordonjkearley dynamicsfromelasticneutronscatteringviadirectmeasurementoftherunningtimeintegralofthevanhovedistributionfunction
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