Laser-induced thermal grating spectroscopy based on femtosecond laser multi-photon absorption

Abstract Laser-induced grating spectroscopy (LIGS) is for the first time explored in a configuration based on the crossing of two focused femtosecond (fs) laser pulses (800-nm wavelength) and a focused continuous-wave (cw) laser beam (532-nm wavelength). A thermal grating was formed by multi-photon...

Descripción completa

Guardado en:
Detalles Bibliográficos
Autores principales: Maria Ruchkina, Dina Hot, Pengji Ding, Ali Hosseinnia, Per-Erik Bengtsson, Zhongshan Li, Joakim Bood, Anna-Lena Sahlberg
Formato: article
Lenguaje:EN
Publicado: Nature Portfolio 2021
Materias:
R
Q
Acceso en línea:https://doaj.org/article/a14b14efa625449a8fadee4b0ad17762
Etiquetas: Agregar Etiqueta
Sin Etiquetas, Sea el primero en etiquetar este registro!
id oai:doaj.org-article:a14b14efa625449a8fadee4b0ad17762
record_format dspace
spelling oai:doaj.org-article:a14b14efa625449a8fadee4b0ad177622021-12-02T16:51:03ZLaser-induced thermal grating spectroscopy based on femtosecond laser multi-photon absorption10.1038/s41598-021-89269-22045-2322https://doaj.org/article/a14b14efa625449a8fadee4b0ad177622021-05-01T00:00:00Zhttps://doi.org/10.1038/s41598-021-89269-2https://doaj.org/toc/2045-2322Abstract Laser-induced grating spectroscopy (LIGS) is for the first time explored in a configuration based on the crossing of two focused femtosecond (fs) laser pulses (800-nm wavelength) and a focused continuous-wave (cw) laser beam (532-nm wavelength). A thermal grating was formed by multi-photon absorption of the fs-laser pulses by $$\hbox {N}_{{2}}$$ N 2 with a pulse energy around 700 $$\upmu $$ μ J ( $$\sim $$ ∼ 45 TW/ $$\hbox {cm}^{2}$$ cm 2 ). The feasibility of this LIGS configuration was investigated for thermometry in heated nitrogen gas flows. The temperature was varied from room temperature up to 750 K, producing strong single-shot LIGS signals. A model based on the solution of the linearized hydrodynamic equations was used to extract temperature information from single-shot experimental data, and the results show excellent agreement with the thermocouple measurements. Furthermore, the fluorescence produced by the fs-laser pulses was investigated. This study indicates an 8-photon absorption pathway for $$\hbox {N}_{{2}}$$ N 2 in order to reach the $$\hbox {B}^{3}\Pi _{g}$$ B 3 Π g state from the ground state, and 8 + 5 photon excitation to reach the $$\hbox {B}^{2}\Sigma _{u}^{+}$$ B 2 Σ u + state of the $$\hbox {N}_{2}^{+}$$ N 2 + ion. At pulse energies higher than 1 mJ, the LIGS signal was disturbed due to the generation of plasma. Additionally, measurements in argon gas and air were performed, where the LIGS signal for argon shows lower intensity compared to air and $$\hbox {N}_{{2}}$$ N 2 .Maria RuchkinaDina HotPengji DingAli HosseinniaPer-Erik BengtssonZhongshan LiJoakim BoodAnna-Lena SahlbergNature PortfolioarticleMedicineRScienceQENScientific Reports, Vol 11, Iss 1, Pp 1-13 (2021)
institution DOAJ
collection DOAJ
language EN
topic Medicine
R
Science
Q
spellingShingle Medicine
R
Science
Q
Maria Ruchkina
Dina Hot
Pengji Ding
Ali Hosseinnia
Per-Erik Bengtsson
Zhongshan Li
Joakim Bood
Anna-Lena Sahlberg
Laser-induced thermal grating spectroscopy based on femtosecond laser multi-photon absorption
description Abstract Laser-induced grating spectroscopy (LIGS) is for the first time explored in a configuration based on the crossing of two focused femtosecond (fs) laser pulses (800-nm wavelength) and a focused continuous-wave (cw) laser beam (532-nm wavelength). A thermal grating was formed by multi-photon absorption of the fs-laser pulses by $$\hbox {N}_{{2}}$$ N 2 with a pulse energy around 700 $$\upmu $$ μ J ( $$\sim $$ ∼ 45 TW/ $$\hbox {cm}^{2}$$ cm 2 ). The feasibility of this LIGS configuration was investigated for thermometry in heated nitrogen gas flows. The temperature was varied from room temperature up to 750 K, producing strong single-shot LIGS signals. A model based on the solution of the linearized hydrodynamic equations was used to extract temperature information from single-shot experimental data, and the results show excellent agreement with the thermocouple measurements. Furthermore, the fluorescence produced by the fs-laser pulses was investigated. This study indicates an 8-photon absorption pathway for $$\hbox {N}_{{2}}$$ N 2 in order to reach the $$\hbox {B}^{3}\Pi _{g}$$ B 3 Π g state from the ground state, and 8 + 5 photon excitation to reach the $$\hbox {B}^{2}\Sigma _{u}^{+}$$ B 2 Σ u + state of the $$\hbox {N}_{2}^{+}$$ N 2 + ion. At pulse energies higher than 1 mJ, the LIGS signal was disturbed due to the generation of plasma. Additionally, measurements in argon gas and air were performed, where the LIGS signal for argon shows lower intensity compared to air and $$\hbox {N}_{{2}}$$ N 2 .
format article
author Maria Ruchkina
Dina Hot
Pengji Ding
Ali Hosseinnia
Per-Erik Bengtsson
Zhongshan Li
Joakim Bood
Anna-Lena Sahlberg
author_facet Maria Ruchkina
Dina Hot
Pengji Ding
Ali Hosseinnia
Per-Erik Bengtsson
Zhongshan Li
Joakim Bood
Anna-Lena Sahlberg
author_sort Maria Ruchkina
title Laser-induced thermal grating spectroscopy based on femtosecond laser multi-photon absorption
title_short Laser-induced thermal grating spectroscopy based on femtosecond laser multi-photon absorption
title_full Laser-induced thermal grating spectroscopy based on femtosecond laser multi-photon absorption
title_fullStr Laser-induced thermal grating spectroscopy based on femtosecond laser multi-photon absorption
title_full_unstemmed Laser-induced thermal grating spectroscopy based on femtosecond laser multi-photon absorption
title_sort laser-induced thermal grating spectroscopy based on femtosecond laser multi-photon absorption
publisher Nature Portfolio
publishDate 2021
url https://doaj.org/article/a14b14efa625449a8fadee4b0ad17762
work_keys_str_mv AT mariaruchkina laserinducedthermalgratingspectroscopybasedonfemtosecondlasermultiphotonabsorption
AT dinahot laserinducedthermalgratingspectroscopybasedonfemtosecondlasermultiphotonabsorption
AT pengjiding laserinducedthermalgratingspectroscopybasedonfemtosecondlasermultiphotonabsorption
AT alihosseinnia laserinducedthermalgratingspectroscopybasedonfemtosecondlasermultiphotonabsorption
AT pererikbengtsson laserinducedthermalgratingspectroscopybasedonfemtosecondlasermultiphotonabsorption
AT zhongshanli laserinducedthermalgratingspectroscopybasedonfemtosecondlasermultiphotonabsorption
AT joakimbood laserinducedthermalgratingspectroscopybasedonfemtosecondlasermultiphotonabsorption
AT annalenasahlberg laserinducedthermalgratingspectroscopybasedonfemtosecondlasermultiphotonabsorption
_version_ 1718382997738094592