Fundamental limits of electron and nuclear spin qubit lifetimes in an isolated self-assembled quantum dot
Abstract Combining external control with long spin lifetime and coherence is a key challenge for solid state spin qubits. Tunnel coupling with electron Fermi reservoir provides robust charge state control in semiconductor quantum dots, but results in undesired relaxation of electron and nuclear spin...
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Nature Portfolio
2021
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oai:doaj.org-article:a14ee07b5c1f41418c96d2a4cad0efc12021-12-02T13:35:05ZFundamental limits of electron and nuclear spin qubit lifetimes in an isolated self-assembled quantum dot10.1038/s41534-021-00378-22056-6387https://doaj.org/article/a14ee07b5c1f41418c96d2a4cad0efc12021-02-01T00:00:00Zhttps://doi.org/10.1038/s41534-021-00378-2https://doaj.org/toc/2056-6387Abstract Combining external control with long spin lifetime and coherence is a key challenge for solid state spin qubits. Tunnel coupling with electron Fermi reservoir provides robust charge state control in semiconductor quantum dots, but results in undesired relaxation of electron and nuclear spins through mechanisms that lack complete understanding. Here, we unravel the contributions of tunnelling-assisted and phonon-assisted spin relaxation mechanisms by systematically adjusting the tunnelling coupling in a wide range, including the limit of an isolated quantum dot. These experiments reveal fundamental limits and trade-offs of quantum dot spin dynamics: while reduced tunnelling can be used to achieve electron spin qubit lifetimes exceeding 1 s, the optical spin initialisation fidelity is reduced below 80%, limited by Auger recombination. Comprehensive understanding of electron-nuclear spin relaxation attained here provides a roadmap for design of the optimal operating conditions in quantum dot spin qubits.George GillardIan M. GriffithsGautham RagunathanAta UlhaqCallum McEwanEdmund ClarkeEvgeny A. ChekhovichNature PortfolioarticlePhysicsQC1-999Electronic computers. Computer scienceQA75.5-76.95ENnpj Quantum Information, Vol 7, Iss 1, Pp 1-8 (2021) |
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Physics QC1-999 Electronic computers. Computer science QA75.5-76.95 |
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Physics QC1-999 Electronic computers. Computer science QA75.5-76.95 George Gillard Ian M. Griffiths Gautham Ragunathan Ata Ulhaq Callum McEwan Edmund Clarke Evgeny A. Chekhovich Fundamental limits of electron and nuclear spin qubit lifetimes in an isolated self-assembled quantum dot |
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Abstract Combining external control with long spin lifetime and coherence is a key challenge for solid state spin qubits. Tunnel coupling with electron Fermi reservoir provides robust charge state control in semiconductor quantum dots, but results in undesired relaxation of electron and nuclear spins through mechanisms that lack complete understanding. Here, we unravel the contributions of tunnelling-assisted and phonon-assisted spin relaxation mechanisms by systematically adjusting the tunnelling coupling in a wide range, including the limit of an isolated quantum dot. These experiments reveal fundamental limits and trade-offs of quantum dot spin dynamics: while reduced tunnelling can be used to achieve electron spin qubit lifetimes exceeding 1 s, the optical spin initialisation fidelity is reduced below 80%, limited by Auger recombination. Comprehensive understanding of electron-nuclear spin relaxation attained here provides a roadmap for design of the optimal operating conditions in quantum dot spin qubits. |
format |
article |
author |
George Gillard Ian M. Griffiths Gautham Ragunathan Ata Ulhaq Callum McEwan Edmund Clarke Evgeny A. Chekhovich |
author_facet |
George Gillard Ian M. Griffiths Gautham Ragunathan Ata Ulhaq Callum McEwan Edmund Clarke Evgeny A. Chekhovich |
author_sort |
George Gillard |
title |
Fundamental limits of electron and nuclear spin qubit lifetimes in an isolated self-assembled quantum dot |
title_short |
Fundamental limits of electron and nuclear spin qubit lifetimes in an isolated self-assembled quantum dot |
title_full |
Fundamental limits of electron and nuclear spin qubit lifetimes in an isolated self-assembled quantum dot |
title_fullStr |
Fundamental limits of electron and nuclear spin qubit lifetimes in an isolated self-assembled quantum dot |
title_full_unstemmed |
Fundamental limits of electron and nuclear spin qubit lifetimes in an isolated self-assembled quantum dot |
title_sort |
fundamental limits of electron and nuclear spin qubit lifetimes in an isolated self-assembled quantum dot |
publisher |
Nature Portfolio |
publishDate |
2021 |
url |
https://doaj.org/article/a14ee07b5c1f41418c96d2a4cad0efc1 |
work_keys_str_mv |
AT georgegillard fundamentallimitsofelectronandnuclearspinqubitlifetimesinanisolatedselfassembledquantumdot AT ianmgriffiths fundamentallimitsofelectronandnuclearspinqubitlifetimesinanisolatedselfassembledquantumdot AT gauthamragunathan fundamentallimitsofelectronandnuclearspinqubitlifetimesinanisolatedselfassembledquantumdot AT ataulhaq fundamentallimitsofelectronandnuclearspinqubitlifetimesinanisolatedselfassembledquantumdot AT callummcewan fundamentallimitsofelectronandnuclearspinqubitlifetimesinanisolatedselfassembledquantumdot AT edmundclarke fundamentallimitsofelectronandnuclearspinqubitlifetimesinanisolatedselfassembledquantumdot AT evgenyachekhovich fundamentallimitsofelectronandnuclearspinqubitlifetimesinanisolatedselfassembledquantumdot |
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1718392690682363904 |