Surpassing the single-atom catalytic activity limit through paired Pt-O-Pt ensemble built from isolated Pt1 atoms

Single-atom metal catalysts offer maximized material efficiency, but there is large room to improve the intrinsic activity per metal atom for many reactions. Here, the authors demonstrate that the solution for CO oxidation is to tackle the issue of lacking neighboring Pt atoms in the single-atom Pt1...

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Autores principales:	Hui Wang, Jin-Xun Liu, Lawrence F. Allard, Sungsik Lee, Jilei Liu, Hang Li, Jianqiang Wang, Jun Wang, Se H. Oh, Wei Li, Maria Flytzani-Stephanopoulos, Meiqing Shen, Bryan R. Goldsmith, Ming Yang
Formato:	article
Lenguaje:	EN
Publicado:	Nature Portfolio 2019
Materias:	Science Q
Acceso en línea:	https://doaj.org/article/a33f54bc4a9c461f95ad3d4423c82ee0
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spelling	oai:doaj.org-article:a33f54bc4a9c461f95ad3d4423c82ee02021-12-02T16:57:30ZSurpassing the single-atom catalytic activity limit through paired Pt-O-Pt ensemble built from isolated Pt1 atoms10.1038/s41467-019-11856-92041-1723https://doaj.org/article/a33f54bc4a9c461f95ad3d4423c82ee02019-08-01T00:00:00Zhttps://doi.org/10.1038/s41467-019-11856-9https://doaj.org/toc/2041-1723Single-atom metal catalysts offer maximized material efficiency, but there is large room to improve the intrinsic activity per metal atom for many reactions. Here, the authors demonstrate that the solution for CO oxidation is to tackle the issue of lacking neighboring Pt atoms in the single-atom Pt1/CeO2 system.Hui WangJin-Xun LiuLawrence F. AllardSungsik LeeJilei LiuHang LiJianqiang WangJun WangSe H. OhWei LiMaria Flytzani-StephanopoulosMeiqing ShenBryan R. GoldsmithMing YangNature PortfolioarticleScienceQENNature Communications, Vol 10, Iss 1, Pp 1-12 (2019)
institution	DOAJ
collection	DOAJ
language	EN
topic	Science Q
spellingShingle	Science Q Hui Wang Jin-Xun Liu Lawrence F. Allard Sungsik Lee Jilei Liu Hang Li Jianqiang Wang Jun Wang Se H. Oh Wei Li Maria Flytzani-Stephanopoulos Meiqing Shen Bryan R. Goldsmith Ming Yang Surpassing the single-atom catalytic activity limit through paired Pt-O-Pt ensemble built from isolated Pt1 atoms
description	Single-atom metal catalysts offer maximized material efficiency, but there is large room to improve the intrinsic activity per metal atom for many reactions. Here, the authors demonstrate that the solution for CO oxidation is to tackle the issue of lacking neighboring Pt atoms in the single-atom Pt1/CeO2 system.
format	article
author	Hui Wang Jin-Xun Liu Lawrence F. Allard Sungsik Lee Jilei Liu Hang Li Jianqiang Wang Jun Wang Se H. Oh Wei Li Maria Flytzani-Stephanopoulos Meiqing Shen Bryan R. Goldsmith Ming Yang
author_facet	Hui Wang Jin-Xun Liu Lawrence F. Allard Sungsik Lee Jilei Liu Hang Li Jianqiang Wang Jun Wang Se H. Oh Wei Li Maria Flytzani-Stephanopoulos Meiqing Shen Bryan R. Goldsmith Ming Yang
author_sort	Hui Wang
title	Surpassing the single-atom catalytic activity limit through paired Pt-O-Pt ensemble built from isolated Pt1 atoms
title_short	Surpassing the single-atom catalytic activity limit through paired Pt-O-Pt ensemble built from isolated Pt1 atoms
title_full	Surpassing the single-atom catalytic activity limit through paired Pt-O-Pt ensemble built from isolated Pt1 atoms
title_fullStr	Surpassing the single-atom catalytic activity limit through paired Pt-O-Pt ensemble built from isolated Pt1 atoms
title_full_unstemmed	Surpassing the single-atom catalytic activity limit through paired Pt-O-Pt ensemble built from isolated Pt1 atoms
title_sort	surpassing the single-atom catalytic activity limit through paired pt-o-pt ensemble built from isolated pt1 atoms
publisher	Nature Portfolio
publishDate	2019
url	https://doaj.org/article/a33f54bc4a9c461f95ad3d4423c82ee0
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Surpassing the single-atom catalytic activity limit through paired Pt-O-Pt ensemble built from isolated Pt1 atoms

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