Elucidating the origins of multimode vibrational coherences of polyatomic molecules induced by intense laser fields

Nuclear dynamics of polyatomic molecules involves multiple degrees of freedom and is challenging to explore. Here the authors study the internuclear distance-dependent depletion and bond-softening induced vibrational wavepacket dynamics of CH3I molecules using femtosecond XUV transient absorption sp...

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Autores principales: Zhengrong Wei, Jialin Li, Lin Wang, Soo Teck See, Mark Hyunpong Jhon, Yingfeng Zhang, Fan Shi, Minghui Yang, Zhi-Heng Loh
Formato: article
Lenguaje:EN
Publicado: Nature Portfolio 2017
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Acceso en línea:https://doaj.org/article/a399aba689a448c0b7e85f27323a4c61
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Sumario:Nuclear dynamics of polyatomic molecules involves multiple degrees of freedom and is challenging to explore. Here the authors study the internuclear distance-dependent depletion and bond-softening induced vibrational wavepacket dynamics of CH3I molecules using femtosecond XUV transient absorption spectroscopy.