Fermi Surface Mapping and the Nature of Charge-Density-Wave Order in the Kagome Superconductor CsV_{3}Sb_{5}

The recently discovered family of AV_{3}Sb_{5} (A: K, Rb Cs) kagome metals possess a unique combination of nontrivial band topology, superconducting ground states, and signatures of electron correlations manifest via competing charge density wave order. Little is understood regarding the nature of t...

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Autores principales: Brenden R. Ortiz, Samuel M. L. Teicher, Linus Kautzsch, Paul M. Sarte, Noah Ratcliff, John Harter, Jacob P. C. Ruff, Ram Seshadri, Stephen D. Wilson
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Publicado: American Physical Society 2021
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spelling oai:doaj.org-article:a771c7e3da6c43e2af191981028c4e962021-11-11T15:48:48ZFermi Surface Mapping and the Nature of Charge-Density-Wave Order in the Kagome Superconductor CsV_{3}Sb_{5}10.1103/PhysRevX.11.0410302160-3308https://doaj.org/article/a771c7e3da6c43e2af191981028c4e962021-11-01T00:00:00Zhttp://doi.org/10.1103/PhysRevX.11.041030http://doi.org/10.1103/PhysRevX.11.041030https://doaj.org/toc/2160-3308The recently discovered family of AV_{3}Sb_{5} (A: K, Rb Cs) kagome metals possess a unique combination of nontrivial band topology, superconducting ground states, and signatures of electron correlations manifest via competing charge density wave order. Little is understood regarding the nature of the charge density wave (CDW) instability inherent to these compounds and the potential correlation with the onset of a large anomalous Hall response. To understand the impact of the CDW order on the electronic structure in these systems, we present quantum oscillation measurements on single crystals of CsV_{3}Sb_{5}. Our data provide direct evidence that the CDW invokes a substantial reconstruction of the Fermi surface pockets associated with the vanadium orbitals and the kagome lattice framework. In conjunction with density functional theory modeling, we are able to identify split oscillation frequencies originating from reconstructed pockets built from vanadium orbitals and Dirac-like bands. Complementary diffraction measurements are further able to demonstrate that the CDW instability has a correlated phasing of distortions between neighboring V_{3}Sb_{5} planes, and the average structure in the CDW state is proposed. These results provide critical insights into the underlying CDW instability in AV_{3}Sb_{5} kagome metals and support minimal models of CDW order arising from within the vanadium-based kagome lattice.Brenden R. OrtizSamuel M. L. TeicherLinus KautzschPaul M. SarteNoah RatcliffJohn HarterJacob P. C. RuffRam SeshadriStephen D. WilsonAmerican Physical SocietyarticlePhysicsQC1-999ENPhysical Review X, Vol 11, Iss 4, p 041030 (2021)
institution DOAJ
collection DOAJ
language EN
topic Physics
QC1-999
spellingShingle Physics
QC1-999
Brenden R. Ortiz
Samuel M. L. Teicher
Linus Kautzsch
Paul M. Sarte
Noah Ratcliff
John Harter
Jacob P. C. Ruff
Ram Seshadri
Stephen D. Wilson
Fermi Surface Mapping and the Nature of Charge-Density-Wave Order in the Kagome Superconductor CsV_{3}Sb_{5}
description The recently discovered family of AV_{3}Sb_{5} (A: K, Rb Cs) kagome metals possess a unique combination of nontrivial band topology, superconducting ground states, and signatures of electron correlations manifest via competing charge density wave order. Little is understood regarding the nature of the charge density wave (CDW) instability inherent to these compounds and the potential correlation with the onset of a large anomalous Hall response. To understand the impact of the CDW order on the electronic structure in these systems, we present quantum oscillation measurements on single crystals of CsV_{3}Sb_{5}. Our data provide direct evidence that the CDW invokes a substantial reconstruction of the Fermi surface pockets associated with the vanadium orbitals and the kagome lattice framework. In conjunction with density functional theory modeling, we are able to identify split oscillation frequencies originating from reconstructed pockets built from vanadium orbitals and Dirac-like bands. Complementary diffraction measurements are further able to demonstrate that the CDW instability has a correlated phasing of distortions between neighboring V_{3}Sb_{5} planes, and the average structure in the CDW state is proposed. These results provide critical insights into the underlying CDW instability in AV_{3}Sb_{5} kagome metals and support minimal models of CDW order arising from within the vanadium-based kagome lattice.
format article
author Brenden R. Ortiz
Samuel M. L. Teicher
Linus Kautzsch
Paul M. Sarte
Noah Ratcliff
John Harter
Jacob P. C. Ruff
Ram Seshadri
Stephen D. Wilson
author_facet Brenden R. Ortiz
Samuel M. L. Teicher
Linus Kautzsch
Paul M. Sarte
Noah Ratcliff
John Harter
Jacob P. C. Ruff
Ram Seshadri
Stephen D. Wilson
author_sort Brenden R. Ortiz
title Fermi Surface Mapping and the Nature of Charge-Density-Wave Order in the Kagome Superconductor CsV_{3}Sb_{5}
title_short Fermi Surface Mapping and the Nature of Charge-Density-Wave Order in the Kagome Superconductor CsV_{3}Sb_{5}
title_full Fermi Surface Mapping and the Nature of Charge-Density-Wave Order in the Kagome Superconductor CsV_{3}Sb_{5}
title_fullStr Fermi Surface Mapping and the Nature of Charge-Density-Wave Order in the Kagome Superconductor CsV_{3}Sb_{5}
title_full_unstemmed Fermi Surface Mapping and the Nature of Charge-Density-Wave Order in the Kagome Superconductor CsV_{3}Sb_{5}
title_sort fermi surface mapping and the nature of charge-density-wave order in the kagome superconductor csv_{3}sb_{5}
publisher American Physical Society
publishDate 2021
url https://doaj.org/article/a771c7e3da6c43e2af191981028c4e96
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