Coupling between intra- and intermolecular motions in liquid water revealed by two-dimensional terahertz-infrared-visible spectroscopy
Liquid water molecules are in constant vibrational motion, but probing how their local behaviour influences collective dynamics remains a challenge. Here, the authors present terahertz-infrared spectroscopy to elucidate coupling of the O-H stretch vibration to collective, delocalized intermolecular...
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Nature Portfolio
2018
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oai:doaj.org-article:a78e161c491a48998225c364832c75192021-12-02T15:34:06ZCoupling between intra- and intermolecular motions in liquid water revealed by two-dimensional terahertz-infrared-visible spectroscopy10.1038/s41467-018-03303-y2041-1723https://doaj.org/article/a78e161c491a48998225c364832c75192018-02-01T00:00:00Zhttps://doi.org/10.1038/s41467-018-03303-yhttps://doaj.org/toc/2041-1723Liquid water molecules are in constant vibrational motion, but probing how their local behaviour influences collective dynamics remains a challenge. Here, the authors present terahertz-infrared spectroscopy to elucidate coupling of the O-H stretch vibration to collective, delocalized intermolecular modes.Maksim GrechkoTaisuke HasegawaFrancesco D’AngeloHironobu ItoDmitry TurchinovichYuki NagataMischa BonnNature PortfolioarticleScienceQENNature Communications, Vol 9, Iss 1, Pp 1-8 (2018) |
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Science Q Maksim Grechko Taisuke Hasegawa Francesco D’Angelo Hironobu Ito Dmitry Turchinovich Yuki Nagata Mischa Bonn Coupling between intra- and intermolecular motions in liquid water revealed by two-dimensional terahertz-infrared-visible spectroscopy |
description |
Liquid water molecules are in constant vibrational motion, but probing how their local behaviour influences collective dynamics remains a challenge. Here, the authors present terahertz-infrared spectroscopy to elucidate coupling of the O-H stretch vibration to collective, delocalized intermolecular modes. |
format |
article |
author |
Maksim Grechko Taisuke Hasegawa Francesco D’Angelo Hironobu Ito Dmitry Turchinovich Yuki Nagata Mischa Bonn |
author_facet |
Maksim Grechko Taisuke Hasegawa Francesco D’Angelo Hironobu Ito Dmitry Turchinovich Yuki Nagata Mischa Bonn |
author_sort |
Maksim Grechko |
title |
Coupling between intra- and intermolecular motions in liquid water revealed by two-dimensional terahertz-infrared-visible spectroscopy |
title_short |
Coupling between intra- and intermolecular motions in liquid water revealed by two-dimensional terahertz-infrared-visible spectroscopy |
title_full |
Coupling between intra- and intermolecular motions in liquid water revealed by two-dimensional terahertz-infrared-visible spectroscopy |
title_fullStr |
Coupling between intra- and intermolecular motions in liquid water revealed by two-dimensional terahertz-infrared-visible spectroscopy |
title_full_unstemmed |
Coupling between intra- and intermolecular motions in liquid water revealed by two-dimensional terahertz-infrared-visible spectroscopy |
title_sort |
coupling between intra- and intermolecular motions in liquid water revealed by two-dimensional terahertz-infrared-visible spectroscopy |
publisher |
Nature Portfolio |
publishDate |
2018 |
url |
https://doaj.org/article/a78e161c491a48998225c364832c7519 |
work_keys_str_mv |
AT maksimgrechko couplingbetweenintraandintermolecularmotionsinliquidwaterrevealedbytwodimensionalterahertzinfraredvisiblespectroscopy AT taisukehasegawa couplingbetweenintraandintermolecularmotionsinliquidwaterrevealedbytwodimensionalterahertzinfraredvisiblespectroscopy AT francescodangelo couplingbetweenintraandintermolecularmotionsinliquidwaterrevealedbytwodimensionalterahertzinfraredvisiblespectroscopy AT hironobuito couplingbetweenintraandintermolecularmotionsinliquidwaterrevealedbytwodimensionalterahertzinfraredvisiblespectroscopy AT dmitryturchinovich couplingbetweenintraandintermolecularmotionsinliquidwaterrevealedbytwodimensionalterahertzinfraredvisiblespectroscopy AT yukinagata couplingbetweenintraandintermolecularmotionsinliquidwaterrevealedbytwodimensionalterahertzinfraredvisiblespectroscopy AT mischabonn couplingbetweenintraandintermolecularmotionsinliquidwaterrevealedbytwodimensionalterahertzinfraredvisiblespectroscopy |
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1718386920401141760 |