Coupling between intra- and intermolecular motions in liquid water revealed by two-dimensional terahertz-infrared-visible spectroscopy

Liquid water molecules are in constant vibrational motion, but probing how their local behaviour influences collective dynamics remains a challenge. Here, the authors present terahertz-infrared spectroscopy to elucidate coupling of the O-H stretch vibration to collective, delocalized intermolecular...

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Autores principales: Maksim Grechko, Taisuke Hasegawa, Francesco D’Angelo, Hironobu Ito, Dmitry Turchinovich, Yuki Nagata, Mischa Bonn
Formato: article
Lenguaje:EN
Publicado: Nature Portfolio 2018
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Acceso en línea:https://doaj.org/article/a78e161c491a48998225c364832c7519
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spelling oai:doaj.org-article:a78e161c491a48998225c364832c75192021-12-02T15:34:06ZCoupling between intra- and intermolecular motions in liquid water revealed by two-dimensional terahertz-infrared-visible spectroscopy10.1038/s41467-018-03303-y2041-1723https://doaj.org/article/a78e161c491a48998225c364832c75192018-02-01T00:00:00Zhttps://doi.org/10.1038/s41467-018-03303-yhttps://doaj.org/toc/2041-1723Liquid water molecules are in constant vibrational motion, but probing how their local behaviour influences collective dynamics remains a challenge. Here, the authors present terahertz-infrared spectroscopy to elucidate coupling of the O-H stretch vibration to collective, delocalized intermolecular modes.Maksim GrechkoTaisuke HasegawaFrancesco D’AngeloHironobu ItoDmitry TurchinovichYuki NagataMischa BonnNature PortfolioarticleScienceQENNature Communications, Vol 9, Iss 1, Pp 1-8 (2018)
institution DOAJ
collection DOAJ
language EN
topic Science
Q
spellingShingle Science
Q
Maksim Grechko
Taisuke Hasegawa
Francesco D’Angelo
Hironobu Ito
Dmitry Turchinovich
Yuki Nagata
Mischa Bonn
Coupling between intra- and intermolecular motions in liquid water revealed by two-dimensional terahertz-infrared-visible spectroscopy
description Liquid water molecules are in constant vibrational motion, but probing how their local behaviour influences collective dynamics remains a challenge. Here, the authors present terahertz-infrared spectroscopy to elucidate coupling of the O-H stretch vibration to collective, delocalized intermolecular modes.
format article
author Maksim Grechko
Taisuke Hasegawa
Francesco D’Angelo
Hironobu Ito
Dmitry Turchinovich
Yuki Nagata
Mischa Bonn
author_facet Maksim Grechko
Taisuke Hasegawa
Francesco D’Angelo
Hironobu Ito
Dmitry Turchinovich
Yuki Nagata
Mischa Bonn
author_sort Maksim Grechko
title Coupling between intra- and intermolecular motions in liquid water revealed by two-dimensional terahertz-infrared-visible spectroscopy
title_short Coupling between intra- and intermolecular motions in liquid water revealed by two-dimensional terahertz-infrared-visible spectroscopy
title_full Coupling between intra- and intermolecular motions in liquid water revealed by two-dimensional terahertz-infrared-visible spectroscopy
title_fullStr Coupling between intra- and intermolecular motions in liquid water revealed by two-dimensional terahertz-infrared-visible spectroscopy
title_full_unstemmed Coupling between intra- and intermolecular motions in liquid water revealed by two-dimensional terahertz-infrared-visible spectroscopy
title_sort coupling between intra- and intermolecular motions in liquid water revealed by two-dimensional terahertz-infrared-visible spectroscopy
publisher Nature Portfolio
publishDate 2018
url https://doaj.org/article/a78e161c491a48998225c364832c7519
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