Enhanced methanol production by two-stage reaction of CO2 hydrogenation at atmospheric pressure
Methanol can be produced from CO2 hydrogenation. CO2 was hydrogenated to CH3OH in one-stage reaction at atmospheric pressure. The result was highly selective to CH3OH but insufficient conversion of CO2 using Cu/Zn/Al2O3. A two-stage reaction was carried out with high and low temperatures, respective...
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2022
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oai:doaj.org-article:ab03302cc57a460f8af799aeee6de8b82021-11-28T04:29:21ZEnhanced methanol production by two-stage reaction of CO2 hydrogenation at atmospheric pressure1873-390510.1016/j.catcom.2021.106373https://doaj.org/article/ab03302cc57a460f8af799aeee6de8b82022-02-01T00:00:00Zhttp://www.sciencedirect.com/science/article/pii/S1566736721000960https://doaj.org/toc/1873-3905Methanol can be produced from CO2 hydrogenation. CO2 was hydrogenated to CH3OH in one-stage reaction at atmospheric pressure. The result was highly selective to CH3OH but insufficient conversion of CO2 using Cu/Zn/Al2O3. A two-stage reaction was carried out with high and low temperatures, respectively. CO2 was hydrogenated to carbon monoxide (CO) and H2O in the first-stage at high temperatures. Subsequently, after removing H2O, CO was further hydrogenated to CH3OH in the second-stage at low temperatures. The CH3OH yield was 3.4 times higher than that of single-stage reaction. This concept achieves CO2 hydrogenation towards more CH3OH production.Ya-Ning YangChao-Wei HuangVan-Huy NguyenJeffrey C.-S. WuElsevierarticleCarbon dioxideCarbon monoxideHydrogenationMethanolTwo-stage reactionChemistryQD1-999ENCatalysis Communications, Vol 162, Iss , Pp 106373- (2022) |
institution |
DOAJ |
collection |
DOAJ |
language |
EN |
topic |
Carbon dioxide Carbon monoxide Hydrogenation Methanol Two-stage reaction Chemistry QD1-999 |
spellingShingle |
Carbon dioxide Carbon monoxide Hydrogenation Methanol Two-stage reaction Chemistry QD1-999 Ya-Ning Yang Chao-Wei Huang Van-Huy Nguyen Jeffrey C.-S. Wu Enhanced methanol production by two-stage reaction of CO2 hydrogenation at atmospheric pressure |
description |
Methanol can be produced from CO2 hydrogenation. CO2 was hydrogenated to CH3OH in one-stage reaction at atmospheric pressure. The result was highly selective to CH3OH but insufficient conversion of CO2 using Cu/Zn/Al2O3. A two-stage reaction was carried out with high and low temperatures, respectively. CO2 was hydrogenated to carbon monoxide (CO) and H2O in the first-stage at high temperatures. Subsequently, after removing H2O, CO was further hydrogenated to CH3OH in the second-stage at low temperatures. The CH3OH yield was 3.4 times higher than that of single-stage reaction. This concept achieves CO2 hydrogenation towards more CH3OH production. |
format |
article |
author |
Ya-Ning Yang Chao-Wei Huang Van-Huy Nguyen Jeffrey C.-S. Wu |
author_facet |
Ya-Ning Yang Chao-Wei Huang Van-Huy Nguyen Jeffrey C.-S. Wu |
author_sort |
Ya-Ning Yang |
title |
Enhanced methanol production by two-stage reaction of CO2 hydrogenation at atmospheric pressure |
title_short |
Enhanced methanol production by two-stage reaction of CO2 hydrogenation at atmospheric pressure |
title_full |
Enhanced methanol production by two-stage reaction of CO2 hydrogenation at atmospheric pressure |
title_fullStr |
Enhanced methanol production by two-stage reaction of CO2 hydrogenation at atmospheric pressure |
title_full_unstemmed |
Enhanced methanol production by two-stage reaction of CO2 hydrogenation at atmospheric pressure |
title_sort |
enhanced methanol production by two-stage reaction of co2 hydrogenation at atmospheric pressure |
publisher |
Elsevier |
publishDate |
2022 |
url |
https://doaj.org/article/ab03302cc57a460f8af799aeee6de8b8 |
work_keys_str_mv |
AT yaningyang enhancedmethanolproductionbytwostagereactionofco2hydrogenationatatmosphericpressure AT chaoweihuang enhancedmethanolproductionbytwostagereactionofco2hydrogenationatatmosphericpressure AT vanhuynguyen enhancedmethanolproductionbytwostagereactionofco2hydrogenationatatmosphericpressure AT jeffreycswu enhancedmethanolproductionbytwostagereactionofco2hydrogenationatatmosphericpressure |
_version_ |
1718408398688485376 |