Enhanced methanol production by two-stage reaction of CO2 hydrogenation at atmospheric pressure

Methanol can be produced from CO2 hydrogenation. CO2 was hydrogenated to CH3OH in one-stage reaction at atmospheric pressure. The result was highly selective to CH3OH but insufficient conversion of CO2 using Cu/Zn/Al2O3. A two-stage reaction was carried out with high and low temperatures, respective...

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Autores principales: Ya-Ning Yang, Chao-Wei Huang, Van-Huy Nguyen, Jeffrey C.-S. Wu
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Lenguaje:EN
Publicado: Elsevier 2022
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Acceso en línea:https://doaj.org/article/ab03302cc57a460f8af799aeee6de8b8
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spelling oai:doaj.org-article:ab03302cc57a460f8af799aeee6de8b82021-11-28T04:29:21ZEnhanced methanol production by two-stage reaction of CO2 hydrogenation at atmospheric pressure1873-390510.1016/j.catcom.2021.106373https://doaj.org/article/ab03302cc57a460f8af799aeee6de8b82022-02-01T00:00:00Zhttp://www.sciencedirect.com/science/article/pii/S1566736721000960https://doaj.org/toc/1873-3905Methanol can be produced from CO2 hydrogenation. CO2 was hydrogenated to CH3OH in one-stage reaction at atmospheric pressure. The result was highly selective to CH3OH but insufficient conversion of CO2 using Cu/Zn/Al2O3. A two-stage reaction was carried out with high and low temperatures, respectively. CO2 was hydrogenated to carbon monoxide (CO) and H2O in the first-stage at high temperatures. Subsequently, after removing H2O, CO was further hydrogenated to CH3OH in the second-stage at low temperatures. The CH3OH yield was 3.4 times higher than that of single-stage reaction. This concept achieves CO2 hydrogenation towards more CH3OH production.Ya-Ning YangChao-Wei HuangVan-Huy NguyenJeffrey C.-S. WuElsevierarticleCarbon dioxideCarbon monoxideHydrogenationMethanolTwo-stage reactionChemistryQD1-999ENCatalysis Communications, Vol 162, Iss , Pp 106373- (2022)
institution DOAJ
collection DOAJ
language EN
topic Carbon dioxide
Carbon monoxide
Hydrogenation
Methanol
Two-stage reaction
Chemistry
QD1-999
spellingShingle Carbon dioxide
Carbon monoxide
Hydrogenation
Methanol
Two-stage reaction
Chemistry
QD1-999
Ya-Ning Yang
Chao-Wei Huang
Van-Huy Nguyen
Jeffrey C.-S. Wu
Enhanced methanol production by two-stage reaction of CO2 hydrogenation at atmospheric pressure
description Methanol can be produced from CO2 hydrogenation. CO2 was hydrogenated to CH3OH in one-stage reaction at atmospheric pressure. The result was highly selective to CH3OH but insufficient conversion of CO2 using Cu/Zn/Al2O3. A two-stage reaction was carried out with high and low temperatures, respectively. CO2 was hydrogenated to carbon monoxide (CO) and H2O in the first-stage at high temperatures. Subsequently, after removing H2O, CO was further hydrogenated to CH3OH in the second-stage at low temperatures. The CH3OH yield was 3.4 times higher than that of single-stage reaction. This concept achieves CO2 hydrogenation towards more CH3OH production.
format article
author Ya-Ning Yang
Chao-Wei Huang
Van-Huy Nguyen
Jeffrey C.-S. Wu
author_facet Ya-Ning Yang
Chao-Wei Huang
Van-Huy Nguyen
Jeffrey C.-S. Wu
author_sort Ya-Ning Yang
title Enhanced methanol production by two-stage reaction of CO2 hydrogenation at atmospheric pressure
title_short Enhanced methanol production by two-stage reaction of CO2 hydrogenation at atmospheric pressure
title_full Enhanced methanol production by two-stage reaction of CO2 hydrogenation at atmospheric pressure
title_fullStr Enhanced methanol production by two-stage reaction of CO2 hydrogenation at atmospheric pressure
title_full_unstemmed Enhanced methanol production by two-stage reaction of CO2 hydrogenation at atmospheric pressure
title_sort enhanced methanol production by two-stage reaction of co2 hydrogenation at atmospheric pressure
publisher Elsevier
publishDate 2022
url https://doaj.org/article/ab03302cc57a460f8af799aeee6de8b8
work_keys_str_mv AT yaningyang enhancedmethanolproductionbytwostagereactionofco2hydrogenationatatmosphericpressure
AT chaoweihuang enhancedmethanolproductionbytwostagereactionofco2hydrogenationatatmosphericpressure
AT vanhuynguyen enhancedmethanolproductionbytwostagereactionofco2hydrogenationatatmosphericpressure
AT jeffreycswu enhancedmethanolproductionbytwostagereactionofco2hydrogenationatatmosphericpressure
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