Electron correlation driven non-adiabatic relaxation in molecules excited by an ultrashort extreme ultraviolet pulse

The many-body quantum nature of molecules determines their static and dynamic properties, but remains the main obstacle in their accurate description. Here, the authors employ ultrafast spectroscopic methods to explore the dynamics of highly excited organic molecules, revealing many-body effects and...

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Auteurs principaux: A. Marciniak, V. Despré, V. Loriot, G. Karras, M. Hervé, L. Quintard, F. Catoire, C. Joblin, E. Constant, A. I. Kuleff, F. Lépine
Format: article
Langue:EN
Publié: Nature Portfolio 2019
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Accès en ligne:https://doaj.org/article/ac2461ded8d541e4b63c4452f4b18c12
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Résumé:The many-body quantum nature of molecules determines their static and dynamic properties, but remains the main obstacle in their accurate description. Here, the authors employ ultrafast spectroscopic methods to explore the dynamics of highly excited organic molecules, revealing many-body effects and hints of coherent vibronic dynamics which persist despite their molecular complexity.