Controlling plasmon-exciton interactions through photothermal reshaping

We investigated the plasmon-exciton interactions in an individual gold nanorod (GNR) with monolayer MoS2 at room temperature with the single-particle spectroscopy technique. To control the plasmon-exciton interaction, we tuned the local surface plasmon resonance of an individual GNR in-situ by emplo...

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Autores principales: Hu Aiqin, Liu Shuai, Zhao Jingyi, Wen Te, Zhang Weidong, Gong Qihuang, Meng Yongqiang, Ye Yu, Lu Guowei
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Publicado: Institue of Optics and Electronics, Chinese Academy of Sciences 2020
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Acceso en línea:https://doaj.org/article/adb3655fad8442979896eb860da7463f
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spelling oai:doaj.org-article:adb3655fad8442979896eb860da7463f2021-11-10T10:13:15ZControlling plasmon-exciton interactions through photothermal reshaping2096-457910.29026/oea.2020.190017https://doaj.org/article/adb3655fad8442979896eb860da7463f2020-01-01T00:00:00Zhttp://www.oejournal.org/article/doi/10.29026/oea.2020.190017https://doaj.org/toc/2096-4579We investigated the plasmon-exciton interactions in an individual gold nanorod (GNR) with monolayer MoS2 at room temperature with the single-particle spectroscopy technique. To control the plasmon-exciton interaction, we tuned the local surface plasmon resonance of an individual GNR in-situ by employing the photothermal reshaping effect. The scattering spectra of the GNR-MoS2 hybrids exhibited two dips at the frequencies of the A and B excitons of monolayer MoS2, which were caused by the plasmon-induced resonance energy transfer effect. The resonance energy transfer rate increased when the surface plasmon resonance of the nanorod matched well with the exciton transition energy. Also, we demonstrated that the plasmon-enhanced fluorescence process dominated the photoluminescence of the GNR-MoS2 hybrid. These results provide a flexible way to control the plasmon-exciton interaction in an all-solid-state operating system at room temperature.Hu AiqinLiu ShuaiZhao JingyiWen TeZhang WeidongGong QihuangMeng YongqiangYe YuLu GuoweiInstitue of Optics and Electronics, Chinese Academy of Sciencesarticlegold nanorodmos2hybridscatteringphotoluminescencesingle nanoparticleOptics. LightQC350-467ENOpto-Electronic Advances, Vol 3, Iss 1, Pp 190017-1-190017-8 (2020)
institution DOAJ
collection DOAJ
language EN
topic gold nanorod
mos2
hybrid
scattering
photoluminescence
single nanoparticle
Optics. Light
QC350-467
spellingShingle gold nanorod
mos2
hybrid
scattering
photoluminescence
single nanoparticle
Optics. Light
QC350-467
Hu Aiqin
Liu Shuai
Zhao Jingyi
Wen Te
Zhang Weidong
Gong Qihuang
Meng Yongqiang
Ye Yu
Lu Guowei
Controlling plasmon-exciton interactions through photothermal reshaping
description We investigated the plasmon-exciton interactions in an individual gold nanorod (GNR) with monolayer MoS2 at room temperature with the single-particle spectroscopy technique. To control the plasmon-exciton interaction, we tuned the local surface plasmon resonance of an individual GNR in-situ by employing the photothermal reshaping effect. The scattering spectra of the GNR-MoS2 hybrids exhibited two dips at the frequencies of the A and B excitons of monolayer MoS2, which were caused by the plasmon-induced resonance energy transfer effect. The resonance energy transfer rate increased when the surface plasmon resonance of the nanorod matched well with the exciton transition energy. Also, we demonstrated that the plasmon-enhanced fluorescence process dominated the photoluminescence of the GNR-MoS2 hybrid. These results provide a flexible way to control the plasmon-exciton interaction in an all-solid-state operating system at room temperature.
format article
author Hu Aiqin
Liu Shuai
Zhao Jingyi
Wen Te
Zhang Weidong
Gong Qihuang
Meng Yongqiang
Ye Yu
Lu Guowei
author_facet Hu Aiqin
Liu Shuai
Zhao Jingyi
Wen Te
Zhang Weidong
Gong Qihuang
Meng Yongqiang
Ye Yu
Lu Guowei
author_sort Hu Aiqin
title Controlling plasmon-exciton interactions through photothermal reshaping
title_short Controlling plasmon-exciton interactions through photothermal reshaping
title_full Controlling plasmon-exciton interactions through photothermal reshaping
title_fullStr Controlling plasmon-exciton interactions through photothermal reshaping
title_full_unstemmed Controlling plasmon-exciton interactions through photothermal reshaping
title_sort controlling plasmon-exciton interactions through photothermal reshaping
publisher Institue of Optics and Electronics, Chinese Academy of Sciences
publishDate 2020
url https://doaj.org/article/adb3655fad8442979896eb860da7463f
work_keys_str_mv AT huaiqin controllingplasmonexcitoninteractionsthroughphotothermalreshaping
AT liushuai controllingplasmonexcitoninteractionsthroughphotothermalreshaping
AT zhaojingyi controllingplasmonexcitoninteractionsthroughphotothermalreshaping
AT wente controllingplasmonexcitoninteractionsthroughphotothermalreshaping
AT zhangweidong controllingplasmonexcitoninteractionsthroughphotothermalreshaping
AT gongqihuang controllingplasmonexcitoninteractionsthroughphotothermalreshaping
AT mengyongqiang controllingplasmonexcitoninteractionsthroughphotothermalreshaping
AT yeyu controllingplasmonexcitoninteractionsthroughphotothermalreshaping
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