Facile Synthesis of MgO-Modified Carbon Adsorbents with Microwave- Assisted Methods: Effect of MgO Particles and Porosities on CO2 Capture
Abstract In this study, magnesium oxide (MgO)-modified carbon adsorbents were fabricated using a nitrogen-enriched carbon precursor by microwave-assisted irradiation for CO2 capture. The X-ray diffraction (XRD) patterns showed the characteristic diffraction peaks of MgO at 43° and 62.5°, and no impu...
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2017
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oai:doaj.org-article:af7f439a95de436ea7ed052aac8a13042021-12-02T12:32:01ZFacile Synthesis of MgO-Modified Carbon Adsorbents with Microwave- Assisted Methods: Effect of MgO Particles and Porosities on CO2 Capture10.1038/s41598-017-06091-52045-2322https://doaj.org/article/af7f439a95de436ea7ed052aac8a13042017-07-01T00:00:00Zhttps://doi.org/10.1038/s41598-017-06091-5https://doaj.org/toc/2045-2322Abstract In this study, magnesium oxide (MgO)-modified carbon adsorbents were fabricated using a nitrogen-enriched carbon precursor by microwave-assisted irradiation for CO2 capture. The X-ray diffraction (XRD) patterns showed the characteristic diffraction peaks of MgO at 43° and 62.5°, and no impurities were apparent. By changing the microwave reaction time, the spherical structure of the parent material was transformed to a hybrid structure with MgO crystalline particles in a carbon matrix. The morphology evolution and properties of the prepared materials were also investigated using transmission electron microscopy and N2 adsorption, respectively. On optimising the conditions, the prepared sample attained a high CO2 uptake of 1.22 mmol/g (5.3 wt.%) under flue gas conditions (15% CO2 in N2). It was found that MgO affected the CO2 capture behaviour by enhancing the fundamental characteristics of the carbon surfaces.Young-Jung HeoSoo-Jin ParkNature PortfolioarticleMedicineRScienceQENScientific Reports, Vol 7, Iss 1, Pp 1-9 (2017) |
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Medicine R Science Q Young-Jung Heo Soo-Jin Park Facile Synthesis of MgO-Modified Carbon Adsorbents with Microwave- Assisted Methods: Effect of MgO Particles and Porosities on CO2 Capture |
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Abstract In this study, magnesium oxide (MgO)-modified carbon adsorbents were fabricated using a nitrogen-enriched carbon precursor by microwave-assisted irradiation for CO2 capture. The X-ray diffraction (XRD) patterns showed the characteristic diffraction peaks of MgO at 43° and 62.5°, and no impurities were apparent. By changing the microwave reaction time, the spherical structure of the parent material was transformed to a hybrid structure with MgO crystalline particles in a carbon matrix. The morphology evolution and properties of the prepared materials were also investigated using transmission electron microscopy and N2 adsorption, respectively. On optimising the conditions, the prepared sample attained a high CO2 uptake of 1.22 mmol/g (5.3 wt.%) under flue gas conditions (15% CO2 in N2). It was found that MgO affected the CO2 capture behaviour by enhancing the fundamental characteristics of the carbon surfaces. |
format |
article |
author |
Young-Jung Heo Soo-Jin Park |
author_facet |
Young-Jung Heo Soo-Jin Park |
author_sort |
Young-Jung Heo |
title |
Facile Synthesis of MgO-Modified Carbon Adsorbents with Microwave- Assisted Methods: Effect of MgO Particles and Porosities on CO2 Capture |
title_short |
Facile Synthesis of MgO-Modified Carbon Adsorbents with Microwave- Assisted Methods: Effect of MgO Particles and Porosities on CO2 Capture |
title_full |
Facile Synthesis of MgO-Modified Carbon Adsorbents with Microwave- Assisted Methods: Effect of MgO Particles and Porosities on CO2 Capture |
title_fullStr |
Facile Synthesis of MgO-Modified Carbon Adsorbents with Microwave- Assisted Methods: Effect of MgO Particles and Porosities on CO2 Capture |
title_full_unstemmed |
Facile Synthesis of MgO-Modified Carbon Adsorbents with Microwave- Assisted Methods: Effect of MgO Particles and Porosities on CO2 Capture |
title_sort |
facile synthesis of mgo-modified carbon adsorbents with microwave- assisted methods: effect of mgo particles and porosities on co2 capture |
publisher |
Nature Portfolio |
publishDate |
2017 |
url |
https://doaj.org/article/af7f439a95de436ea7ed052aac8a1304 |
work_keys_str_mv |
AT youngjungheo facilesynthesisofmgomodifiedcarbonadsorbentswithmicrowaveassistedmethodseffectofmgoparticlesandporositiesonco2capture AT soojinpark facilesynthesisofmgomodifiedcarbonadsorbentswithmicrowaveassistedmethodseffectofmgoparticlesandporositiesonco2capture |
_version_ |
1718394235093254144 |