Facile Synthesis of MgO-Modified Carbon Adsorbents with Microwave- Assisted Methods: Effect of MgO Particles and Porosities on CO2 Capture

Abstract In this study, magnesium oxide (MgO)-modified carbon adsorbents were fabricated using a nitrogen-enriched carbon precursor by microwave-assisted irradiation for CO2 capture. The X-ray diffraction (XRD) patterns showed the characteristic diffraction peaks of MgO at 43° and 62.5°, and no impu...

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Autores principales: Young-Jung Heo, Soo-Jin Park
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Publicado: Nature Portfolio 2017
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Acceso en línea:https://doaj.org/article/af7f439a95de436ea7ed052aac8a1304
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spelling oai:doaj.org-article:af7f439a95de436ea7ed052aac8a13042021-12-02T12:32:01ZFacile Synthesis of MgO-Modified Carbon Adsorbents with Microwave- Assisted Methods: Effect of MgO Particles and Porosities on CO2 Capture10.1038/s41598-017-06091-52045-2322https://doaj.org/article/af7f439a95de436ea7ed052aac8a13042017-07-01T00:00:00Zhttps://doi.org/10.1038/s41598-017-06091-5https://doaj.org/toc/2045-2322Abstract In this study, magnesium oxide (MgO)-modified carbon adsorbents were fabricated using a nitrogen-enriched carbon precursor by microwave-assisted irradiation for CO2 capture. The X-ray diffraction (XRD) patterns showed the characteristic diffraction peaks of MgO at 43° and 62.5°, and no impurities were apparent. By changing the microwave reaction time, the spherical structure of the parent material was transformed to a hybrid structure with MgO crystalline particles in a carbon matrix. The morphology evolution and properties of the prepared materials were also investigated using transmission electron microscopy and N2 adsorption, respectively. On optimising the conditions, the prepared sample attained a high CO2 uptake of 1.22 mmol/g (5.3 wt.%) under flue gas conditions (15% CO2 in N2). It was found that MgO affected the CO2 capture behaviour by enhancing the fundamental characteristics of the carbon surfaces.Young-Jung HeoSoo-Jin ParkNature PortfolioarticleMedicineRScienceQENScientific Reports, Vol 7, Iss 1, Pp 1-9 (2017)
institution DOAJ
collection DOAJ
language EN
topic Medicine
R
Science
Q
spellingShingle Medicine
R
Science
Q
Young-Jung Heo
Soo-Jin Park
Facile Synthesis of MgO-Modified Carbon Adsorbents with Microwave- Assisted Methods: Effect of MgO Particles and Porosities on CO2 Capture
description Abstract In this study, magnesium oxide (MgO)-modified carbon adsorbents were fabricated using a nitrogen-enriched carbon precursor by microwave-assisted irradiation for CO2 capture. The X-ray diffraction (XRD) patterns showed the characteristic diffraction peaks of MgO at 43° and 62.5°, and no impurities were apparent. By changing the microwave reaction time, the spherical structure of the parent material was transformed to a hybrid structure with MgO crystalline particles in a carbon matrix. The morphology evolution and properties of the prepared materials were also investigated using transmission electron microscopy and N2 adsorption, respectively. On optimising the conditions, the prepared sample attained a high CO2 uptake of 1.22 mmol/g (5.3 wt.%) under flue gas conditions (15% CO2 in N2). It was found that MgO affected the CO2 capture behaviour by enhancing the fundamental characteristics of the carbon surfaces.
format article
author Young-Jung Heo
Soo-Jin Park
author_facet Young-Jung Heo
Soo-Jin Park
author_sort Young-Jung Heo
title Facile Synthesis of MgO-Modified Carbon Adsorbents with Microwave- Assisted Methods: Effect of MgO Particles and Porosities on CO2 Capture
title_short Facile Synthesis of MgO-Modified Carbon Adsorbents with Microwave- Assisted Methods: Effect of MgO Particles and Porosities on CO2 Capture
title_full Facile Synthesis of MgO-Modified Carbon Adsorbents with Microwave- Assisted Methods: Effect of MgO Particles and Porosities on CO2 Capture
title_fullStr Facile Synthesis of MgO-Modified Carbon Adsorbents with Microwave- Assisted Methods: Effect of MgO Particles and Porosities on CO2 Capture
title_full_unstemmed Facile Synthesis of MgO-Modified Carbon Adsorbents with Microwave- Assisted Methods: Effect of MgO Particles and Porosities on CO2 Capture
title_sort facile synthesis of mgo-modified carbon adsorbents with microwave- assisted methods: effect of mgo particles and porosities on co2 capture
publisher Nature Portfolio
publishDate 2017
url https://doaj.org/article/af7f439a95de436ea7ed052aac8a1304
work_keys_str_mv AT youngjungheo facilesynthesisofmgomodifiedcarbonadsorbentswithmicrowaveassistedmethodseffectofmgoparticlesandporositiesonco2capture
AT soojinpark facilesynthesisofmgomodifiedcarbonadsorbentswithmicrowaveassistedmethodseffectofmgoparticlesandporositiesonco2capture
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