Correlating advanced microscopies reveals atomic-scale mechanisms limiting lithium-ion battery lifetime
The longevity of a lithium-ion battery is limited by cathode degradation. Combining atom probe tomography and scanning transmission electron microscopy reveals that the degradation results from atomic-scale irreversible structural changes once lithium leaves the cathode during charging, thereby inhi...
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Nature Portfolio
2021
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oai:doaj.org-article:b007b0f9e0ab413ab1ab3015666f115e2021-12-02T16:04:21ZCorrelating advanced microscopies reveals atomic-scale mechanisms limiting lithium-ion battery lifetime10.1038/s41467-021-24121-92041-1723https://doaj.org/article/b007b0f9e0ab413ab1ab3015666f115e2021-06-01T00:00:00Zhttps://doi.org/10.1038/s41467-021-24121-9https://doaj.org/toc/2041-1723The longevity of a lithium-ion battery is limited by cathode degradation. Combining atom probe tomography and scanning transmission electron microscopy reveals that the degradation results from atomic-scale irreversible structural changes once lithium leaves the cathode during charging, thereby inhibiting lithium intercalation back into the cathode as the battery discharges. This information unveils possible routes for improving the lifetime of lithium-ion batteries.Baptiste GaultJonathan D. PoplawskyNature PortfolioarticleScienceQENNature Communications, Vol 12, Iss 1, Pp 1-3 (2021) |
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Science Q Baptiste Gault Jonathan D. Poplawsky Correlating advanced microscopies reveals atomic-scale mechanisms limiting lithium-ion battery lifetime |
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The longevity of a lithium-ion battery is limited by cathode degradation. Combining atom probe tomography and scanning transmission electron microscopy reveals that the degradation results from atomic-scale irreversible structural changes once lithium leaves the cathode during charging, thereby inhibiting lithium intercalation back into the cathode as the battery discharges. This information unveils possible routes for improving the lifetime of lithium-ion batteries. |
format |
article |
author |
Baptiste Gault Jonathan D. Poplawsky |
author_facet |
Baptiste Gault Jonathan D. Poplawsky |
author_sort |
Baptiste Gault |
title |
Correlating advanced microscopies reveals atomic-scale mechanisms limiting lithium-ion battery lifetime |
title_short |
Correlating advanced microscopies reveals atomic-scale mechanisms limiting lithium-ion battery lifetime |
title_full |
Correlating advanced microscopies reveals atomic-scale mechanisms limiting lithium-ion battery lifetime |
title_fullStr |
Correlating advanced microscopies reveals atomic-scale mechanisms limiting lithium-ion battery lifetime |
title_full_unstemmed |
Correlating advanced microscopies reveals atomic-scale mechanisms limiting lithium-ion battery lifetime |
title_sort |
correlating advanced microscopies reveals atomic-scale mechanisms limiting lithium-ion battery lifetime |
publisher |
Nature Portfolio |
publishDate |
2021 |
url |
https://doaj.org/article/b007b0f9e0ab413ab1ab3015666f115e |
work_keys_str_mv |
AT baptistegault correlatingadvancedmicroscopiesrevealsatomicscalemechanismslimitinglithiumionbatterylifetime AT jonathandpoplawsky correlatingadvancedmicroscopiesrevealsatomicscalemechanismslimitinglithiumionbatterylifetime |
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1718385227202560000 |