Conical-intersection dynamics and ground-state chemistry probed by extreme-ultraviolet time-resolved photoelectron spectroscopy

Recent progress in extreme-ultraviolet table-top light sources is enabling advances in ultrafast molecular dynamics. Here the authors demonstrate time-resolved photoelectron spectroscopy with such a source, observing how a molecular wave packet crosses a conical intersection, performs large-amplitud...

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Autores principales: A. von Conta, A. Tehlar, A. Schletter, Y. Arasaki, K. Takatsuka, H. J. Wörner
Formato: article
Lenguaje:EN
Publicado: Nature Portfolio 2018
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Acceso en línea:https://doaj.org/article/b11670bad4994c199b866864f0755565
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Sumario:Recent progress in extreme-ultraviolet table-top light sources is enabling advances in ultrafast molecular dynamics. Here the authors demonstrate time-resolved photoelectron spectroscopy with such a source, observing how a molecular wave packet crosses a conical intersection, performs large-amplitude motion and eventually dissociates.