Magneto-ionic suppression of magnetic vortices
Magneto-ionics refers to the non-volatile control of the magnetic properties of materials by voltage-driven ion migration. This phenomenon constitutes one of the most important magnetoelectric mechanisms and, so far, it has been employed to modify the magnetic easy axis of thin films, their coercivi...
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2021
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oai:doaj.org-article:b348b7b06da340e492af25eabf237a1c2021-11-11T14:23:41ZMagneto-ionic suppression of magnetic vortices1468-69961878-551410.1080/14686996.2021.1988830https://doaj.org/article/b348b7b06da340e492af25eabf237a1c2021-12-01T00:00:00Zhttp://dx.doi.org/10.1080/14686996.2021.1988830https://doaj.org/toc/1468-6996https://doaj.org/toc/1878-5514Magneto-ionics refers to the non-volatile control of the magnetic properties of materials by voltage-driven ion migration. This phenomenon constitutes one of the most important magnetoelectric mechanisms and, so far, it has been employed to modify the magnetic easy axis of thin films, their coercivity or their net magnetization. Herein, a novel magneto-ionic effect is demonstrated: the transition from vortex to coherent rotation states, caused by voltage-induced ion motion, in arrays of patterned nanopillars. Electrolyte-gated Co/GdOx bilayered nanopillars are chosen as a model system. Electron microscopy observations reveal that, upon voltage application, oxygen ions diffuse from GdOx to Co, resulting in the development of paramagnetic oxide phases (CoOx) along sporadic diffusion channels. This breaks up the initial magnetization configuration of the ferromagnetic pillars (i.e. vortex states) and leads to the formation of small ferromagnetic nanoclusters, embedded in the CoOx matrix, which behave as single-domain nanoparticles. As a result, a decrease in the net magnetic moment is observed, together with a drastic change in the shape of the hysteresis loop. Micromagnetic simulations are used to interpret these findings. These results pave the way towards a new potential application of magnetoelectricity: the magneto-ionic control of magnetic vortex states.Yu ChenAliona NicolencoPau MoletAgustin MihiEva PellicerJordi SortTaylor & Francis Grouparticlemagnetoelectricmagneto-ionicsvortexvoltage control of magnetismMaterials of engineering and construction. Mechanics of materialsTA401-492BiotechnologyTP248.13-248.65ENScience and Technology of Advanced Materials, Vol 22, Iss 1, Pp 972-984 (2021) |
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magnetoelectric magneto-ionics vortex voltage control of magnetism Materials of engineering and construction. Mechanics of materials TA401-492 Biotechnology TP248.13-248.65 |
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magnetoelectric magneto-ionics vortex voltage control of magnetism Materials of engineering and construction. Mechanics of materials TA401-492 Biotechnology TP248.13-248.65 Yu Chen Aliona Nicolenco Pau Molet Agustin Mihi Eva Pellicer Jordi Sort Magneto-ionic suppression of magnetic vortices |
description |
Magneto-ionics refers to the non-volatile control of the magnetic properties of materials by voltage-driven ion migration. This phenomenon constitutes one of the most important magnetoelectric mechanisms and, so far, it has been employed to modify the magnetic easy axis of thin films, their coercivity or their net magnetization. Herein, a novel magneto-ionic effect is demonstrated: the transition from vortex to coherent rotation states, caused by voltage-induced ion motion, in arrays of patterned nanopillars. Electrolyte-gated Co/GdOx bilayered nanopillars are chosen as a model system. Electron microscopy observations reveal that, upon voltage application, oxygen ions diffuse from GdOx to Co, resulting in the development of paramagnetic oxide phases (CoOx) along sporadic diffusion channels. This breaks up the initial magnetization configuration of the ferromagnetic pillars (i.e. vortex states) and leads to the formation of small ferromagnetic nanoclusters, embedded in the CoOx matrix, which behave as single-domain nanoparticles. As a result, a decrease in the net magnetic moment is observed, together with a drastic change in the shape of the hysteresis loop. Micromagnetic simulations are used to interpret these findings. These results pave the way towards a new potential application of magnetoelectricity: the magneto-ionic control of magnetic vortex states. |
format |
article |
author |
Yu Chen Aliona Nicolenco Pau Molet Agustin Mihi Eva Pellicer Jordi Sort |
author_facet |
Yu Chen Aliona Nicolenco Pau Molet Agustin Mihi Eva Pellicer Jordi Sort |
author_sort |
Yu Chen |
title |
Magneto-ionic suppression of magnetic vortices |
title_short |
Magneto-ionic suppression of magnetic vortices |
title_full |
Magneto-ionic suppression of magnetic vortices |
title_fullStr |
Magneto-ionic suppression of magnetic vortices |
title_full_unstemmed |
Magneto-ionic suppression of magnetic vortices |
title_sort |
magneto-ionic suppression of magnetic vortices |
publisher |
Taylor & Francis Group |
publishDate |
2021 |
url |
https://doaj.org/article/b348b7b06da340e492af25eabf237a1c |
work_keys_str_mv |
AT yuchen magnetoionicsuppressionofmagneticvortices AT alionanicolenco magnetoionicsuppressionofmagneticvortices AT paumolet magnetoionicsuppressionofmagneticvortices AT agustinmihi magnetoionicsuppressionofmagneticvortices AT evapellicer magnetoionicsuppressionofmagneticvortices AT jordisort magnetoionicsuppressionofmagneticvortices |
_version_ |
1718438975830491136 |