Magneto-ionic suppression of magnetic vortices

Magneto-ionics refers to the non-volatile control of the magnetic properties of materials by voltage-driven ion migration. This phenomenon constitutes one of the most important magnetoelectric mechanisms and, so far, it has been employed to modify the magnetic easy axis of thin films, their coercivi...

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Autores principales: Yu Chen, Aliona Nicolenco, Pau Molet, Agustin Mihi, Eva Pellicer, Jordi Sort
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Publicado: Taylor & Francis Group 2021
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Acceso en línea:https://doaj.org/article/b348b7b06da340e492af25eabf237a1c
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spelling oai:doaj.org-article:b348b7b06da340e492af25eabf237a1c2021-11-11T14:23:41ZMagneto-ionic suppression of magnetic vortices1468-69961878-551410.1080/14686996.2021.1988830https://doaj.org/article/b348b7b06da340e492af25eabf237a1c2021-12-01T00:00:00Zhttp://dx.doi.org/10.1080/14686996.2021.1988830https://doaj.org/toc/1468-6996https://doaj.org/toc/1878-5514Magneto-ionics refers to the non-volatile control of the magnetic properties of materials by voltage-driven ion migration. This phenomenon constitutes one of the most important magnetoelectric mechanisms and, so far, it has been employed to modify the magnetic easy axis of thin films, their coercivity or their net magnetization. Herein, a novel magneto-ionic effect is demonstrated: the transition from vortex to coherent rotation states, caused by voltage-induced ion motion, in arrays of patterned nanopillars. Electrolyte-gated Co/GdOx bilayered nanopillars are chosen as a model system. Electron microscopy observations reveal that, upon voltage application, oxygen ions diffuse from GdOx to Co, resulting in the development of paramagnetic oxide phases (CoOx) along sporadic diffusion channels. This breaks up the initial magnetization configuration of the ferromagnetic pillars (i.e. vortex states) and leads to the formation of small ferromagnetic nanoclusters, embedded in the CoOx matrix, which behave as single-domain nanoparticles. As a result, a decrease in the net magnetic moment is observed, together with a drastic change in the shape of the hysteresis loop. Micromagnetic simulations are used to interpret these findings. These results pave the way towards a new potential application of magnetoelectricity: the magneto-ionic control of magnetic vortex states.Yu ChenAliona NicolencoPau MoletAgustin MihiEva PellicerJordi SortTaylor & Francis Grouparticlemagnetoelectricmagneto-ionicsvortexvoltage control of magnetismMaterials of engineering and construction. Mechanics of materialsTA401-492BiotechnologyTP248.13-248.65ENScience and Technology of Advanced Materials, Vol 22, Iss 1, Pp 972-984 (2021)
institution DOAJ
collection DOAJ
language EN
topic magnetoelectric
magneto-ionics
vortex
voltage control of magnetism
Materials of engineering and construction. Mechanics of materials
TA401-492
Biotechnology
TP248.13-248.65
spellingShingle magnetoelectric
magneto-ionics
vortex
voltage control of magnetism
Materials of engineering and construction. Mechanics of materials
TA401-492
Biotechnology
TP248.13-248.65
Yu Chen
Aliona Nicolenco
Pau Molet
Agustin Mihi
Eva Pellicer
Jordi Sort
Magneto-ionic suppression of magnetic vortices
description Magneto-ionics refers to the non-volatile control of the magnetic properties of materials by voltage-driven ion migration. This phenomenon constitutes one of the most important magnetoelectric mechanisms and, so far, it has been employed to modify the magnetic easy axis of thin films, their coercivity or their net magnetization. Herein, a novel magneto-ionic effect is demonstrated: the transition from vortex to coherent rotation states, caused by voltage-induced ion motion, in arrays of patterned nanopillars. Electrolyte-gated Co/GdOx bilayered nanopillars are chosen as a model system. Electron microscopy observations reveal that, upon voltage application, oxygen ions diffuse from GdOx to Co, resulting in the development of paramagnetic oxide phases (CoOx) along sporadic diffusion channels. This breaks up the initial magnetization configuration of the ferromagnetic pillars (i.e. vortex states) and leads to the formation of small ferromagnetic nanoclusters, embedded in the CoOx matrix, which behave as single-domain nanoparticles. As a result, a decrease in the net magnetic moment is observed, together with a drastic change in the shape of the hysteresis loop. Micromagnetic simulations are used to interpret these findings. These results pave the way towards a new potential application of magnetoelectricity: the magneto-ionic control of magnetic vortex states.
format article
author Yu Chen
Aliona Nicolenco
Pau Molet
Agustin Mihi
Eva Pellicer
Jordi Sort
author_facet Yu Chen
Aliona Nicolenco
Pau Molet
Agustin Mihi
Eva Pellicer
Jordi Sort
author_sort Yu Chen
title Magneto-ionic suppression of magnetic vortices
title_short Magneto-ionic suppression of magnetic vortices
title_full Magneto-ionic suppression of magnetic vortices
title_fullStr Magneto-ionic suppression of magnetic vortices
title_full_unstemmed Magneto-ionic suppression of magnetic vortices
title_sort magneto-ionic suppression of magnetic vortices
publisher Taylor & Francis Group
publishDate 2021
url https://doaj.org/article/b348b7b06da340e492af25eabf237a1c
work_keys_str_mv AT yuchen magnetoionicsuppressionofmagneticvortices
AT alionanicolenco magnetoionicsuppressionofmagneticvortices
AT paumolet magnetoionicsuppressionofmagneticvortices
AT agustinmihi magnetoionicsuppressionofmagneticvortices
AT evapellicer magnetoionicsuppressionofmagneticvortices
AT jordisort magnetoionicsuppressionofmagneticvortices
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