Neighboring Pd single atoms surpass isolated single atoms for selective hydrodehalogenation catalysis

Single atom catalysts have exhibited high selectivity for hydrogenation, yet improved selectively is often accompanied by loss of activity. Here the authors report that synergistic interactions of neighboring Pd single atoms lead to both high activity and selectivity for hydrodehalogenation catalysi...

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Main Authors: Chiheng Chu, Dahong Huang, Srishti Gupta, Seunghyun Weon, Junfeng Niu, Eli Stavitski, Christopher Muhich, Jae-Hong Kim
Format: article
Language:EN
Published: Nature Portfolio 2021
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Online Access:https://doaj.org/article/b46bd6aa174148a18d26f85fe0b51e8b
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Summary:Single atom catalysts have exhibited high selectivity for hydrogenation, yet improved selectively is often accompanied by loss of activity. Here the authors report that synergistic interactions of neighboring Pd single atoms lead to both high activity and selectivity for hydrodehalogenation catalysis.