Doping strain induced bi-Ti3+ pairs for efficient N2 activation and electrocatalytic fixation

Electrocatalytic N2 conversion to ammonia offers a low-carbon alternative to industrial ammonia production, although the rational design of active, efficient catalysts remains limited. Here, authors show Ti3+-pair sites in anatase TiO2 to be active for aqueous N2 electroreduction to ammonia.

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Autores principales:	Na Cao, Zheng Chen, Ketao Zang, Jie Xu, Jun Zhong, Jun Luo, Xin Xu, Gengfeng Zheng
Formato:	article
Lenguaje:	EN
Publicado:	Nature Portfolio 2019
Materias:	Science Q
Acceso en línea:	https://doaj.org/article/bcb1fdd101b8491d9f433fe339cc9633
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spelling	oai:doaj.org-article:bcb1fdd101b8491d9f433fe339cc96332021-12-02T15:35:40ZDoping strain induced bi-Ti3+ pairs for efficient N2 activation and electrocatalytic fixation10.1038/s41467-019-10888-52041-1723https://doaj.org/article/bcb1fdd101b8491d9f433fe339cc96332019-06-01T00:00:00Zhttps://doi.org/10.1038/s41467-019-10888-5https://doaj.org/toc/2041-1723Electrocatalytic N2 conversion to ammonia offers a low-carbon alternative to industrial ammonia production, although the rational design of active, efficient catalysts remains limited. Here, authors show Ti3+-pair sites in anatase TiO2 to be active for aqueous N2 electroreduction to ammonia.Na CaoZheng ChenKetao ZangJie XuJun ZhongJun LuoXin XuGengfeng ZhengNature PortfolioarticleScienceQENNature Communications, Vol 10, Iss 1, Pp 1-12 (2019)
institution	DOAJ
collection	DOAJ
language	EN
topic	Science Q
spellingShingle	Science Q Na Cao Zheng Chen Ketao Zang Jie Xu Jun Zhong Jun Luo Xin Xu Gengfeng Zheng Doping strain induced bi-Ti3+ pairs for efficient N2 activation and electrocatalytic fixation
description	Electrocatalytic N2 conversion to ammonia offers a low-carbon alternative to industrial ammonia production, although the rational design of active, efficient catalysts remains limited. Here, authors show Ti3+-pair sites in anatase TiO2 to be active for aqueous N2 electroreduction to ammonia.
format	article
author	Na Cao Zheng Chen Ketao Zang Jie Xu Jun Zhong Jun Luo Xin Xu Gengfeng Zheng
author_facet	Na Cao Zheng Chen Ketao Zang Jie Xu Jun Zhong Jun Luo Xin Xu Gengfeng Zheng
author_sort	Na Cao
title	Doping strain induced bi-Ti3+ pairs for efficient N2 activation and electrocatalytic fixation
title_short	Doping strain induced bi-Ti3+ pairs for efficient N2 activation and electrocatalytic fixation
title_full	Doping strain induced bi-Ti3+ pairs for efficient N2 activation and electrocatalytic fixation
title_fullStr	Doping strain induced bi-Ti3+ pairs for efficient N2 activation and electrocatalytic fixation
title_full_unstemmed	Doping strain induced bi-Ti3+ pairs for efficient N2 activation and electrocatalytic fixation
title_sort	doping strain induced bi-ti3+ pairs for efficient n2 activation and electrocatalytic fixation
publisher	Nature Portfolio
publishDate	2019
url	https://doaj.org/article/bcb1fdd101b8491d9f433fe339cc9633
work_keys_str_mv	AT nacao dopingstraininducedbiti3pairsforefficientn2activationandelectrocatalyticfixation AT zhengchen dopingstraininducedbiti3pairsforefficientn2activationandelectrocatalyticfixation AT ketaozang dopingstraininducedbiti3pairsforefficientn2activationandelectrocatalyticfixation AT jiexu dopingstraininducedbiti3pairsforefficientn2activationandelectrocatalyticfixation AT junzhong dopingstraininducedbiti3pairsforefficientn2activationandelectrocatalyticfixation AT junluo dopingstraininducedbiti3pairsforefficientn2activationandelectrocatalyticfixation AT xinxu dopingstraininducedbiti3pairsforefficientn2activationandelectrocatalyticfixation AT gengfengzheng dopingstraininducedbiti3pairsforefficientn2activationandelectrocatalyticfixation
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Doping strain induced bi-Ti3+ pairs for efficient N2 activation and electrocatalytic fixation

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