Excited-state vibrational dynamics toward the polaron in methylammonium lead iodide perovskite
Elucidating electron-phonon coupling in hybrid organic-inorganic perovskites may help us to understand the high photovoltaic efficiency. Here, the authors observe low-frequency Raman modes and related nuclear displacements of the Pb–I framework, indicating how these vibrational motions lead to polar...
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Nature Portfolio
2018
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oai:doaj.org-article:bd6e6e7f3aaf425880488f0fe476e6752021-12-02T13:24:16ZExcited-state vibrational dynamics toward the polaron in methylammonium lead iodide perovskite10.1038/s41467-018-04946-72041-1723https://doaj.org/article/bd6e6e7f3aaf425880488f0fe476e6752018-06-01T00:00:00Zhttps://doi.org/10.1038/s41467-018-04946-7https://doaj.org/toc/2041-1723Elucidating electron-phonon coupling in hybrid organic-inorganic perovskites may help us to understand the high photovoltaic efficiency. Here, the authors observe low-frequency Raman modes and related nuclear displacements of the Pb–I framework, indicating how these vibrational motions lead to polaron formation in perovskites.Myeongkee ParkAmanda J. NeukirchSebastian E. Reyes-LilloMinliang LaiScott R. EllisDaniel DietzeJeffrey B. NeatonPeidong YangSergei TretiakRichard A. MathiesNature PortfolioarticleScienceQENNature Communications, Vol 9, Iss 1, Pp 1-9 (2018) |
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Science Q Myeongkee Park Amanda J. Neukirch Sebastian E. Reyes-Lillo Minliang Lai Scott R. Ellis Daniel Dietze Jeffrey B. Neaton Peidong Yang Sergei Tretiak Richard A. Mathies Excited-state vibrational dynamics toward the polaron in methylammonium lead iodide perovskite |
description |
Elucidating electron-phonon coupling in hybrid organic-inorganic perovskites may help us to understand the high photovoltaic efficiency. Here, the authors observe low-frequency Raman modes and related nuclear displacements of the Pb–I framework, indicating how these vibrational motions lead to polaron formation in perovskites. |
format |
article |
author |
Myeongkee Park Amanda J. Neukirch Sebastian E. Reyes-Lillo Minliang Lai Scott R. Ellis Daniel Dietze Jeffrey B. Neaton Peidong Yang Sergei Tretiak Richard A. Mathies |
author_facet |
Myeongkee Park Amanda J. Neukirch Sebastian E. Reyes-Lillo Minliang Lai Scott R. Ellis Daniel Dietze Jeffrey B. Neaton Peidong Yang Sergei Tretiak Richard A. Mathies |
author_sort |
Myeongkee Park |
title |
Excited-state vibrational dynamics toward the polaron in methylammonium lead iodide perovskite |
title_short |
Excited-state vibrational dynamics toward the polaron in methylammonium lead iodide perovskite |
title_full |
Excited-state vibrational dynamics toward the polaron in methylammonium lead iodide perovskite |
title_fullStr |
Excited-state vibrational dynamics toward the polaron in methylammonium lead iodide perovskite |
title_full_unstemmed |
Excited-state vibrational dynamics toward the polaron in methylammonium lead iodide perovskite |
title_sort |
excited-state vibrational dynamics toward the polaron in methylammonium lead iodide perovskite |
publisher |
Nature Portfolio |
publishDate |
2018 |
url |
https://doaj.org/article/bd6e6e7f3aaf425880488f0fe476e675 |
work_keys_str_mv |
AT myeongkeepark excitedstatevibrationaldynamicstowardthepolaroninmethylammoniumleadiodideperovskite AT amandajneukirch excitedstatevibrationaldynamicstowardthepolaroninmethylammoniumleadiodideperovskite AT sebastianereyeslillo excitedstatevibrationaldynamicstowardthepolaroninmethylammoniumleadiodideperovskite AT minlianglai excitedstatevibrationaldynamicstowardthepolaroninmethylammoniumleadiodideperovskite AT scottrellis excitedstatevibrationaldynamicstowardthepolaroninmethylammoniumleadiodideperovskite AT danieldietze excitedstatevibrationaldynamicstowardthepolaroninmethylammoniumleadiodideperovskite AT jeffreybneaton excitedstatevibrationaldynamicstowardthepolaroninmethylammoniumleadiodideperovskite AT peidongyang excitedstatevibrationaldynamicstowardthepolaroninmethylammoniumleadiodideperovskite AT sergeitretiak excitedstatevibrationaldynamicstowardthepolaroninmethylammoniumleadiodideperovskite AT richardamathies excitedstatevibrationaldynamicstowardthepolaroninmethylammoniumleadiodideperovskite |
_version_ |
1718393117307043840 |