Excited-state vibrational dynamics toward the polaron in methylammonium lead iodide perovskite

Elucidating electron-phonon coupling in hybrid organic-inorganic perovskites may help us to understand the high photovoltaic efficiency. Here, the authors observe low-frequency Raman modes and related nuclear displacements of the Pb–I framework, indicating how these vibrational motions lead to polar...

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Autores principales: Myeongkee Park, Amanda J. Neukirch, Sebastian E. Reyes-Lillo, Minliang Lai, Scott R. Ellis, Daniel Dietze, Jeffrey B. Neaton, Peidong Yang, Sergei Tretiak, Richard A. Mathies
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Publicado: Nature Portfolio 2018
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Acceso en línea:https://doaj.org/article/bd6e6e7f3aaf425880488f0fe476e675
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spelling oai:doaj.org-article:bd6e6e7f3aaf425880488f0fe476e6752021-12-02T13:24:16ZExcited-state vibrational dynamics toward the polaron in methylammonium lead iodide perovskite10.1038/s41467-018-04946-72041-1723https://doaj.org/article/bd6e6e7f3aaf425880488f0fe476e6752018-06-01T00:00:00Zhttps://doi.org/10.1038/s41467-018-04946-7https://doaj.org/toc/2041-1723Elucidating electron-phonon coupling in hybrid organic-inorganic perovskites may help us to understand the high photovoltaic efficiency. Here, the authors observe low-frequency Raman modes and related nuclear displacements of the Pb–I framework, indicating how these vibrational motions lead to polaron formation in perovskites.Myeongkee ParkAmanda J. NeukirchSebastian E. Reyes-LilloMinliang LaiScott R. EllisDaniel DietzeJeffrey B. NeatonPeidong YangSergei TretiakRichard A. MathiesNature PortfolioarticleScienceQENNature Communications, Vol 9, Iss 1, Pp 1-9 (2018)
institution DOAJ
collection DOAJ
language EN
topic Science
Q
spellingShingle Science
Q
Myeongkee Park
Amanda J. Neukirch
Sebastian E. Reyes-Lillo
Minliang Lai
Scott R. Ellis
Daniel Dietze
Jeffrey B. Neaton
Peidong Yang
Sergei Tretiak
Richard A. Mathies
Excited-state vibrational dynamics toward the polaron in methylammonium lead iodide perovskite
description Elucidating electron-phonon coupling in hybrid organic-inorganic perovskites may help us to understand the high photovoltaic efficiency. Here, the authors observe low-frequency Raman modes and related nuclear displacements of the Pb–I framework, indicating how these vibrational motions lead to polaron formation in perovskites.
format article
author Myeongkee Park
Amanda J. Neukirch
Sebastian E. Reyes-Lillo
Minliang Lai
Scott R. Ellis
Daniel Dietze
Jeffrey B. Neaton
Peidong Yang
Sergei Tretiak
Richard A. Mathies
author_facet Myeongkee Park
Amanda J. Neukirch
Sebastian E. Reyes-Lillo
Minliang Lai
Scott R. Ellis
Daniel Dietze
Jeffrey B. Neaton
Peidong Yang
Sergei Tretiak
Richard A. Mathies
author_sort Myeongkee Park
title Excited-state vibrational dynamics toward the polaron in methylammonium lead iodide perovskite
title_short Excited-state vibrational dynamics toward the polaron in methylammonium lead iodide perovskite
title_full Excited-state vibrational dynamics toward the polaron in methylammonium lead iodide perovskite
title_fullStr Excited-state vibrational dynamics toward the polaron in methylammonium lead iodide perovskite
title_full_unstemmed Excited-state vibrational dynamics toward the polaron in methylammonium lead iodide perovskite
title_sort excited-state vibrational dynamics toward the polaron in methylammonium lead iodide perovskite
publisher Nature Portfolio
publishDate 2018
url https://doaj.org/article/bd6e6e7f3aaf425880488f0fe476e675
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