Probing ultrafast ππ*/nπ* internal conversion in organic chromophores via K-edge resonant absorption

Probing ultrafast ππ*/nπ* internal conversion in organic chromophores via K-edge resonant absorption

Many photo-induced processes such as photosynthesis occur in organic molecules, but their femtosecond excited-state dynamics are difficult to track. Here, the authors exploit the element and site selectivity of soft X-ray absorption to sensitively follow the ultrafast ππ*/nπ* electronic relaxation o...

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Autores principales: T. J. A. Wolf, R. H. Myhre, J. P. Cryan, S. Coriani, R. J. Squibb, A. Battistoni, N. Berrah, C. Bostedt, P. Bucksbaum, G. Coslovich, R. Feifel, K. J. Gaffney, J. Grilj, T. J. Martinez, S. Miyabe, S. P. Moeller, M. Mucke, A. Natan, R. Obaid, T. Osipov, O. Plekan, S. Wang, H. Koch, M. Gühr
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Lenguaje:EN
Publicado: Nature Portfolio 2017
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Acceso en línea:https://doaj.org/article/bf84fb1d3c9c472f9e0e1473e557de0e
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spelling oai:doaj.org-article:bf84fb1d3c9c472f9e0e1473e557de0e2021-12-02T13:24:04ZProbing ultrafast ππ*/nπ* internal conversion in organic chromophores via K-edge resonant absorption10.1038/s41467-017-00069-72041-1723https://doaj.org/article/bf84fb1d3c9c472f9e0e1473e557de0e2017-06-01T00:00:00Zhttps://doi.org/10.1038/s41467-017-00069-7https://doaj.org/toc/2041-1723Many photo-induced processes such as photosynthesis occur in organic molecules, but their femtosecond excited-state dynamics are difficult to track. Here, the authors exploit the element and site selectivity of soft X-ray absorption to sensitively follow the ultrafast ππ*/nπ* electronic relaxation of hetero-organic molecules.T. J. A. WolfR. H. MyhreJ. P. CryanS. CorianiR. J. SquibbA. BattistoniN. BerrahC. BostedtP. BucksbaumG. CoslovichR. FeifelK. J. GaffneyJ. GriljT. J. MartinezS. MiyabeS. P. MoellerM. MuckeA. NatanR. ObaidT. OsipovO. PlekanS. WangH. KochM. GührNature PortfolioarticleScienceQENNature Communications, Vol 8, Iss 1, Pp 1-7 (2017)
institution DOAJ
collection DOAJ
language EN
topic Science
Q
spellingShingle Science
Q
T. J. A. Wolf
R. H. Myhre
J. P. Cryan
S. Coriani
R. J. Squibb
A. Battistoni
N. Berrah
C. Bostedt
P. Bucksbaum
G. Coslovich
R. Feifel
K. J. Gaffney
J. Grilj
T. J. Martinez
S. Miyabe
S. P. Moeller
M. Mucke
A. Natan
R. Obaid
T. Osipov
O. Plekan
S. Wang
H. Koch
M. Gühr
Probing ultrafast ππ*/nπ* internal conversion in organic chromophores via K-edge resonant absorption
description Many photo-induced processes such as photosynthesis occur in organic molecules, but their femtosecond excited-state dynamics are difficult to track. Here, the authors exploit the element and site selectivity of soft X-ray absorption to sensitively follow the ultrafast ππ*/nπ* electronic relaxation of hetero-organic molecules.
format article
author T. J. A. Wolf
R. H. Myhre
J. P. Cryan
S. Coriani
R. J. Squibb
A. Battistoni
N. Berrah
C. Bostedt
P. Bucksbaum
G. Coslovich
R. Feifel
K. J. Gaffney
J. Grilj
T. J. Martinez
S. Miyabe
S. P. Moeller
M. Mucke
A. Natan
R. Obaid
T. Osipov
O. Plekan
S. Wang
H. Koch
M. Gühr
author_facet T. J. A. Wolf
R. H. Myhre
J. P. Cryan
S. Coriani
R. J. Squibb
A. Battistoni
N. Berrah
C. Bostedt
P. Bucksbaum
G. Coslovich
R. Feifel
K. J. Gaffney
J. Grilj
T. J. Martinez
S. Miyabe
S. P. Moeller
M. Mucke
A. Natan
R. Obaid
T. Osipov
O. Plekan
S. Wang
H. Koch
M. Gühr
author_sort T. J. A. Wolf
title Probing ultrafast ππ*/nπ* internal conversion in organic chromophores via K-edge resonant absorption
title_short Probing ultrafast ππ*/nπ* internal conversion in organic chromophores via K-edge resonant absorption
title_full Probing ultrafast ππ*/nπ* internal conversion in organic chromophores via K-edge resonant absorption
title_fullStr Probing ultrafast ππ*/nπ* internal conversion in organic chromophores via K-edge resonant absorption
title_full_unstemmed Probing ultrafast ππ*/nπ* internal conversion in organic chromophores via K-edge resonant absorption
title_sort probing ultrafast ππ*/nπ* internal conversion in organic chromophores via k-edge resonant absorption
publisher Nature Portfolio
publishDate 2017
url https://doaj.org/article/bf84fb1d3c9c472f9e0e1473e557de0e
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