High J c and low anisotropy of hydrogen doped NdFeAsO superconducting thin film
Abstract The recent realisations of hydrogen doped LnFeAsO (Ln = Nd and Sm) superconducting epitaxial thin films call for further investigation of their structural and electrical transport properties. Here, we report on the microstructure of a NdFeAs(O,H) epitaxial thin film and its temperature, fie...
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2021
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oai:doaj.org-article:c2a19a46f01643c68947688753620bdd2021-12-02T15:54:05ZHigh J c and low anisotropy of hydrogen doped NdFeAsO superconducting thin film10.1038/s41598-021-85216-32045-2322https://doaj.org/article/c2a19a46f01643c68947688753620bdd2021-03-01T00:00:00Zhttps://doi.org/10.1038/s41598-021-85216-3https://doaj.org/toc/2045-2322Abstract The recent realisations of hydrogen doped LnFeAsO (Ln = Nd and Sm) superconducting epitaxial thin films call for further investigation of their structural and electrical transport properties. Here, we report on the microstructure of a NdFeAs(O,H) epitaxial thin film and its temperature, field, and orientation dependencies of the resistivity and the critical current density J c. The superconducting transition temperature T c is comparable to NdFeAs(O,F). Transmission electron microscopy investigation supported that hydrogen is homogenously substituted for oxygen. A high self-field J c of over 10 MA/cm2 was recorded at 5 K, which is likely to be caused by a short London penetration depth. The anisotropic Ginzburg–Landau scaling for the angle dependence of J c yielded temperature-dependent scaling parameters γJ that decreased from 1.6 at 30 K to 1.3 at 5 K. This is opposite to the behaviour of NdFeAs(O,F). Additionally, γJ of NdFeAs(O,H) is smaller than that of NdFeAs(O,F). Our results indicate that heavily electron doping by means of hydrogen substitution for oxygen in LnFeAsO is highly beneficial for achieving high J c with low anisotropy without compromising T c, which is favourable for high-field magnet applications.Kazumasa IidaJens HänischKeisuke KondoMingyu ChenTakafumi HatanoChao WangHikaru SaitoSatoshi HataHiroshi IkutaNature PortfolioarticleMedicineRScienceQENScientific Reports, Vol 11, Iss 1, Pp 1-9 (2021) |
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Medicine R Science Q Kazumasa Iida Jens Hänisch Keisuke Kondo Mingyu Chen Takafumi Hatano Chao Wang Hikaru Saito Satoshi Hata Hiroshi Ikuta High J c and low anisotropy of hydrogen doped NdFeAsO superconducting thin film |
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Abstract The recent realisations of hydrogen doped LnFeAsO (Ln = Nd and Sm) superconducting epitaxial thin films call for further investigation of their structural and electrical transport properties. Here, we report on the microstructure of a NdFeAs(O,H) epitaxial thin film and its temperature, field, and orientation dependencies of the resistivity and the critical current density J c. The superconducting transition temperature T c is comparable to NdFeAs(O,F). Transmission electron microscopy investigation supported that hydrogen is homogenously substituted for oxygen. A high self-field J c of over 10 MA/cm2 was recorded at 5 K, which is likely to be caused by a short London penetration depth. The anisotropic Ginzburg–Landau scaling for the angle dependence of J c yielded temperature-dependent scaling parameters γJ that decreased from 1.6 at 30 K to 1.3 at 5 K. This is opposite to the behaviour of NdFeAs(O,F). Additionally, γJ of NdFeAs(O,H) is smaller than that of NdFeAs(O,F). Our results indicate that heavily electron doping by means of hydrogen substitution for oxygen in LnFeAsO is highly beneficial for achieving high J c with low anisotropy without compromising T c, which is favourable for high-field magnet applications. |
format |
article |
author |
Kazumasa Iida Jens Hänisch Keisuke Kondo Mingyu Chen Takafumi Hatano Chao Wang Hikaru Saito Satoshi Hata Hiroshi Ikuta |
author_facet |
Kazumasa Iida Jens Hänisch Keisuke Kondo Mingyu Chen Takafumi Hatano Chao Wang Hikaru Saito Satoshi Hata Hiroshi Ikuta |
author_sort |
Kazumasa Iida |
title |
High J c and low anisotropy of hydrogen doped NdFeAsO superconducting thin film |
title_short |
High J c and low anisotropy of hydrogen doped NdFeAsO superconducting thin film |
title_full |
High J c and low anisotropy of hydrogen doped NdFeAsO superconducting thin film |
title_fullStr |
High J c and low anisotropy of hydrogen doped NdFeAsO superconducting thin film |
title_full_unstemmed |
High J c and low anisotropy of hydrogen doped NdFeAsO superconducting thin film |
title_sort |
high j c and low anisotropy of hydrogen doped ndfeaso superconducting thin film |
publisher |
Nature Portfolio |
publishDate |
2021 |
url |
https://doaj.org/article/c2a19a46f01643c68947688753620bdd |
work_keys_str_mv |
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