Double layer charging driven carbon dioxide adsorption limits the rate of electrochemical carbon dioxide reduction on Gold

Electrochemical CO2 reduction is a potential route to the sustainable production of valuable fuels and chemicals. In this joint experimental-theoretical work, the authors address the issue of the rate-limiting step on Gold and present insights from multi-scale simulations into the importance of the...

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Autores principales:	Stefan Ringe, Carlos G. Morales-Guio, Leanne D. Chen, Meredith Fields, Thomas F. Jaramillo, Christopher Hahn, Karen Chan
Formato:	article
Lenguaje:	EN
Publicado:	Nature Portfolio 2020
Materias:	Science Q
Acceso en línea:	https://doaj.org/article/c7cdd1d894b34fb6963760d4a0cc152a
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spelling	oai:doaj.org-article:c7cdd1d894b34fb6963760d4a0cc152a2021-12-02T14:41:23ZDouble layer charging driven carbon dioxide adsorption limits the rate of electrochemical carbon dioxide reduction on Gold10.1038/s41467-019-13777-z2041-1723https://doaj.org/article/c7cdd1d894b34fb6963760d4a0cc152a2020-01-01T00:00:00Zhttps://doi.org/10.1038/s41467-019-13777-zhttps://doaj.org/toc/2041-1723Electrochemical CO2 reduction is a potential route to the sustainable production of valuable fuels and chemicals. In this joint experimental-theoretical work, the authors address the issue of the rate-limiting step on Gold and present insights from multi-scale simulations into the importance of the electric double layer on reaction kinetics and mass transport.Stefan RingeCarlos G. Morales-GuioLeanne D. ChenMeredith FieldsThomas F. JaramilloChristopher HahnKaren ChanNature PortfolioarticleScienceQENNature Communications, Vol 11, Iss 1, Pp 1-11 (2020)
institution	DOAJ
collection	DOAJ
language	EN
topic	Science Q
spellingShingle	Science Q Stefan Ringe Carlos G. Morales-Guio Leanne D. Chen Meredith Fields Thomas F. Jaramillo Christopher Hahn Karen Chan Double layer charging driven carbon dioxide adsorption limits the rate of electrochemical carbon dioxide reduction on Gold
description	Electrochemical CO2 reduction is a potential route to the sustainable production of valuable fuels and chemicals. In this joint experimental-theoretical work, the authors address the issue of the rate-limiting step on Gold and present insights from multi-scale simulations into the importance of the electric double layer on reaction kinetics and mass transport.
format	article
author	Stefan Ringe Carlos G. Morales-Guio Leanne D. Chen Meredith Fields Thomas F. Jaramillo Christopher Hahn Karen Chan
author_facet	Stefan Ringe Carlos G. Morales-Guio Leanne D. Chen Meredith Fields Thomas F. Jaramillo Christopher Hahn Karen Chan
author_sort	Stefan Ringe
title	Double layer charging driven carbon dioxide adsorption limits the rate of electrochemical carbon dioxide reduction on Gold
title_short	Double layer charging driven carbon dioxide adsorption limits the rate of electrochemical carbon dioxide reduction on Gold
title_full	Double layer charging driven carbon dioxide adsorption limits the rate of electrochemical carbon dioxide reduction on Gold
title_fullStr	Double layer charging driven carbon dioxide adsorption limits the rate of electrochemical carbon dioxide reduction on Gold
title_full_unstemmed	Double layer charging driven carbon dioxide adsorption limits the rate of electrochemical carbon dioxide reduction on Gold
title_sort	double layer charging driven carbon dioxide adsorption limits the rate of electrochemical carbon dioxide reduction on gold
publisher	Nature Portfolio
publishDate	2020
url	https://doaj.org/article/c7cdd1d894b34fb6963760d4a0cc152a
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Double layer charging driven carbon dioxide adsorption limits the rate of electrochemical carbon dioxide reduction on Gold

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