Distinguishing physical mechanisms using GISAXS experiments and linear theory: the importance of high wavenumbers

Abstract In this work we analyze GISAXS measurements of the structure factor of Si surfaces evolving during 1 keV Ar+ ion bombardment. Using newly-developed methods sensitive to the full range of experimentally-available wavenumbers q, we extract the linear amplification rate R(q) governing surface...

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Autores principales: Scott A. Norris, Joy C. Perkinson, Mahsa Mokhtarzadeh, Eitan Anzenberg, Michael J. Aziz, Karl F. Ludwig
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Publicado: Nature Portfolio 2017
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spelling oai:doaj.org-article:c8b23817e2504bc9bfe5290fd0990bb82021-12-02T11:52:35ZDistinguishing physical mechanisms using GISAXS experiments and linear theory: the importance of high wavenumbers10.1038/s41598-017-01059-x2045-2322https://doaj.org/article/c8b23817e2504bc9bfe5290fd0990bb82017-05-01T00:00:00Zhttps://doi.org/10.1038/s41598-017-01059-xhttps://doaj.org/toc/2045-2322Abstract In this work we analyze GISAXS measurements of the structure factor of Si surfaces evolving during 1 keV Ar+ ion bombardment. Using newly-developed methods sensitive to the full range of experimentally-available wavenumbers q, we extract the linear amplification rate R(q) governing surface stability over a range of wavenumbers 4–5 times larger than has previously been obtained. Comparing with theoretical models also retaining full wavenumber-dependence, we find an excellent fit of the experimental data over the full range of irradiation angles and wavenumbers. Moreover, the fitted parameter values represent experimental evaluation of the magnitudes of most physical mechanisms currently believed to be important to the pattern-formation process. In all cases, the extracted values agree well with direct observations or atomistic simulations of the same quantities, suggesting that GISAXS analysis may allow more powerful comparison between experiment and theory than had previously been thought.Scott A. NorrisJoy C. PerkinsonMahsa MokhtarzadehEitan AnzenbergMichael J. AzizKarl F. LudwigNature PortfolioarticleMedicineRScienceQENScientific Reports, Vol 7, Iss 1, Pp 1-12 (2017)
institution DOAJ
collection DOAJ
language EN
topic Medicine
R
Science
Q
spellingShingle Medicine
R
Science
Q
Scott A. Norris
Joy C. Perkinson
Mahsa Mokhtarzadeh
Eitan Anzenberg
Michael J. Aziz
Karl F. Ludwig
Distinguishing physical mechanisms using GISAXS experiments and linear theory: the importance of high wavenumbers
description Abstract In this work we analyze GISAXS measurements of the structure factor of Si surfaces evolving during 1 keV Ar+ ion bombardment. Using newly-developed methods sensitive to the full range of experimentally-available wavenumbers q, we extract the linear amplification rate R(q) governing surface stability over a range of wavenumbers 4–5 times larger than has previously been obtained. Comparing with theoretical models also retaining full wavenumber-dependence, we find an excellent fit of the experimental data over the full range of irradiation angles and wavenumbers. Moreover, the fitted parameter values represent experimental evaluation of the magnitudes of most physical mechanisms currently believed to be important to the pattern-formation process. In all cases, the extracted values agree well with direct observations or atomistic simulations of the same quantities, suggesting that GISAXS analysis may allow more powerful comparison between experiment and theory than had previously been thought.
format article
author Scott A. Norris
Joy C. Perkinson
Mahsa Mokhtarzadeh
Eitan Anzenberg
Michael J. Aziz
Karl F. Ludwig
author_facet Scott A. Norris
Joy C. Perkinson
Mahsa Mokhtarzadeh
Eitan Anzenberg
Michael J. Aziz
Karl F. Ludwig
author_sort Scott A. Norris
title Distinguishing physical mechanisms using GISAXS experiments and linear theory: the importance of high wavenumbers
title_short Distinguishing physical mechanisms using GISAXS experiments and linear theory: the importance of high wavenumbers
title_full Distinguishing physical mechanisms using GISAXS experiments and linear theory: the importance of high wavenumbers
title_fullStr Distinguishing physical mechanisms using GISAXS experiments and linear theory: the importance of high wavenumbers
title_full_unstemmed Distinguishing physical mechanisms using GISAXS experiments and linear theory: the importance of high wavenumbers
title_sort distinguishing physical mechanisms using gisaxs experiments and linear theory: the importance of high wavenumbers
publisher Nature Portfolio
publishDate 2017
url https://doaj.org/article/c8b23817e2504bc9bfe5290fd0990bb8
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