Observing collisions beyond the secular approximation limit

Ultrafast molecular relaxation can be probed with short laser pulses. Here the authors study collisional behavior of a N2O and He mixture beyond secular approximation by aligning them using laser pulses and probing their rotational echoes.

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Detalles Bibliográficos
Autores principales: Junyang Ma, Haisu Zhang, Bruno Lavorel, Franck Billard, Edouard Hertz, Jian Wu, Christian Boulet, Jean-Michel Hartmann, Olivier Faucher
Formato: article
Lenguaje:EN
Publicado: Nature Portfolio 2019
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Acceso en línea:https://doaj.org/article/c969a1b619bd4db69541e927d24647a6
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Descripción
Sumario:Ultrafast molecular relaxation can be probed with short laser pulses. Here the authors study collisional behavior of a N2O and He mixture beyond secular approximation by aligning them using laser pulses and probing their rotational echoes.