Resolving sub-angstrom ambient motion through reconstruction from vibrational spectra

Tracking single molecule movements is a challenging task, but highly desired for applications and fundamental studies. Here the authors reconstruct the sub-angstrom relative movements of a molecule interacting with a metal adatom, by measuring its vibrational spectrum in a self-assembled monolayer,...

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Auteurs principaux: Jack Griffiths, Tamás Földes, Bart de Nijs, Rohit Chikkaraddy, Demelza Wright, William M. Deacon, Dénes Berta, Charlie Readman, David-Benjamin Grys, Edina Rosta, Jeremy J. Baumberg
Format: article
Langue:EN
Publié: Nature Portfolio 2021
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Accès en ligne:https://doaj.org/article/c9cfd2b93ad4428287b225ed1c2efee2
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Résumé:Tracking single molecule movements is a challenging task, but highly desired for applications and fundamental studies. Here the authors reconstruct the sub-angstrom relative movements of a molecule interacting with a metal adatom, by measuring its vibrational spectrum in a self-assembled monolayer, continuously modified by the adatom in a nanoparticle-on-mirror construct.