On Process Intensification through Membrane Storage Reactors

In this work, a dynamic, one-dimensional, first principle-based model of a novel membrane storage reactor (MSR) process is developed and simulated. The resulting governing equations are rendered dimensionless and are shown to feature two dimensionless groups that can be used to affect process perfor...

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Autores principales:	John Lowd, Theodore Tsotsis, Vasilios I. Manousiouthakis
Formato:	article
Lenguaje:	EN
Publicado:	MDPI AG 2021
Materias:	membrane intensification storage reactor process model Physics QC1-999 Chemistry QD1-999
Acceso en línea:	https://doaj.org/article/cd26f450a1104fa2804c15019c6e1a8c
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id	oai:doaj.org-article:cd26f450a1104fa2804c15019c6e1a8c
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spelling	oai:doaj.org-article:cd26f450a1104fa2804c15019c6e1a8c2021-11-25T18:59:16ZOn Process Intensification through Membrane Storage Reactors10.3390/separations81101952297-8739https://doaj.org/article/cd26f450a1104fa2804c15019c6e1a8c2021-10-01T00:00:00Zhttps://www.mdpi.com/2297-8739/8/11/195https://doaj.org/toc/2297-8739In this work, a dynamic, one-dimensional, first principle-based model of a novel membrane storage reactor (MSR) process is developed and simulated. The resulting governing equations are rendered dimensionless and are shown to feature two dimensionless groups that can be used to affect process performance. The novel process is shown to intensify production of a desired species through the creation of two physically distinct domains separated by a semipermeable boundary, and dynamic operation. A number of metrics are then introduced and applied to a case study on Steam Methane Reforming, for which a parametric study is carried out which establishes the superior performance of the MSR when compared to a reactor operating at steady state (SSR).John LowdTheodore TsotsisVasilios I. ManousiouthakisMDPI AGarticlemembraneintensificationstoragereactorprocessmodelPhysicsQC1-999ChemistryQD1-999ENSeparations, Vol 8, Iss 195, p 195 (2021)
institution	DOAJ
collection	DOAJ
language	EN
topic	membrane intensification storage reactor process model Physics QC1-999 Chemistry QD1-999
spellingShingle	membrane intensification storage reactor process model Physics QC1-999 Chemistry QD1-999 John Lowd Theodore Tsotsis Vasilios I. Manousiouthakis On Process Intensification through Membrane Storage Reactors
description	In this work, a dynamic, one-dimensional, first principle-based model of a novel membrane storage reactor (MSR) process is developed and simulated. The resulting governing equations are rendered dimensionless and are shown to feature two dimensionless groups that can be used to affect process performance. The novel process is shown to intensify production of a desired species through the creation of two physically distinct domains separated by a semipermeable boundary, and dynamic operation. A number of metrics are then introduced and applied to a case study on Steam Methane Reforming, for which a parametric study is carried out which establishes the superior performance of the MSR when compared to a reactor operating at steady state (SSR).
format	article
author	John Lowd Theodore Tsotsis Vasilios I. Manousiouthakis
author_facet	John Lowd Theodore Tsotsis Vasilios I. Manousiouthakis
author_sort	John Lowd
title	On Process Intensification through Membrane Storage Reactors
title_short	On Process Intensification through Membrane Storage Reactors
title_full	On Process Intensification through Membrane Storage Reactors
title_fullStr	On Process Intensification through Membrane Storage Reactors
title_full_unstemmed	On Process Intensification through Membrane Storage Reactors
title_sort	on process intensification through membrane storage reactors
publisher	MDPI AG
publishDate	2021
url	https://doaj.org/article/cd26f450a1104fa2804c15019c6e1a8c
work_keys_str_mv	AT johnlowd onprocessintensificationthroughmembranestoragereactors AT theodoretsotsis onprocessintensificationthroughmembranestoragereactors AT vasiliosimanousiouthakis onprocessintensificationthroughmembranestoragereactors
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On Process Intensification through Membrane Storage Reactors

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