Rationally designed Sb2S3/PDI composites with enhanced visible light photoactivity
Constructing organic-inorganic semiconductor heterojunctions is an efficient way to inhibit the recombination of photogenerated charge carriers and enhance photocatalytic performance of semiconductor. Herein, a novel heterojunction antimony sulfide-perylene diimides (Sb2S3-PDI) heterojunction has be...
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2022
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oai:doaj.org-article:ce518838853f40b281ceaa4daa75a5f32021-11-24T04:27:31ZRationally designed Sb2S3/PDI composites with enhanced visible light photoactivity1873-390510.1016/j.catcom.2021.106368https://doaj.org/article/ce518838853f40b281ceaa4daa75a5f32022-02-01T00:00:00Zhttp://www.sciencedirect.com/science/article/pii/S1566736721000911https://doaj.org/toc/1873-3905Constructing organic-inorganic semiconductor heterojunctions is an efficient way to inhibit the recombination of photogenerated charge carriers and enhance photocatalytic performance of semiconductor. Herein, a novel heterojunction antimony sulfide-perylene diimides (Sb2S3-PDI) heterojunction has been fabricated through a facile hydrothermal method. Compared with bare Sb2S3 and PDI, the Sb2S3-PDI hybrid has showed significantly superior activity in photocatalytic reduction of Cr (VI). The superior photocatalytic performance of Sb2S3-PDI hybrid is due to the formation of type-I heterojunction, which leads to a more efficient separation and migration of photogenerated electron-hole pairs. This work is expected to promote continued interest in the construction of organic-inorganic semiconductor composites with enhanced photocatalytic performance.Jin-Ge HaoHui-Qi ChenLei XieZe-Xiang LiJia-Lin ZhangWei-Ya HuangTao DengKang-Qiang LuKai YangElsevierarticleAntimony sulfidePerylene diimidesSemiconductorHeterojunctionsPhotocatalysisChemistryQD1-999ENCatalysis Communications, Vol 162, Iss , Pp 106368- (2022) |
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DOAJ |
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Antimony sulfide Perylene diimides Semiconductor Heterojunctions Photocatalysis Chemistry QD1-999 |
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Antimony sulfide Perylene diimides Semiconductor Heterojunctions Photocatalysis Chemistry QD1-999 Jin-Ge Hao Hui-Qi Chen Lei Xie Ze-Xiang Li Jia-Lin Zhang Wei-Ya Huang Tao Deng Kang-Qiang Lu Kai Yang Rationally designed Sb2S3/PDI composites with enhanced visible light photoactivity |
description |
Constructing organic-inorganic semiconductor heterojunctions is an efficient way to inhibit the recombination of photogenerated charge carriers and enhance photocatalytic performance of semiconductor. Herein, a novel heterojunction antimony sulfide-perylene diimides (Sb2S3-PDI) heterojunction has been fabricated through a facile hydrothermal method. Compared with bare Sb2S3 and PDI, the Sb2S3-PDI hybrid has showed significantly superior activity in photocatalytic reduction of Cr (VI). The superior photocatalytic performance of Sb2S3-PDI hybrid is due to the formation of type-I heterojunction, which leads to a more efficient separation and migration of photogenerated electron-hole pairs. This work is expected to promote continued interest in the construction of organic-inorganic semiconductor composites with enhanced photocatalytic performance. |
format |
article |
author |
Jin-Ge Hao Hui-Qi Chen Lei Xie Ze-Xiang Li Jia-Lin Zhang Wei-Ya Huang Tao Deng Kang-Qiang Lu Kai Yang |
author_facet |
Jin-Ge Hao Hui-Qi Chen Lei Xie Ze-Xiang Li Jia-Lin Zhang Wei-Ya Huang Tao Deng Kang-Qiang Lu Kai Yang |
author_sort |
Jin-Ge Hao |
title |
Rationally designed Sb2S3/PDI composites with enhanced visible light photoactivity |
title_short |
Rationally designed Sb2S3/PDI composites with enhanced visible light photoactivity |
title_full |
Rationally designed Sb2S3/PDI composites with enhanced visible light photoactivity |
title_fullStr |
Rationally designed Sb2S3/PDI composites with enhanced visible light photoactivity |
title_full_unstemmed |
Rationally designed Sb2S3/PDI composites with enhanced visible light photoactivity |
title_sort |
rationally designed sb2s3/pdi composites with enhanced visible light photoactivity |
publisher |
Elsevier |
publishDate |
2022 |
url |
https://doaj.org/article/ce518838853f40b281ceaa4daa75a5f3 |
work_keys_str_mv |
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