Experimental evidence of plasmarons and effective fine structure constant in electron-doped graphene/h-BN heterostructure

Abstract Electron-electron interaction is fundamental in condensed matter physics and can lead to composite quasiparticles called plasmarons, which strongly renormalize the dispersion and carry information of electron-electron coupling strength as defined by the effective fine structure constant $${...

Descripción completa

Guardado en:
Detalles Bibliográficos
Autores principales: Hongyun Zhang, Shuopei Wang, Eryin Wang, Xiaobo Lu, Qian Li, Changhua Bao, Ke Deng, Haoxiong Zhang, Wei Yao, Guorui Chen, Alexei V. Fedorov, Jonathan D. Denlinger, Kenji Watanabe, Takashi Taniguchi, Guangyu Zhang, Shuyun Zhou
Formato: article
Lenguaje:EN
Publicado: Nature Portfolio 2021
Materias:
Acceso en línea:https://doaj.org/article/cebe098d57f84c03b2c3b710f956c57e
Etiquetas: Agregar Etiqueta
Sin Etiquetas, Sea el primero en etiquetar este registro!
id oai:doaj.org-article:cebe098d57f84c03b2c3b710f956c57e
record_format dspace
spelling oai:doaj.org-article:cebe098d57f84c03b2c3b710f956c57e2021-12-02T17:37:31ZExperimental evidence of plasmarons and effective fine structure constant in electron-doped graphene/h-BN heterostructure10.1038/s41535-021-00386-72397-4648https://doaj.org/article/cebe098d57f84c03b2c3b710f956c57e2021-10-01T00:00:00Zhttps://doi.org/10.1038/s41535-021-00386-7https://doaj.org/toc/2397-4648Abstract Electron-electron interaction is fundamental in condensed matter physics and can lead to composite quasiparticles called plasmarons, which strongly renormalize the dispersion and carry information of electron-electron coupling strength as defined by the effective fine structure constant $${\alpha }_{ee}^{* }$$ α e e * . Although h-BN with unique dielectric properties has been widely used as an important substrate for graphene, so far there is no experimental report of plasmarons in graphene/h-BN yet. Here, we report direct experimental observation of plasmaron dispersion in graphene/h-BN heterostructures through angle-resolved photoemission spectroscopy (ARPES) measurements upon in situ electron doping. Characteristic diamond-shaped dispersion is observed near the Dirac cone in both 0° (aligned) and 13.5° (twisted) graphene/h-BN, and the electron-electron interaction strength $${\alpha }_{ee}^{* }$$ α e e * is extracted to be $${\alpha }_{ee}^{* }\approx 0.9\pm 0.1$$ α e e * ≈ 0.9 ± 0.1 , highlighting the important role of electron-electron interaction. Our results suggest graphene/h-BN as an ideal platform for investigating strong electron-electron interaction with weak dielectric screening, and lays fundamental physics for gate-tunable nano-electronics and nano-plasmonics.Hongyun ZhangShuopei WangEryin WangXiaobo LuQian LiChanghua BaoKe DengHaoxiong ZhangWei YaoGuorui ChenAlexei V. FedorovJonathan D. DenlingerKenji WatanabeTakashi TaniguchiGuangyu ZhangShuyun ZhouNature PortfolioarticleMaterials of engineering and construction. Mechanics of materialsTA401-492Atomic physics. Constitution and properties of matterQC170-197ENnpj Quantum Materials, Vol 6, Iss 1, Pp 1-7 (2021)
institution DOAJ
collection DOAJ
language EN
topic Materials of engineering and construction. Mechanics of materials
TA401-492
Atomic physics. Constitution and properties of matter
QC170-197
spellingShingle Materials of engineering and construction. Mechanics of materials
TA401-492
Atomic physics. Constitution and properties of matter
QC170-197
Hongyun Zhang
Shuopei Wang
Eryin Wang
Xiaobo Lu
Qian Li
Changhua Bao
Ke Deng
Haoxiong Zhang
Wei Yao
Guorui Chen
Alexei V. Fedorov
Jonathan D. Denlinger
Kenji Watanabe
Takashi Taniguchi
Guangyu Zhang
Shuyun Zhou
Experimental evidence of plasmarons and effective fine structure constant in electron-doped graphene/h-BN heterostructure
description Abstract Electron-electron interaction is fundamental in condensed matter physics and can lead to composite quasiparticles called plasmarons, which strongly renormalize the dispersion and carry information of electron-electron coupling strength as defined by the effective fine structure constant $${\alpha }_{ee}^{* }$$ α e e * . Although h-BN with unique dielectric properties has been widely used as an important substrate for graphene, so far there is no experimental report of plasmarons in graphene/h-BN yet. Here, we report direct experimental observation of plasmaron dispersion in graphene/h-BN heterostructures through angle-resolved photoemission spectroscopy (ARPES) measurements upon in situ electron doping. Characteristic diamond-shaped dispersion is observed near the Dirac cone in both 0° (aligned) and 13.5° (twisted) graphene/h-BN, and the electron-electron interaction strength $${\alpha }_{ee}^{* }$$ α e e * is extracted to be $${\alpha }_{ee}^{* }\approx 0.9\pm 0.1$$ α e e * ≈ 0.9 ± 0.1 , highlighting the important role of electron-electron interaction. Our results suggest graphene/h-BN as an ideal platform for investigating strong electron-electron interaction with weak dielectric screening, and lays fundamental physics for gate-tunable nano-electronics and nano-plasmonics.
format article
author Hongyun Zhang
Shuopei Wang
Eryin Wang
Xiaobo Lu
Qian Li
Changhua Bao
Ke Deng
Haoxiong Zhang
Wei Yao
Guorui Chen
Alexei V. Fedorov
Jonathan D. Denlinger
Kenji Watanabe
Takashi Taniguchi
Guangyu Zhang
Shuyun Zhou
author_facet Hongyun Zhang
Shuopei Wang
Eryin Wang
Xiaobo Lu
Qian Li
Changhua Bao
Ke Deng
Haoxiong Zhang
Wei Yao
Guorui Chen
Alexei V. Fedorov
Jonathan D. Denlinger
Kenji Watanabe
Takashi Taniguchi
Guangyu Zhang
Shuyun Zhou
author_sort Hongyun Zhang
title Experimental evidence of plasmarons and effective fine structure constant in electron-doped graphene/h-BN heterostructure
title_short Experimental evidence of plasmarons and effective fine structure constant in electron-doped graphene/h-BN heterostructure
title_full Experimental evidence of plasmarons and effective fine structure constant in electron-doped graphene/h-BN heterostructure
title_fullStr Experimental evidence of plasmarons and effective fine structure constant in electron-doped graphene/h-BN heterostructure
title_full_unstemmed Experimental evidence of plasmarons and effective fine structure constant in electron-doped graphene/h-BN heterostructure
title_sort experimental evidence of plasmarons and effective fine structure constant in electron-doped graphene/h-bn heterostructure
publisher Nature Portfolio
publishDate 2021
url https://doaj.org/article/cebe098d57f84c03b2c3b710f956c57e
work_keys_str_mv AT hongyunzhang experimentalevidenceofplasmaronsandeffectivefinestructureconstantinelectrondopedgraphenehbnheterostructure
AT shuopeiwang experimentalevidenceofplasmaronsandeffectivefinestructureconstantinelectrondopedgraphenehbnheterostructure
AT eryinwang experimentalevidenceofplasmaronsandeffectivefinestructureconstantinelectrondopedgraphenehbnheterostructure
AT xiaobolu experimentalevidenceofplasmaronsandeffectivefinestructureconstantinelectrondopedgraphenehbnheterostructure
AT qianli experimentalevidenceofplasmaronsandeffectivefinestructureconstantinelectrondopedgraphenehbnheterostructure
AT changhuabao experimentalevidenceofplasmaronsandeffectivefinestructureconstantinelectrondopedgraphenehbnheterostructure
AT kedeng experimentalevidenceofplasmaronsandeffectivefinestructureconstantinelectrondopedgraphenehbnheterostructure
AT haoxiongzhang experimentalevidenceofplasmaronsandeffectivefinestructureconstantinelectrondopedgraphenehbnheterostructure
AT weiyao experimentalevidenceofplasmaronsandeffectivefinestructureconstantinelectrondopedgraphenehbnheterostructure
AT guoruichen experimentalevidenceofplasmaronsandeffectivefinestructureconstantinelectrondopedgraphenehbnheterostructure
AT alexeivfedorov experimentalevidenceofplasmaronsandeffectivefinestructureconstantinelectrondopedgraphenehbnheterostructure
AT jonathanddenlinger experimentalevidenceofplasmaronsandeffectivefinestructureconstantinelectrondopedgraphenehbnheterostructure
AT kenjiwatanabe experimentalevidenceofplasmaronsandeffectivefinestructureconstantinelectrondopedgraphenehbnheterostructure
AT takashitaniguchi experimentalevidenceofplasmaronsandeffectivefinestructureconstantinelectrondopedgraphenehbnheterostructure
AT guangyuzhang experimentalevidenceofplasmaronsandeffectivefinestructureconstantinelectrondopedgraphenehbnheterostructure
AT shuyunzhou experimentalevidenceofplasmaronsandeffectivefinestructureconstantinelectrondopedgraphenehbnheterostructure
_version_ 1718379910027804672