Experimental evidence of plasmarons and effective fine structure constant in electron-doped graphene/h-BN heterostructure
Abstract Electron-electron interaction is fundamental in condensed matter physics and can lead to composite quasiparticles called plasmarons, which strongly renormalize the dispersion and carry information of electron-electron coupling strength as defined by the effective fine structure constant $${...
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2021
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oai:doaj.org-article:cebe098d57f84c03b2c3b710f956c57e2021-12-02T17:37:31ZExperimental evidence of plasmarons and effective fine structure constant in electron-doped graphene/h-BN heterostructure10.1038/s41535-021-00386-72397-4648https://doaj.org/article/cebe098d57f84c03b2c3b710f956c57e2021-10-01T00:00:00Zhttps://doi.org/10.1038/s41535-021-00386-7https://doaj.org/toc/2397-4648Abstract Electron-electron interaction is fundamental in condensed matter physics and can lead to composite quasiparticles called plasmarons, which strongly renormalize the dispersion and carry information of electron-electron coupling strength as defined by the effective fine structure constant $${\alpha }_{ee}^{* }$$ α e e * . Although h-BN with unique dielectric properties has been widely used as an important substrate for graphene, so far there is no experimental report of plasmarons in graphene/h-BN yet. Here, we report direct experimental observation of plasmaron dispersion in graphene/h-BN heterostructures through angle-resolved photoemission spectroscopy (ARPES) measurements upon in situ electron doping. Characteristic diamond-shaped dispersion is observed near the Dirac cone in both 0° (aligned) and 13.5° (twisted) graphene/h-BN, and the electron-electron interaction strength $${\alpha }_{ee}^{* }$$ α e e * is extracted to be $${\alpha }_{ee}^{* }\approx 0.9\pm 0.1$$ α e e * ≈ 0.9 ± 0.1 , highlighting the important role of electron-electron interaction. Our results suggest graphene/h-BN as an ideal platform for investigating strong electron-electron interaction with weak dielectric screening, and lays fundamental physics for gate-tunable nano-electronics and nano-plasmonics.Hongyun ZhangShuopei WangEryin WangXiaobo LuQian LiChanghua BaoKe DengHaoxiong ZhangWei YaoGuorui ChenAlexei V. FedorovJonathan D. DenlingerKenji WatanabeTakashi TaniguchiGuangyu ZhangShuyun ZhouNature PortfolioarticleMaterials of engineering and construction. Mechanics of materialsTA401-492Atomic physics. Constitution and properties of matterQC170-197ENnpj Quantum Materials, Vol 6, Iss 1, Pp 1-7 (2021) |
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Materials of engineering and construction. Mechanics of materials TA401-492 Atomic physics. Constitution and properties of matter QC170-197 |
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Materials of engineering and construction. Mechanics of materials TA401-492 Atomic physics. Constitution and properties of matter QC170-197 Hongyun Zhang Shuopei Wang Eryin Wang Xiaobo Lu Qian Li Changhua Bao Ke Deng Haoxiong Zhang Wei Yao Guorui Chen Alexei V. Fedorov Jonathan D. Denlinger Kenji Watanabe Takashi Taniguchi Guangyu Zhang Shuyun Zhou Experimental evidence of plasmarons and effective fine structure constant in electron-doped graphene/h-BN heterostructure |
description |
Abstract Electron-electron interaction is fundamental in condensed matter physics and can lead to composite quasiparticles called plasmarons, which strongly renormalize the dispersion and carry information of electron-electron coupling strength as defined by the effective fine structure constant $${\alpha }_{ee}^{* }$$ α e e * . Although h-BN with unique dielectric properties has been widely used as an important substrate for graphene, so far there is no experimental report of plasmarons in graphene/h-BN yet. Here, we report direct experimental observation of plasmaron dispersion in graphene/h-BN heterostructures through angle-resolved photoemission spectroscopy (ARPES) measurements upon in situ electron doping. Characteristic diamond-shaped dispersion is observed near the Dirac cone in both 0° (aligned) and 13.5° (twisted) graphene/h-BN, and the electron-electron interaction strength $${\alpha }_{ee}^{* }$$ α e e * is extracted to be $${\alpha }_{ee}^{* }\approx 0.9\pm 0.1$$ α e e * ≈ 0.9 ± 0.1 , highlighting the important role of electron-electron interaction. Our results suggest graphene/h-BN as an ideal platform for investigating strong electron-electron interaction with weak dielectric screening, and lays fundamental physics for gate-tunable nano-electronics and nano-plasmonics. |
format |
article |
author |
Hongyun Zhang Shuopei Wang Eryin Wang Xiaobo Lu Qian Li Changhua Bao Ke Deng Haoxiong Zhang Wei Yao Guorui Chen Alexei V. Fedorov Jonathan D. Denlinger Kenji Watanabe Takashi Taniguchi Guangyu Zhang Shuyun Zhou |
author_facet |
Hongyun Zhang Shuopei Wang Eryin Wang Xiaobo Lu Qian Li Changhua Bao Ke Deng Haoxiong Zhang Wei Yao Guorui Chen Alexei V. Fedorov Jonathan D. Denlinger Kenji Watanabe Takashi Taniguchi Guangyu Zhang Shuyun Zhou |
author_sort |
Hongyun Zhang |
title |
Experimental evidence of plasmarons and effective fine structure constant in electron-doped graphene/h-BN heterostructure |
title_short |
Experimental evidence of plasmarons and effective fine structure constant in electron-doped graphene/h-BN heterostructure |
title_full |
Experimental evidence of plasmarons and effective fine structure constant in electron-doped graphene/h-BN heterostructure |
title_fullStr |
Experimental evidence of plasmarons and effective fine structure constant in electron-doped graphene/h-BN heterostructure |
title_full_unstemmed |
Experimental evidence of plasmarons and effective fine structure constant in electron-doped graphene/h-BN heterostructure |
title_sort |
experimental evidence of plasmarons and effective fine structure constant in electron-doped graphene/h-bn heterostructure |
publisher |
Nature Portfolio |
publishDate |
2021 |
url |
https://doaj.org/article/cebe098d57f84c03b2c3b710f956c57e |
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