In situ spectroscopy-guided engineering of rhodium single-atom catalysts for CO oxidation

Single-atom catalysts have been studied for CO oxidation, but experimental in situ investigations are limited. Here, the authors use a suite of in situ/operando spectroscopy to identify key intermediates and define design principles to enhance the CO oxidation activity of atomically dispersed Rh on...

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Autores principales:	Max J. Hülsey, Bin Zhang, Zhirui Ma, Hiroyuki Asakura, David A. Do, Wei Chen, Tsunehiro Tanaka, Peng Zhang, Zili Wu, Ning Yan
Formato:	article
Lenguaje:	EN
Publicado:	Nature Portfolio 2019
Materias:	Science Q
Acceso en línea:	https://doaj.org/article/cf99b37cbf1644d5b393e4b9677a36d3
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spelling	oai:doaj.org-article:cf99b37cbf1644d5b393e4b9677a36d32021-12-02T17:31:52ZIn situ spectroscopy-guided engineering of rhodium single-atom catalysts for CO oxidation10.1038/s41467-019-09188-92041-1723https://doaj.org/article/cf99b37cbf1644d5b393e4b9677a36d32019-03-01T00:00:00Zhttps://doi.org/10.1038/s41467-019-09188-9https://doaj.org/toc/2041-1723Single-atom catalysts have been studied for CO oxidation, but experimental in situ investigations are limited. Here, the authors use a suite of in situ/operando spectroscopy to identify key intermediates and define design principles to enhance the CO oxidation activity of atomically dispersed Rh on heteropoly acids.Max J. HülseyBin ZhangZhirui MaHiroyuki AsakuraDavid A. DoWei ChenTsunehiro TanakaPeng ZhangZili WuNing YanNature PortfolioarticleScienceQENNature Communications, Vol 10, Iss 1, Pp 1-10 (2019)
institution	DOAJ
collection	DOAJ
language	EN
topic	Science Q
spellingShingle	Science Q Max J. Hülsey Bin Zhang Zhirui Ma Hiroyuki Asakura David A. Do Wei Chen Tsunehiro Tanaka Peng Zhang Zili Wu Ning Yan In situ spectroscopy-guided engineering of rhodium single-atom catalysts for CO oxidation
description	Single-atom catalysts have been studied for CO oxidation, but experimental in situ investigations are limited. Here, the authors use a suite of in situ/operando spectroscopy to identify key intermediates and define design principles to enhance the CO oxidation activity of atomically dispersed Rh on heteropoly acids.
format	article
author	Max J. Hülsey Bin Zhang Zhirui Ma Hiroyuki Asakura David A. Do Wei Chen Tsunehiro Tanaka Peng Zhang Zili Wu Ning Yan
author_facet	Max J. Hülsey Bin Zhang Zhirui Ma Hiroyuki Asakura David A. Do Wei Chen Tsunehiro Tanaka Peng Zhang Zili Wu Ning Yan
author_sort	Max J. Hülsey
title	In situ spectroscopy-guided engineering of rhodium single-atom catalysts for CO oxidation
title_short	In situ spectroscopy-guided engineering of rhodium single-atom catalysts for CO oxidation
title_full	In situ spectroscopy-guided engineering of rhodium single-atom catalysts for CO oxidation
title_fullStr	In situ spectroscopy-guided engineering of rhodium single-atom catalysts for CO oxidation
title_full_unstemmed	In situ spectroscopy-guided engineering of rhodium single-atom catalysts for CO oxidation
title_sort	in situ spectroscopy-guided engineering of rhodium single-atom catalysts for co oxidation
publisher	Nature Portfolio
publishDate	2019
url	https://doaj.org/article/cf99b37cbf1644d5b393e4b9677a36d3
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In situ spectroscopy-guided engineering of rhodium single-atom catalysts for CO oxidation

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