Phase stabilization by electronic entropy in plutonium
Plutonium has strong electronic correlations, which makes it difficult to establish microscopic understanding of the complicated structural phase diagram. Here the authors identify an electronic contribution to the entropy that stabilises the δ-Pu phase.
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Nature Portfolio
2019
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oai:doaj.org-article:d17b4055c3b54cf197d93be0ec851a3d2021-12-02T15:35:32ZPhase stabilization by electronic entropy in plutonium10.1038/s41467-019-11166-02041-1723https://doaj.org/article/d17b4055c3b54cf197d93be0ec851a3d2019-07-01T00:00:00Zhttps://doi.org/10.1038/s41467-019-11166-0https://doaj.org/toc/2041-1723Plutonium has strong electronic correlations, which makes it difficult to establish microscopic understanding of the complicated structural phase diagram. Here the authors identify an electronic contribution to the entropy that stabilises the δ-Pu phase.N. HarrisonJ. B. BettsM. R. WartenbeF. F. BalakirevS. RichmondM. JaimeP. H. TobashNature PortfolioarticleScienceQENNature Communications, Vol 10, Iss 1, Pp 1-9 (2019) |
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Science Q N. Harrison J. B. Betts M. R. Wartenbe F. F. Balakirev S. Richmond M. Jaime P. H. Tobash Phase stabilization by electronic entropy in plutonium |
description |
Plutonium has strong electronic correlations, which makes it difficult to establish microscopic understanding of the complicated structural phase diagram. Here the authors identify an electronic contribution to the entropy that stabilises the δ-Pu phase. |
format |
article |
author |
N. Harrison J. B. Betts M. R. Wartenbe F. F. Balakirev S. Richmond M. Jaime P. H. Tobash |
author_facet |
N. Harrison J. B. Betts M. R. Wartenbe F. F. Balakirev S. Richmond M. Jaime P. H. Tobash |
author_sort |
N. Harrison |
title |
Phase stabilization by electronic entropy in plutonium |
title_short |
Phase stabilization by electronic entropy in plutonium |
title_full |
Phase stabilization by electronic entropy in plutonium |
title_fullStr |
Phase stabilization by electronic entropy in plutonium |
title_full_unstemmed |
Phase stabilization by electronic entropy in plutonium |
title_sort |
phase stabilization by electronic entropy in plutonium |
publisher |
Nature Portfolio |
publishDate |
2019 |
url |
https://doaj.org/article/d17b4055c3b54cf197d93be0ec851a3d |
work_keys_str_mv |
AT nharrison phasestabilizationbyelectronicentropyinplutonium AT jbbetts phasestabilizationbyelectronicentropyinplutonium AT mrwartenbe phasestabilizationbyelectronicentropyinplutonium AT ffbalakirev phasestabilizationbyelectronicentropyinplutonium AT srichmond phasestabilizationbyelectronicentropyinplutonium AT mjaime phasestabilizationbyelectronicentropyinplutonium AT phtobash phasestabilizationbyelectronicentropyinplutonium |
_version_ |
1718386562982477824 |