Heterogeneous Fe3 single-cluster catalyst for ammonia synthesis via an associative mechanism

The current industrial ammonia synthesis relies on the Haber-Bosch process that is limited by the Brønsted–Evans–Polanyi relation. Here, the authors propose a new strategy that an anchored Fe3 on θ-Al2O3(010) surface serves as a heterogeneous single cluster catalyst for ammonia synthesis from first-...

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Autores principales:	Jin-Cheng Liu, Xue-Lu Ma, Yong Li, Yang-Gang Wang, Hai Xiao, Jun Li
Formato:	article
Lenguaje:	EN
Publicado:	Nature Portfolio 2018
Materias:	Science Q
Acceso en línea:	https://doaj.org/article/d1d7475fdcac4f8aae74d934a892b071
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id	oai:doaj.org-article:d1d7475fdcac4f8aae74d934a892b071
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spelling	oai:doaj.org-article:d1d7475fdcac4f8aae74d934a892b0712021-12-02T16:49:22ZHeterogeneous Fe3 single-cluster catalyst for ammonia synthesis via an associative mechanism10.1038/s41467-018-03795-82041-1723https://doaj.org/article/d1d7475fdcac4f8aae74d934a892b0712018-04-01T00:00:00Zhttps://doi.org/10.1038/s41467-018-03795-8https://doaj.org/toc/2041-1723The current industrial ammonia synthesis relies on the Haber-Bosch process that is limited by the Brønsted–Evans–Polanyi relation. Here, the authors propose a new strategy that an anchored Fe3 on θ-Al2O3(010) surface serves as a heterogeneous single cluster catalyst for ammonia synthesis from first-principles calculations and microkinetic analysis.Jin-Cheng LiuXue-Lu MaYong LiYang-Gang WangHai XiaoJun LiNature PortfolioarticleScienceQENNature Communications, Vol 9, Iss 1, Pp 1-9 (2018)
institution	DOAJ
collection	DOAJ
language	EN
topic	Science Q
spellingShingle	Science Q Jin-Cheng Liu Xue-Lu Ma Yong Li Yang-Gang Wang Hai Xiao Jun Li Heterogeneous Fe3 single-cluster catalyst for ammonia synthesis via an associative mechanism
description	The current industrial ammonia synthesis relies on the Haber-Bosch process that is limited by the Brønsted–Evans–Polanyi relation. Here, the authors propose a new strategy that an anchored Fe3 on θ-Al2O3(010) surface serves as a heterogeneous single cluster catalyst for ammonia synthesis from first-principles calculations and microkinetic analysis.
format	article
author	Jin-Cheng Liu Xue-Lu Ma Yong Li Yang-Gang Wang Hai Xiao Jun Li
author_facet	Jin-Cheng Liu Xue-Lu Ma Yong Li Yang-Gang Wang Hai Xiao Jun Li
author_sort	Jin-Cheng Liu
title	Heterogeneous Fe3 single-cluster catalyst for ammonia synthesis via an associative mechanism
title_short	Heterogeneous Fe3 single-cluster catalyst for ammonia synthesis via an associative mechanism
title_full	Heterogeneous Fe3 single-cluster catalyst for ammonia synthesis via an associative mechanism
title_fullStr	Heterogeneous Fe3 single-cluster catalyst for ammonia synthesis via an associative mechanism
title_full_unstemmed	Heterogeneous Fe3 single-cluster catalyst for ammonia synthesis via an associative mechanism
title_sort	heterogeneous fe3 single-cluster catalyst for ammonia synthesis via an associative mechanism
publisher	Nature Portfolio
publishDate	2018
url	https://doaj.org/article/d1d7475fdcac4f8aae74d934a892b071
work_keys_str_mv	AT jinchengliu heterogeneousfe3singleclustercatalystforammoniasynthesisviaanassociativemechanism AT xueluma heterogeneousfe3singleclustercatalystforammoniasynthesisviaanassociativemechanism AT yongli heterogeneousfe3singleclustercatalystforammoniasynthesisviaanassociativemechanism AT yanggangwang heterogeneousfe3singleclustercatalystforammoniasynthesisviaanassociativemechanism AT haixiao heterogeneousfe3singleclustercatalystforammoniasynthesisviaanassociativemechanism AT junli heterogeneousfe3singleclustercatalystforammoniasynthesisviaanassociativemechanism
_version_	1718383364939972608

Heterogeneous Fe3 single-cluster catalyst for ammonia synthesis via an associative mechanism

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