Improving Photocatalytic Performance from Bi2WO6@MoS2/graphene Hybrids via Gradual Charge Transferred Pathway
Abstract The charge transfer from the main catalyst to the cocatalyst is a key factor to enhance catalytic activity for photocatalytic nanocomposite materials. In order to enhance the charge transfer between Bi2WO6 and graphene, we inlet MoS2 as a “stepping-stone” into Bi2WO6 and graphene. Here, we...
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Nature Portfolio
2017
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oai:doaj.org-article:d7a4f88032f0479a8b9b3fdf991cbe3d2021-12-02T16:06:31ZImproving Photocatalytic Performance from Bi2WO6@MoS2/graphene Hybrids via Gradual Charge Transferred Pathway10.1038/s41598-017-03911-62045-2322https://doaj.org/article/d7a4f88032f0479a8b9b3fdf991cbe3d2017-06-01T00:00:00Zhttps://doi.org/10.1038/s41598-017-03911-6https://doaj.org/toc/2045-2322Abstract The charge transfer from the main catalyst to the cocatalyst is a key factor to enhance catalytic activity for photocatalytic nanocomposite materials. In order to enhance the charge transfer between Bi2WO6 and graphene, we inlet MoS2 as a “stepping-stone” into Bi2WO6 and graphene. Here, we report an effective strategy to synthesize ternary Bi2WO6@MoS2/graphene nanocomposite photocatalyst by a facile two-step hydrothermal method, which is afforded by assembling two cocatalysts, graphene and MoS2, into the Bi2WO6 matrix with a nanoparticle morphology as a visible light harvester. Compared with Bi2WO6/graphene, Bi2WO6/MoS2 and pure Bi2WO6, the Bi2WO6@MoS2/graphene ternary composites exhibit superior photocatalytic activity owing to an enhanced charge carrier separation via gradual charge transferred pathway. This work indicates a promising cocatalyst strategy for designing a more efficient graphene based semiconductor photocatalyst toward degradation of organic pollutants.Ming LiuXin XueShansheng YuXiaoyi WangXiaoying HuHongwei TianHong ChenWeitao ZhengNature PortfolioarticleMedicineRScienceQENScientific Reports, Vol 7, Iss 1, Pp 1-11 (2017) |
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Medicine R Science Q Ming Liu Xin Xue Shansheng Yu Xiaoyi Wang Xiaoying Hu Hongwei Tian Hong Chen Weitao Zheng Improving Photocatalytic Performance from Bi2WO6@MoS2/graphene Hybrids via Gradual Charge Transferred Pathway |
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Abstract The charge transfer from the main catalyst to the cocatalyst is a key factor to enhance catalytic activity for photocatalytic nanocomposite materials. In order to enhance the charge transfer between Bi2WO6 and graphene, we inlet MoS2 as a “stepping-stone” into Bi2WO6 and graphene. Here, we report an effective strategy to synthesize ternary Bi2WO6@MoS2/graphene nanocomposite photocatalyst by a facile two-step hydrothermal method, which is afforded by assembling two cocatalysts, graphene and MoS2, into the Bi2WO6 matrix with a nanoparticle morphology as a visible light harvester. Compared with Bi2WO6/graphene, Bi2WO6/MoS2 and pure Bi2WO6, the Bi2WO6@MoS2/graphene ternary composites exhibit superior photocatalytic activity owing to an enhanced charge carrier separation via gradual charge transferred pathway. This work indicates a promising cocatalyst strategy for designing a more efficient graphene based semiconductor photocatalyst toward degradation of organic pollutants. |
format |
article |
author |
Ming Liu Xin Xue Shansheng Yu Xiaoyi Wang Xiaoying Hu Hongwei Tian Hong Chen Weitao Zheng |
author_facet |
Ming Liu Xin Xue Shansheng Yu Xiaoyi Wang Xiaoying Hu Hongwei Tian Hong Chen Weitao Zheng |
author_sort |
Ming Liu |
title |
Improving Photocatalytic Performance from Bi2WO6@MoS2/graphene Hybrids via Gradual Charge Transferred Pathway |
title_short |
Improving Photocatalytic Performance from Bi2WO6@MoS2/graphene Hybrids via Gradual Charge Transferred Pathway |
title_full |
Improving Photocatalytic Performance from Bi2WO6@MoS2/graphene Hybrids via Gradual Charge Transferred Pathway |
title_fullStr |
Improving Photocatalytic Performance from Bi2WO6@MoS2/graphene Hybrids via Gradual Charge Transferred Pathway |
title_full_unstemmed |
Improving Photocatalytic Performance from Bi2WO6@MoS2/graphene Hybrids via Gradual Charge Transferred Pathway |
title_sort |
improving photocatalytic performance from bi2wo6@mos2/graphene hybrids via gradual charge transferred pathway |
publisher |
Nature Portfolio |
publishDate |
2017 |
url |
https://doaj.org/article/d7a4f88032f0479a8b9b3fdf991cbe3d |
work_keys_str_mv |
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