Vibrational fingerprint of localized excitons in a two-dimensional metal-organic crystal

Long-lived excitons in a two-dimensional metal-organic crystal can be produced by visible light and detected by infrared radiation. Here, the authors show that the excitonic state of a biomimetic macrocycle can be ‘read’ by measuring the vibrations of an adsorbed ligand.

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Detalles Bibliográficos
Autores principales: M. Corva, A. Ferrari, M. Rinaldi, Z. Feng, M. Roiaz, C. Rameshan, G. Rupprechter, R. Costantini, M. Dell’Angela, G. Pastore, G. Comelli, N. Seriani, E. Vesselli
Formato: article
Lenguaje:EN
Publicado: Nature Portfolio 2018
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Acceso en línea:https://doaj.org/article/d8a4633d2c8a496ca78116f1b5bb73cd
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Descripción
Sumario:Long-lived excitons in a two-dimensional metal-organic crystal can be produced by visible light and detected by infrared radiation. Here, the authors show that the excitonic state of a biomimetic macrocycle can be ‘read’ by measuring the vibrations of an adsorbed ligand.