Manipulation of hot carrier cooling dynamics in two-dimensional Dion–Jacobson hybrid perovskites via Rashba band splitting

Hybrid perovskite is a promising class of material for optoelectronic applications due to the slow hot-carrier cooling, yet the process is not well-understood in material with Rashba band splitting. Here, the authors reveal spin-flipping and spin-dependent scattering of hot electrons are responsible...

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Autores principales: Jun Yin, Rounak Naphade, Partha Maity, Luis Gutiérrez-Arzaluz, Dhaifallah Almalawi, Iman S. Roqan, Jean-Luc Brédas, Osman M. Bakr, Omar F. Mohammed
Formato: article
Lenguaje:EN
Publicado: Nature Portfolio 2021
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Acceso en línea:https://doaj.org/article/da5d9a4741f34f75a4c06312ce2f79e1
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Sumario:Hybrid perovskite is a promising class of material for optoelectronic applications due to the slow hot-carrier cooling, yet the process is not well-understood in material with Rashba band splitting. Here, the authors reveal spin-flipping and spin-dependent scattering of hot electrons are responsible for accelerating the cooling at longer delays.