Tuning Pt-CeO2 interactions by high-temperature vapor-phase synthesis for improved reducibility of lattice oxygen

While single-atom catalysts (SACs) have attracted a lot of interest, the nature of the active sites in SACs remains elusive. Here the authors elucidate that depositing single atoms via high temperature synthesis leads to improved reducibility of lattice oxygen on CeO2 yielding low temperature reacti...

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Autores principales:	Xavier Isidro Pereira-Hernández, Andrew DeLaRiva, Valery Muravev, Deepak Kunwar, Haifeng Xiong, Berlin Sudduth, Mark Engelhard, Libor Kovarik, Emiel J. M. Hensen, Yong Wang, Abhaya K. Datye
Formato:	article
Lenguaje:	EN
Publicado:	Nature Portfolio 2019
Materias:	Science Q
Acceso en línea:	https://doaj.org/article/dd453ed979024f8fae1ce776afd07803
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spelling	oai:doaj.org-article:dd453ed979024f8fae1ce776afd078032021-12-02T17:32:10ZTuning Pt-CeO2 interactions by high-temperature vapor-phase synthesis for improved reducibility of lattice oxygen10.1038/s41467-019-09308-52041-1723https://doaj.org/article/dd453ed979024f8fae1ce776afd078032019-03-01T00:00:00Zhttps://doi.org/10.1038/s41467-019-09308-5https://doaj.org/toc/2041-1723While single-atom catalysts (SACs) have attracted a lot of interest, the nature of the active sites in SACs remains elusive. Here the authors elucidate that depositing single atoms via high temperature synthesis leads to improved reducibility of lattice oxygen on CeO2 yielding low temperature reactivity of Pt catalysts in CO oxidation.Xavier Isidro Pereira-HernándezAndrew DeLaRivaValery MuravevDeepak KunwarHaifeng XiongBerlin SudduthMark EngelhardLibor KovarikEmiel J. M. HensenYong WangAbhaya K. DatyeNature PortfolioarticleScienceQENNature Communications, Vol 10, Iss 1, Pp 1-10 (2019)
institution	DOAJ
collection	DOAJ
language	EN
topic	Science Q
spellingShingle	Science Q Xavier Isidro Pereira-Hernández Andrew DeLaRiva Valery Muravev Deepak Kunwar Haifeng Xiong Berlin Sudduth Mark Engelhard Libor Kovarik Emiel J. M. Hensen Yong Wang Abhaya K. Datye Tuning Pt-CeO2 interactions by high-temperature vapor-phase synthesis for improved reducibility of lattice oxygen
description	While single-atom catalysts (SACs) have attracted a lot of interest, the nature of the active sites in SACs remains elusive. Here the authors elucidate that depositing single atoms via high temperature synthesis leads to improved reducibility of lattice oxygen on CeO2 yielding low temperature reactivity of Pt catalysts in CO oxidation.
format	article
author	Xavier Isidro Pereira-Hernández Andrew DeLaRiva Valery Muravev Deepak Kunwar Haifeng Xiong Berlin Sudduth Mark Engelhard Libor Kovarik Emiel J. M. Hensen Yong Wang Abhaya K. Datye
author_facet	Xavier Isidro Pereira-Hernández Andrew DeLaRiva Valery Muravev Deepak Kunwar Haifeng Xiong Berlin Sudduth Mark Engelhard Libor Kovarik Emiel J. M. Hensen Yong Wang Abhaya K. Datye
author_sort	Xavier Isidro Pereira-Hernández
title	Tuning Pt-CeO2 interactions by high-temperature vapor-phase synthesis for improved reducibility of lattice oxygen
title_short	Tuning Pt-CeO2 interactions by high-temperature vapor-phase synthesis for improved reducibility of lattice oxygen
title_full	Tuning Pt-CeO2 interactions by high-temperature vapor-phase synthesis for improved reducibility of lattice oxygen
title_fullStr	Tuning Pt-CeO2 interactions by high-temperature vapor-phase synthesis for improved reducibility of lattice oxygen
title_full_unstemmed	Tuning Pt-CeO2 interactions by high-temperature vapor-phase synthesis for improved reducibility of lattice oxygen
title_sort	tuning pt-ceo2 interactions by high-temperature vapor-phase synthesis for improved reducibility of lattice oxygen
publisher	Nature Portfolio
publishDate	2019
url	https://doaj.org/article/dd453ed979024f8fae1ce776afd07803
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Tuning Pt-CeO2 interactions by high-temperature vapor-phase synthesis for improved reducibility of lattice oxygen

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