Study the plasmonic property of gold nanorods highly above damage threshold via single-pulse spectral hole-burning experiments
Abstract Intense femtosecond laser irradiation reshapes gold nanorods, resulting in a persistent hole in the optical absorption spectrum of the nanorods at the wavelength of the laser. Single-pulse hole-burning experiments were performed in a mixture of nanorods with a broad absorption around 800 nm...
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| Autores principales: | , , |
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| Formato: | article |
| Lenguaje: | EN |
| Publicado: |
Nature Portfolio
2021
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| Materias: | |
| Acceso en línea: | https://doaj.org/article/df0ac019d16143ecbb339d62a4d3a575 |
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| Sumario: | Abstract Intense femtosecond laser irradiation reshapes gold nanorods, resulting in a persistent hole in the optical absorption spectrum of the nanorods at the wavelength of the laser. Single-pulse hole-burning experiments were performed in a mixture of nanorods with a broad absorption around 800 nm with a 35-fs laser with 800 nm wavelength and 6 mJ/pulse. A significant increase in hole burning width at an average fluence of 106 J/m2 has been found, suggesting a tripled damping coefficient of plasmon. This shows that the surface plasmonic effect still occurs at extremely high femtosecond laser fluences just before the nanorods are damaged and the remaining 10% plasmonic enhancement of light is at the fluence of 106 J/m2, which is several orders of magnitude higher than the damage threshold of the gold nanorods. Plasmon–photon interactions may also cause an increase in the damping coefficient. |
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