Resonant X-ray emission spectroscopy from broadband stochastic pulses at an X-ray free electron laser

X-ray absorption and X-ray free electron lasers are important tools to study chemical and structural dynamics, but spectral details like pre-edge features are inherently hard to detect. Here, the authors show that stochastic spectroscopy can yield similar spectral information to monochromatic spectr...

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Autores principales: Franklin D. Fuller, Anton Loukianov, Tsukasa Takanashi, Daehyun You, Yiwen Li, Kiyoshi Ueda, Thomas Fransson, Makina Yabashi, Tetsuo Katayama, Tsu-Chien Weng, Roberto Alonso-Mori, Uwe Bergmann, Jan Kern, Vittal K. Yachandra, Philippe Wernet, Junko Yano
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Lenguaje:EN
Publicado: Nature Portfolio 2021
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Acceso en línea:https://doaj.org/article/e360241e7f52469a966a3346f8fd52ca
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spelling oai:doaj.org-article:e360241e7f52469a966a3346f8fd52ca2021-12-02T17:52:28ZResonant X-ray emission spectroscopy from broadband stochastic pulses at an X-ray free electron laser10.1038/s42004-021-00512-32399-3669https://doaj.org/article/e360241e7f52469a966a3346f8fd52ca2021-06-01T00:00:00Zhttps://doi.org/10.1038/s42004-021-00512-3https://doaj.org/toc/2399-3669X-ray absorption and X-ray free electron lasers are important tools to study chemical and structural dynamics, but spectral details like pre-edge features are inherently hard to detect. Here, the authors show that stochastic spectroscopy can yield similar spectral information to monochromatic spectroscopies, while increasing signal yield and reducing acquisition time.Franklin D. FullerAnton LoukianovTsukasa TakanashiDaehyun YouYiwen LiKiyoshi UedaThomas FranssonMakina YabashiTetsuo KatayamaTsu-Chien WengRoberto Alonso-MoriUwe BergmannJan KernVittal K. YachandraPhilippe WernetJunko YanoNature PortfolioarticleChemistryQD1-999ENCommunications Chemistry, Vol 4, Iss 1, Pp 1-9 (2021)
institution DOAJ
collection DOAJ
language EN
topic Chemistry
QD1-999
spellingShingle Chemistry
QD1-999
Franklin D. Fuller
Anton Loukianov
Tsukasa Takanashi
Daehyun You
Yiwen Li
Kiyoshi Ueda
Thomas Fransson
Makina Yabashi
Tetsuo Katayama
Tsu-Chien Weng
Roberto Alonso-Mori
Uwe Bergmann
Jan Kern
Vittal K. Yachandra
Philippe Wernet
Junko Yano
Resonant X-ray emission spectroscopy from broadband stochastic pulses at an X-ray free electron laser
description X-ray absorption and X-ray free electron lasers are important tools to study chemical and structural dynamics, but spectral details like pre-edge features are inherently hard to detect. Here, the authors show that stochastic spectroscopy can yield similar spectral information to monochromatic spectroscopies, while increasing signal yield and reducing acquisition time.
format article
author Franklin D. Fuller
Anton Loukianov
Tsukasa Takanashi
Daehyun You
Yiwen Li
Kiyoshi Ueda
Thomas Fransson
Makina Yabashi
Tetsuo Katayama
Tsu-Chien Weng
Roberto Alonso-Mori
Uwe Bergmann
Jan Kern
Vittal K. Yachandra
Philippe Wernet
Junko Yano
author_facet Franklin D. Fuller
Anton Loukianov
Tsukasa Takanashi
Daehyun You
Yiwen Li
Kiyoshi Ueda
Thomas Fransson
Makina Yabashi
Tetsuo Katayama
Tsu-Chien Weng
Roberto Alonso-Mori
Uwe Bergmann
Jan Kern
Vittal K. Yachandra
Philippe Wernet
Junko Yano
author_sort Franklin D. Fuller
title Resonant X-ray emission spectroscopy from broadband stochastic pulses at an X-ray free electron laser
title_short Resonant X-ray emission spectroscopy from broadband stochastic pulses at an X-ray free electron laser
title_full Resonant X-ray emission spectroscopy from broadband stochastic pulses at an X-ray free electron laser
title_fullStr Resonant X-ray emission spectroscopy from broadband stochastic pulses at an X-ray free electron laser
title_full_unstemmed Resonant X-ray emission spectroscopy from broadband stochastic pulses at an X-ray free electron laser
title_sort resonant x-ray emission spectroscopy from broadband stochastic pulses at an x-ray free electron laser
publisher Nature Portfolio
publishDate 2021
url https://doaj.org/article/e360241e7f52469a966a3346f8fd52ca
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