Nucleation of Ga droplets self-assembly on GaAs(111)A substrates
Abstract We investigated the nucleation of Ga droplets on singular GaAs(111)A substrates in the view of their use as the seeds for the self-assembled droplet epitaxial quantum dots. A small critical cluster size of 1–2 atoms characterizes the droplet nucleation. Low values of the Hopkins-Skellam ind...
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Nature Portfolio
2021
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oai:doaj.org-article:e373aff5a1c44ae696f1dbad667730712021-12-02T17:04:07ZNucleation of Ga droplets self-assembly on GaAs(111)A substrates10.1038/s41598-021-86339-32045-2322https://doaj.org/article/e373aff5a1c44ae696f1dbad667730712021-03-01T00:00:00Zhttps://doi.org/10.1038/s41598-021-86339-3https://doaj.org/toc/2045-2322Abstract We investigated the nucleation of Ga droplets on singular GaAs(111)A substrates in the view of their use as the seeds for the self-assembled droplet epitaxial quantum dots. A small critical cluster size of 1–2 atoms characterizes the droplet nucleation. Low values of the Hopkins-Skellam index (as low as 0.35) demonstrate a high degree of a spatial order of the droplet ensemble. Around $$350\,^{\circ }\hbox {C}$$ 350 ∘ C the droplet size distribution becomes bimodal. We attribute this observation to the interplay between the local environment and the limitation to the adatom surface diffusion introduced by the Ehrlich–Schwöbel barrier at the terrace edges.Artur TuktamyshevAlexey FedorovSergio BiettiStefano VichiRiccardo TamboneShiro TsukamotoStefano SanguinettiNature PortfolioarticleMedicineRScienceQENScientific Reports, Vol 11, Iss 1, Pp 1-11 (2021) |
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Medicine R Science Q Artur Tuktamyshev Alexey Fedorov Sergio Bietti Stefano Vichi Riccardo Tambone Shiro Tsukamoto Stefano Sanguinetti Nucleation of Ga droplets self-assembly on GaAs(111)A substrates |
description |
Abstract We investigated the nucleation of Ga droplets on singular GaAs(111)A substrates in the view of their use as the seeds for the self-assembled droplet epitaxial quantum dots. A small critical cluster size of 1–2 atoms characterizes the droplet nucleation. Low values of the Hopkins-Skellam index (as low as 0.35) demonstrate a high degree of a spatial order of the droplet ensemble. Around $$350\,^{\circ }\hbox {C}$$ 350 ∘ C the droplet size distribution becomes bimodal. We attribute this observation to the interplay between the local environment and the limitation to the adatom surface diffusion introduced by the Ehrlich–Schwöbel barrier at the terrace edges. |
format |
article |
author |
Artur Tuktamyshev Alexey Fedorov Sergio Bietti Stefano Vichi Riccardo Tambone Shiro Tsukamoto Stefano Sanguinetti |
author_facet |
Artur Tuktamyshev Alexey Fedorov Sergio Bietti Stefano Vichi Riccardo Tambone Shiro Tsukamoto Stefano Sanguinetti |
author_sort |
Artur Tuktamyshev |
title |
Nucleation of Ga droplets self-assembly on GaAs(111)A substrates |
title_short |
Nucleation of Ga droplets self-assembly on GaAs(111)A substrates |
title_full |
Nucleation of Ga droplets self-assembly on GaAs(111)A substrates |
title_fullStr |
Nucleation of Ga droplets self-assembly on GaAs(111)A substrates |
title_full_unstemmed |
Nucleation of Ga droplets self-assembly on GaAs(111)A substrates |
title_sort |
nucleation of ga droplets self-assembly on gaas(111)a substrates |
publisher |
Nature Portfolio |
publishDate |
2021 |
url |
https://doaj.org/article/e373aff5a1c44ae696f1dbad66773071 |
work_keys_str_mv |
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1718381881235341312 |