Doublonlike Excitations and Their Phononic Coupling in a Mott Charge-Density-Wave System
Electron-phonon-driven charge-density waves can in some circumstances allow electronic correlations to become predominant, driving a system into a Mott insulating state. New insight into both the Mott state and preceding charge-density wave may result from observations of the coupled dynamics of the...
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American Physical Society
2021
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oai:doaj.org-article:e3ebd9e40dc9480cb030e6ff03f5afce2021-12-02T13:13:48ZDoublonlike Excitations and Their Phononic Coupling in a Mott Charge-Density-Wave System10.1103/PhysRevX.11.0110592160-3308https://doaj.org/article/e3ebd9e40dc9480cb030e6ff03f5afce2021-03-01T00:00:00Zhttp://doi.org/10.1103/PhysRevX.11.011059http://doi.org/10.1103/PhysRevX.11.011059https://doaj.org/toc/2160-3308Electron-phonon-driven charge-density waves can in some circumstances allow electronic correlations to become predominant, driving a system into a Mott insulating state. New insight into both the Mott state and preceding charge-density wave may result from observations of the coupled dynamics of their underlying degrees of freedom. Here, tunneling injection of single electrons into the upper Hubbard band of the Mott charge-density-wave material 1T-TaS_{2} reveals extraordinarily narrow electronic excitations which couple to amplitude mode phonons associated with the charge-density wave’s periodic lattice distortion. This gives a vivid microscopic view of the interplay between excitations of the Mott state and the lattice dynamics of its charge-density wave precursor.C. J. ButlerM. YoshidaT. HanaguriY. IwasaAmerican Physical SocietyarticlePhysicsQC1-999ENPhysical Review X, Vol 11, Iss 1, p 011059 (2021) |
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Physics QC1-999 |
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Physics QC1-999 C. J. Butler M. Yoshida T. Hanaguri Y. Iwasa Doublonlike Excitations and Their Phononic Coupling in a Mott Charge-Density-Wave System |
description |
Electron-phonon-driven charge-density waves can in some circumstances allow electronic correlations to become predominant, driving a system into a Mott insulating state. New insight into both the Mott state and preceding charge-density wave may result from observations of the coupled dynamics of their underlying degrees of freedom. Here, tunneling injection of single electrons into the upper Hubbard band of the Mott charge-density-wave material 1T-TaS_{2} reveals extraordinarily narrow electronic excitations which couple to amplitude mode phonons associated with the charge-density wave’s periodic lattice distortion. This gives a vivid microscopic view of the interplay between excitations of the Mott state and the lattice dynamics of its charge-density wave precursor. |
format |
article |
author |
C. J. Butler M. Yoshida T. Hanaguri Y. Iwasa |
author_facet |
C. J. Butler M. Yoshida T. Hanaguri Y. Iwasa |
author_sort |
C. J. Butler |
title |
Doublonlike Excitations and Their Phononic Coupling in a Mott Charge-Density-Wave System |
title_short |
Doublonlike Excitations and Their Phononic Coupling in a Mott Charge-Density-Wave System |
title_full |
Doublonlike Excitations and Their Phononic Coupling in a Mott Charge-Density-Wave System |
title_fullStr |
Doublonlike Excitations and Their Phononic Coupling in a Mott Charge-Density-Wave System |
title_full_unstemmed |
Doublonlike Excitations and Their Phononic Coupling in a Mott Charge-Density-Wave System |
title_sort |
doublonlike excitations and their phononic coupling in a mott charge-density-wave system |
publisher |
American Physical Society |
publishDate |
2021 |
url |
https://doaj.org/article/e3ebd9e40dc9480cb030e6ff03f5afce |
work_keys_str_mv |
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