Anomalous metal segregation in lithium-rich material provides design rules for stable cathode in lithium-ion battery

The authors show that after cycling the model cathode material Li2Ru0.5Mn0.5O3 undergoes ruthenium segregation and even exsolution at the reconstructed oxide surface, which triggers a progressive degradation process. The insights enable new dimensions in choosing dopants for stabilized cathode surfa...

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Autores principales: Ruoqian Lin, Enyuan Hu, Mingjie Liu, Yi Wang, Hao Cheng, Jinpeng Wu, Jin-Cheng Zheng, Qin Wu, Seongmin Bak, Xiao Tong, Rui Zhang, Wanli Yang, Kristin A. Persson, Xiqian Yu, Xiao-Qing Yang, Huolin L. Xin
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Lenguaje:EN
Publicado: Nature Portfolio 2019
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Acceso en línea:https://doaj.org/article/e8ded79027d84f6fb4ccf35a3214684b
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spelling oai:doaj.org-article:e8ded79027d84f6fb4ccf35a3214684b2021-12-02T15:35:58ZAnomalous metal segregation in lithium-rich material provides design rules for stable cathode in lithium-ion battery10.1038/s41467-019-09248-02041-1723https://doaj.org/article/e8ded79027d84f6fb4ccf35a3214684b2019-04-01T00:00:00Zhttps://doi.org/10.1038/s41467-019-09248-0https://doaj.org/toc/2041-1723The authors show that after cycling the model cathode material Li2Ru0.5Mn0.5O3 undergoes ruthenium segregation and even exsolution at the reconstructed oxide surface, which triggers a progressive degradation process. The insights enable new dimensions in choosing dopants for stabilized cathode surface.Ruoqian LinEnyuan HuMingjie LiuYi WangHao ChengJinpeng WuJin-Cheng ZhengQin WuSeongmin BakXiao TongRui ZhangWanli YangKristin A. PerssonXiqian YuXiao-Qing YangHuolin L. XinNature PortfolioarticleScienceQENNature Communications, Vol 10, Iss 1, Pp 1-11 (2019)
institution DOAJ
collection DOAJ
language EN
topic Science
Q
spellingShingle Science
Q
Ruoqian Lin
Enyuan Hu
Mingjie Liu
Yi Wang
Hao Cheng
Jinpeng Wu
Jin-Cheng Zheng
Qin Wu
Seongmin Bak
Xiao Tong
Rui Zhang
Wanli Yang
Kristin A. Persson
Xiqian Yu
Xiao-Qing Yang
Huolin L. Xin
Anomalous metal segregation in lithium-rich material provides design rules for stable cathode in lithium-ion battery
description The authors show that after cycling the model cathode material Li2Ru0.5Mn0.5O3 undergoes ruthenium segregation and even exsolution at the reconstructed oxide surface, which triggers a progressive degradation process. The insights enable new dimensions in choosing dopants for stabilized cathode surface.
format article
author Ruoqian Lin
Enyuan Hu
Mingjie Liu
Yi Wang
Hao Cheng
Jinpeng Wu
Jin-Cheng Zheng
Qin Wu
Seongmin Bak
Xiao Tong
Rui Zhang
Wanli Yang
Kristin A. Persson
Xiqian Yu
Xiao-Qing Yang
Huolin L. Xin
author_facet Ruoqian Lin
Enyuan Hu
Mingjie Liu
Yi Wang
Hao Cheng
Jinpeng Wu
Jin-Cheng Zheng
Qin Wu
Seongmin Bak
Xiao Tong
Rui Zhang
Wanli Yang
Kristin A. Persson
Xiqian Yu
Xiao-Qing Yang
Huolin L. Xin
author_sort Ruoqian Lin
title Anomalous metal segregation in lithium-rich material provides design rules for stable cathode in lithium-ion battery
title_short Anomalous metal segregation in lithium-rich material provides design rules for stable cathode in lithium-ion battery
title_full Anomalous metal segregation in lithium-rich material provides design rules for stable cathode in lithium-ion battery
title_fullStr Anomalous metal segregation in lithium-rich material provides design rules for stable cathode in lithium-ion battery
title_full_unstemmed Anomalous metal segregation in lithium-rich material provides design rules for stable cathode in lithium-ion battery
title_sort anomalous metal segregation in lithium-rich material provides design rules for stable cathode in lithium-ion battery
publisher Nature Portfolio
publishDate 2019
url https://doaj.org/article/e8ded79027d84f6fb4ccf35a3214684b
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