Light-induced formation of partially reduced oxygen species limits the lifetime of photosystem 1-based biocathodes

Photobiodevices use photosynthetic proteins such as those of the photosystem 1 (PS1) to enable light-induced charge separation, but they suffer from limited long-term stability. Here authors employ scanning photoelectrochemical microscopy on a PS1 biocathode and find that several pathways generate o...

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Autores principales: Fangyuan Zhao, Steffen Hardt, Volker Hartmann, Huijie Zhang, Marc M. Nowaczyk, Matthias Rögner, Nicolas Plumeré, Wolfgang Schuhmann, Felipe Conzuelo
Formato: article
Lenguaje:EN
Publicado: Nature Portfolio 2018
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Acceso en línea:https://doaj.org/article/eca6069b8969446a87ce91c47064ee48
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Sumario:Photobiodevices use photosynthetic proteins such as those of the photosystem 1 (PS1) to enable light-induced charge separation, but they suffer from limited long-term stability. Here authors employ scanning photoelectrochemical microscopy on a PS1 biocathode and find that several pathways generate oxygen radicals.