Measurement of linear response functions in Nuclear Magnetic Resonance
Abstract We measure multi-time correlation functions of a set of Pauli operators on a two-level system, which can be used to retrieve its associated linear response functions. The two-level system is an effective spin constructed from the nuclear spins of 1H atoms in a solution of 13C-labeled chloro...
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Nature Portfolio
2017
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oai:doaj.org-article:ed2e737a40cf40d48094adba08556e1a2021-12-02T15:05:21ZMeasurement of linear response functions in Nuclear Magnetic Resonance10.1038/s41598-017-13037-42045-2322https://doaj.org/article/ed2e737a40cf40d48094adba08556e1a2017-10-01T00:00:00Zhttps://doi.org/10.1038/s41598-017-13037-4https://doaj.org/toc/2045-2322Abstract We measure multi-time correlation functions of a set of Pauli operators on a two-level system, which can be used to retrieve its associated linear response functions. The two-level system is an effective spin constructed from the nuclear spins of 1H atoms in a solution of 13C-labeled chloroform. Response functions characterize the linear response of the system to a family of perturbations, allowing us to compute physical quantities such as the magnetic susceptibility of the effective spin. We use techniques exported from quantum information to measure time correlations on the two-level system. This approach requires the use of an ancillary qubit encoded in the nuclear spins of the 13C atoms and a sequence of controlled operations. Moreover, we demonstrate the ability of such a quantum platform to compute time-correlation functions of arbitrary order, which relate to higher-order corrections of perturbative methods. Particularly, we show three-time correlation functions for arbitrary times, and we also measure time correlation functions at fixed times up to tenth order.Tao XinJulen S. PedernalesLucas LamataEnrique SolanoGui-Lu LongNature PortfolioarticleMedicineRScienceQENScientific Reports, Vol 7, Iss 1, Pp 1-9 (2017) |
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Medicine R Science Q Tao Xin Julen S. Pedernales Lucas Lamata Enrique Solano Gui-Lu Long Measurement of linear response functions in Nuclear Magnetic Resonance |
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Abstract We measure multi-time correlation functions of a set of Pauli operators on a two-level system, which can be used to retrieve its associated linear response functions. The two-level system is an effective spin constructed from the nuclear spins of 1H atoms in a solution of 13C-labeled chloroform. Response functions characterize the linear response of the system to a family of perturbations, allowing us to compute physical quantities such as the magnetic susceptibility of the effective spin. We use techniques exported from quantum information to measure time correlations on the two-level system. This approach requires the use of an ancillary qubit encoded in the nuclear spins of the 13C atoms and a sequence of controlled operations. Moreover, we demonstrate the ability of such a quantum platform to compute time-correlation functions of arbitrary order, which relate to higher-order corrections of perturbative methods. Particularly, we show three-time correlation functions for arbitrary times, and we also measure time correlation functions at fixed times up to tenth order. |
format |
article |
author |
Tao Xin Julen S. Pedernales Lucas Lamata Enrique Solano Gui-Lu Long |
author_facet |
Tao Xin Julen S. Pedernales Lucas Lamata Enrique Solano Gui-Lu Long |
author_sort |
Tao Xin |
title |
Measurement of linear response functions in Nuclear Magnetic Resonance |
title_short |
Measurement of linear response functions in Nuclear Magnetic Resonance |
title_full |
Measurement of linear response functions in Nuclear Magnetic Resonance |
title_fullStr |
Measurement of linear response functions in Nuclear Magnetic Resonance |
title_full_unstemmed |
Measurement of linear response functions in Nuclear Magnetic Resonance |
title_sort |
measurement of linear response functions in nuclear magnetic resonance |
publisher |
Nature Portfolio |
publishDate |
2017 |
url |
https://doaj.org/article/ed2e737a40cf40d48094adba08556e1a |
work_keys_str_mv |
AT taoxin measurementoflinearresponsefunctionsinnuclearmagneticresonance AT julenspedernales measurementoflinearresponsefunctionsinnuclearmagneticresonance AT lucaslamata measurementoflinearresponsefunctionsinnuclearmagneticresonance AT enriquesolano measurementoflinearresponsefunctionsinnuclearmagneticresonance AT guilulong measurementoflinearresponsefunctionsinnuclearmagneticresonance |
_version_ |
1718388865491795968 |