Electroreforming of Biomass for Value-Added Products
Humanity’s overreliance on fossil fuels for chemical and energy production has resulted in uncontrollable carbon emissions that have warranted widespread concern regarding global warming. To address this issue, there is a growing body of research on renewable resources such as biomass, of which cell...
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MDPI AG
2021
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oai:doaj.org-article:ee1e62d6f79146d8b4e5bd43e25bd4542021-11-25T18:23:46ZElectroreforming of Biomass for Value-Added Products10.3390/mi121114052072-666Xhttps://doaj.org/article/ee1e62d6f79146d8b4e5bd43e25bd4542021-11-01T00:00:00Zhttps://www.mdpi.com/2072-666X/12/11/1405https://doaj.org/toc/2072-666XHumanity’s overreliance on fossil fuels for chemical and energy production has resulted in uncontrollable carbon emissions that have warranted widespread concern regarding global warming. To address this issue, there is a growing body of research on renewable resources such as biomass, of which cellulose is the most abundant type. In particular, the electrochemical reforming of biomass is especially promising, as it allows greater control over valorization processes and requires milder conditions. Driven by renewable electricity, electroreforming of biomass can be green and sustainable. Moreover, green hydrogen generation can be coupled to anodic biomass electroforming, which has attracted ever-increasing attention. The following review is a summary of recent developments related to electroreforming cellulose and its derivatives (glucose, hydroxymethylfurfural, levulinic acid). The electroreforming of biomass can be achieved on the anode of an electrochemical cell through electrooxidation, as well as on the cathode through electroreduction. Recent advances in the anodic electroreforming of cellulose and cellulose-derived glucose and 5-hydrooxylmethoylfurural (5-HMF) are first summarized. Then, the key achievements in the cathodic electroreforming of cellulose and cellulose-derived 5-HMF and levulinic acid are discussed. Afterward, the emerging research focusing on coupling hydrogen evolution with anodic biomass reforming for the cogeneration of green hydrogen fuel and value-added chemicals is reviewed. The final chapter of this paper provides our perspective on the challenges and future research directions of biomass electroreforming.Zi Iun LaiLi Quan LeeHong LiMDPI AGarticlebiomass electroreformingelectrooxidationelectrochemical hydrogenationcellulosegreen hydrogenMechanical engineering and machineryTJ1-1570ENMicromachines, Vol 12, Iss 1405, p 1405 (2021) |
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biomass electroreforming electrooxidation electrochemical hydrogenation cellulose green hydrogen Mechanical engineering and machinery TJ1-1570 |
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biomass electroreforming electrooxidation electrochemical hydrogenation cellulose green hydrogen Mechanical engineering and machinery TJ1-1570 Zi Iun Lai Li Quan Lee Hong Li Electroreforming of Biomass for Value-Added Products |
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Humanity’s overreliance on fossil fuels for chemical and energy production has resulted in uncontrollable carbon emissions that have warranted widespread concern regarding global warming. To address this issue, there is a growing body of research on renewable resources such as biomass, of which cellulose is the most abundant type. In particular, the electrochemical reforming of biomass is especially promising, as it allows greater control over valorization processes and requires milder conditions. Driven by renewable electricity, electroreforming of biomass can be green and sustainable. Moreover, green hydrogen generation can be coupled to anodic biomass electroforming, which has attracted ever-increasing attention. The following review is a summary of recent developments related to electroreforming cellulose and its derivatives (glucose, hydroxymethylfurfural, levulinic acid). The electroreforming of biomass can be achieved on the anode of an electrochemical cell through electrooxidation, as well as on the cathode through electroreduction. Recent advances in the anodic electroreforming of cellulose and cellulose-derived glucose and 5-hydrooxylmethoylfurural (5-HMF) are first summarized. Then, the key achievements in the cathodic electroreforming of cellulose and cellulose-derived 5-HMF and levulinic acid are discussed. Afterward, the emerging research focusing on coupling hydrogen evolution with anodic biomass reforming for the cogeneration of green hydrogen fuel and value-added chemicals is reviewed. The final chapter of this paper provides our perspective on the challenges and future research directions of biomass electroreforming. |
format |
article |
author |
Zi Iun Lai Li Quan Lee Hong Li |
author_facet |
Zi Iun Lai Li Quan Lee Hong Li |
author_sort |
Zi Iun Lai |
title |
Electroreforming of Biomass for Value-Added Products |
title_short |
Electroreforming of Biomass for Value-Added Products |
title_full |
Electroreforming of Biomass for Value-Added Products |
title_fullStr |
Electroreforming of Biomass for Value-Added Products |
title_full_unstemmed |
Electroreforming of Biomass for Value-Added Products |
title_sort |
electroreforming of biomass for value-added products |
publisher |
MDPI AG |
publishDate |
2021 |
url |
https://doaj.org/article/ee1e62d6f79146d8b4e5bd43e25bd454 |
work_keys_str_mv |
AT ziiunlai electroreformingofbiomassforvalueaddedproducts AT liquanlee electroreformingofbiomassforvalueaddedproducts AT hongli electroreformingofbiomassforvalueaddedproducts |
_version_ |
1718411233581858816 |