Characterization of aerosol particles during a high pollution episode over Mexico City

Abstract More than 7 thousand wildfires were recorded over Mexico in 2019, affecting almost 640 thousand hectares. Most of these fires occurred during the spring season generating dense smoke plumes, impacting urban areas in the central part of the Mexican plateau. From May 10 to 17, 2019, biomass b...

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Autores principales: Giovanni Carabali, José Villanueva-Macias, Luis A. Ladino, Harry Álvarez-Ospina, Graciela B. Raga, Gema Andraca-Ayala, Javier Miranda, Michel Grutter, Ma. Montserrat Silva, David Riveros-Rosas
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Publicado: Nature Portfolio 2021
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Acceso en línea:https://doaj.org/article/f0bbc8f7b1a44d5d8c6956965a06f97e
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spelling oai:doaj.org-article:f0bbc8f7b1a44d5d8c6956965a06f97e2021-11-21T12:19:00ZCharacterization of aerosol particles during a high pollution episode over Mexico City10.1038/s41598-021-01873-42045-2322https://doaj.org/article/f0bbc8f7b1a44d5d8c6956965a06f97e2021-11-01T00:00:00Zhttps://doi.org/10.1038/s41598-021-01873-4https://doaj.org/toc/2045-2322Abstract More than 7 thousand wildfires were recorded over Mexico in 2019, affecting almost 640 thousand hectares. Most of these fires occurred during the spring season generating dense smoke plumes, impacting urban areas in the central part of the Mexican plateau. From May 10 to 17, 2019, biomass burning (BB) plumes affected Mexico City (MC) and diffused across the basin, producing PM2.5 levels ~ 2 times higher than the nation's air quality standards. Average PM2.5 concentrations increased sharply from 29.4 ± 7.2 µg m−3 to 65.1 ± 13.6 µg m−3 when the dense smoke plumes were detected. The higher particle concentration impacted the aerosol optical depth (AOD) as values ~ 3 times greater than the annual mean (0.32 ± 0.12) were measured, which resulted in a 17% loss of global horizontal irradiation (GHI). Under these severe pollution conditions, the visibility (V a ) was reduced by ~ 80%. The high incidence of strong absorbent particles, such as soot and tarballs was revealed through electron microscopy and X-ray fluorescence (XRF) analysis. These techniques show chemical similarities between MC aerosols and those from the high-altitude (~ 4010 m. a. g. l.) Altzomoni Atmospheric Observatory, evidencing a strong influence of the BB emissions, suggesting a regional transport of these pollutants.Giovanni CarabaliJosé Villanueva-MaciasLuis A. LadinoHarry Álvarez-OspinaGraciela B. RagaGema Andraca-AyalaJavier MirandaMichel GrutterMa. Montserrat SilvaDavid Riveros-RosasNature PortfolioarticleMedicineRScienceQENScientific Reports, Vol 11, Iss 1, Pp 1-14 (2021)
institution DOAJ
collection DOAJ
language EN
topic Medicine
R
Science
Q
spellingShingle Medicine
R
Science
Q
Giovanni Carabali
José Villanueva-Macias
Luis A. Ladino
Harry Álvarez-Ospina
Graciela B. Raga
Gema Andraca-Ayala
Javier Miranda
Michel Grutter
Ma. Montserrat Silva
David Riveros-Rosas
Characterization of aerosol particles during a high pollution episode over Mexico City
description Abstract More than 7 thousand wildfires were recorded over Mexico in 2019, affecting almost 640 thousand hectares. Most of these fires occurred during the spring season generating dense smoke plumes, impacting urban areas in the central part of the Mexican plateau. From May 10 to 17, 2019, biomass burning (BB) plumes affected Mexico City (MC) and diffused across the basin, producing PM2.5 levels ~ 2 times higher than the nation's air quality standards. Average PM2.5 concentrations increased sharply from 29.4 ± 7.2 µg m−3 to 65.1 ± 13.6 µg m−3 when the dense smoke plumes were detected. The higher particle concentration impacted the aerosol optical depth (AOD) as values ~ 3 times greater than the annual mean (0.32 ± 0.12) were measured, which resulted in a 17% loss of global horizontal irradiation (GHI). Under these severe pollution conditions, the visibility (V a ) was reduced by ~ 80%. The high incidence of strong absorbent particles, such as soot and tarballs was revealed through electron microscopy and X-ray fluorescence (XRF) analysis. These techniques show chemical similarities between MC aerosols and those from the high-altitude (~ 4010 m. a. g. l.) Altzomoni Atmospheric Observatory, evidencing a strong influence of the BB emissions, suggesting a regional transport of these pollutants.
format article
author Giovanni Carabali
José Villanueva-Macias
Luis A. Ladino
Harry Álvarez-Ospina
Graciela B. Raga
Gema Andraca-Ayala
Javier Miranda
Michel Grutter
Ma. Montserrat Silva
David Riveros-Rosas
author_facet Giovanni Carabali
José Villanueva-Macias
Luis A. Ladino
Harry Álvarez-Ospina
Graciela B. Raga
Gema Andraca-Ayala
Javier Miranda
Michel Grutter
Ma. Montserrat Silva
David Riveros-Rosas
author_sort Giovanni Carabali
title Characterization of aerosol particles during a high pollution episode over Mexico City
title_short Characterization of aerosol particles during a high pollution episode over Mexico City
title_full Characterization of aerosol particles during a high pollution episode over Mexico City
title_fullStr Characterization of aerosol particles during a high pollution episode over Mexico City
title_full_unstemmed Characterization of aerosol particles during a high pollution episode over Mexico City
title_sort characterization of aerosol particles during a high pollution episode over mexico city
publisher Nature Portfolio
publishDate 2021
url https://doaj.org/article/f0bbc8f7b1a44d5d8c6956965a06f97e
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