Light-Induced Subpicosecond Lattice Symmetry Switch in MoTe_{2}
The recent development of ultrashort laser pulses allows for optical control of structural and electronic properties of complex quantum materials. The layered transition-metal dichalcogenide MoTe_{2}, which can crystallize into several different structures with distinct topological and electronic pr...
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American Physical Society
2019
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oai:doaj.org-article:f0bfc4ab9c5b44fabfea6a374b4f58972021-12-02T13:22:14ZLight-Induced Subpicosecond Lattice Symmetry Switch in MoTe_{2}10.1103/PhysRevX.9.0210362160-3308https://doaj.org/article/f0bfc4ab9c5b44fabfea6a374b4f58972019-05-01T00:00:00Zhttp://doi.org/10.1103/PhysRevX.9.021036http://doi.org/10.1103/PhysRevX.9.021036https://doaj.org/toc/2160-3308The recent development of ultrashort laser pulses allows for optical control of structural and electronic properties of complex quantum materials. The layered transition-metal dichalcogenide MoTe_{2}, which can crystallize into several different structures with distinct topological and electronic properties, provides possibilities to control or switch between different phases. In this study, we report a photoinduced subpicosecond structural transition between the type-II Weyl semimetal phase and normal-semimetal phase in bulk crystalline MoTe_{2} by using ultrafast pump-probe and time-resolved second-harmonic-generation spectroscopy. The phase transition is most clearly characterized by the dramatic change of the shear oscillation mode and the intensity loss of second-harmonic generation. This work opens up new possibilities for ultrafast manipulation of the topological properties of solids, enabling potentially practical applications for a topological switch device with ultrafast excitations.M. Y. ZhangZ. X. WangY. N. LiL. Y. ShiD. WuT. LinS. J. ZhangY. Q. LiuQ. M. LiuJ. WangT. DongN. L. WangAmerican Physical SocietyarticlePhysicsQC1-999ENPhysical Review X, Vol 9, Iss 2, p 021036 (2019) |
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Physics QC1-999 M. Y. Zhang Z. X. Wang Y. N. Li L. Y. Shi D. Wu T. Lin S. J. Zhang Y. Q. Liu Q. M. Liu J. Wang T. Dong N. L. Wang Light-Induced Subpicosecond Lattice Symmetry Switch in MoTe_{2} |
description |
The recent development of ultrashort laser pulses allows for optical control of structural and electronic properties of complex quantum materials. The layered transition-metal dichalcogenide MoTe_{2}, which can crystallize into several different structures with distinct topological and electronic properties, provides possibilities to control or switch between different phases. In this study, we report a photoinduced subpicosecond structural transition between the type-II Weyl semimetal phase and normal-semimetal phase in bulk crystalline MoTe_{2} by using ultrafast pump-probe and time-resolved second-harmonic-generation spectroscopy. The phase transition is most clearly characterized by the dramatic change of the shear oscillation mode and the intensity loss of second-harmonic generation. This work opens up new possibilities for ultrafast manipulation of the topological properties of solids, enabling potentially practical applications for a topological switch device with ultrafast excitations. |
format |
article |
author |
M. Y. Zhang Z. X. Wang Y. N. Li L. Y. Shi D. Wu T. Lin S. J. Zhang Y. Q. Liu Q. M. Liu J. Wang T. Dong N. L. Wang |
author_facet |
M. Y. Zhang Z. X. Wang Y. N. Li L. Y. Shi D. Wu T. Lin S. J. Zhang Y. Q. Liu Q. M. Liu J. Wang T. Dong N. L. Wang |
author_sort |
M. Y. Zhang |
title |
Light-Induced Subpicosecond Lattice Symmetry Switch in MoTe_{2} |
title_short |
Light-Induced Subpicosecond Lattice Symmetry Switch in MoTe_{2} |
title_full |
Light-Induced Subpicosecond Lattice Symmetry Switch in MoTe_{2} |
title_fullStr |
Light-Induced Subpicosecond Lattice Symmetry Switch in MoTe_{2} |
title_full_unstemmed |
Light-Induced Subpicosecond Lattice Symmetry Switch in MoTe_{2} |
title_sort |
light-induced subpicosecond lattice symmetry switch in mote_{2} |
publisher |
American Physical Society |
publishDate |
2019 |
url |
https://doaj.org/article/f0bfc4ab9c5b44fabfea6a374b4f5897 |
work_keys_str_mv |
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1718393187560587264 |