Light-Induced Subpicosecond Lattice Symmetry Switch in MoTe_{2}

The recent development of ultrashort laser pulses allows for optical control of structural and electronic properties of complex quantum materials. The layered transition-metal dichalcogenide MoTe_{2}, which can crystallize into several different structures with distinct topological and electronic pr...

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Autores principales: M. Y. Zhang, Z. X. Wang, Y. N. Li, L. Y. Shi, D. Wu, T. Lin, S. J. Zhang, Y. Q. Liu, Q. M. Liu, J. Wang, T. Dong, N. L. Wang
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Publicado: American Physical Society 2019
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Acceso en línea:https://doaj.org/article/f0bfc4ab9c5b44fabfea6a374b4f5897
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spelling oai:doaj.org-article:f0bfc4ab9c5b44fabfea6a374b4f58972021-12-02T13:22:14ZLight-Induced Subpicosecond Lattice Symmetry Switch in MoTe_{2}10.1103/PhysRevX.9.0210362160-3308https://doaj.org/article/f0bfc4ab9c5b44fabfea6a374b4f58972019-05-01T00:00:00Zhttp://doi.org/10.1103/PhysRevX.9.021036http://doi.org/10.1103/PhysRevX.9.021036https://doaj.org/toc/2160-3308The recent development of ultrashort laser pulses allows for optical control of structural and electronic properties of complex quantum materials. The layered transition-metal dichalcogenide MoTe_{2}, which can crystallize into several different structures with distinct topological and electronic properties, provides possibilities to control or switch between different phases. In this study, we report a photoinduced subpicosecond structural transition between the type-II Weyl semimetal phase and normal-semimetal phase in bulk crystalline MoTe_{2} by using ultrafast pump-probe and time-resolved second-harmonic-generation spectroscopy. The phase transition is most clearly characterized by the dramatic change of the shear oscillation mode and the intensity loss of second-harmonic generation. This work opens up new possibilities for ultrafast manipulation of the topological properties of solids, enabling potentially practical applications for a topological switch device with ultrafast excitations.M. Y. ZhangZ. X. WangY. N. LiL. Y. ShiD. WuT. LinS. J. ZhangY. Q. LiuQ. M. LiuJ. WangT. DongN. L. WangAmerican Physical SocietyarticlePhysicsQC1-999ENPhysical Review X, Vol 9, Iss 2, p 021036 (2019)
institution DOAJ
collection DOAJ
language EN
topic Physics
QC1-999
spellingShingle Physics
QC1-999
M. Y. Zhang
Z. X. Wang
Y. N. Li
L. Y. Shi
D. Wu
T. Lin
S. J. Zhang
Y. Q. Liu
Q. M. Liu
J. Wang
T. Dong
N. L. Wang
Light-Induced Subpicosecond Lattice Symmetry Switch in MoTe_{2}
description The recent development of ultrashort laser pulses allows for optical control of structural and electronic properties of complex quantum materials. The layered transition-metal dichalcogenide MoTe_{2}, which can crystallize into several different structures with distinct topological and electronic properties, provides possibilities to control or switch between different phases. In this study, we report a photoinduced subpicosecond structural transition between the type-II Weyl semimetal phase and normal-semimetal phase in bulk crystalline MoTe_{2} by using ultrafast pump-probe and time-resolved second-harmonic-generation spectroscopy. The phase transition is most clearly characterized by the dramatic change of the shear oscillation mode and the intensity loss of second-harmonic generation. This work opens up new possibilities for ultrafast manipulation of the topological properties of solids, enabling potentially practical applications for a topological switch device with ultrafast excitations.
format article
author M. Y. Zhang
Z. X. Wang
Y. N. Li
L. Y. Shi
D. Wu
T. Lin
S. J. Zhang
Y. Q. Liu
Q. M. Liu
J. Wang
T. Dong
N. L. Wang
author_facet M. Y. Zhang
Z. X. Wang
Y. N. Li
L. Y. Shi
D. Wu
T. Lin
S. J. Zhang
Y. Q. Liu
Q. M. Liu
J. Wang
T. Dong
N. L. Wang
author_sort M. Y. Zhang
title Light-Induced Subpicosecond Lattice Symmetry Switch in MoTe_{2}
title_short Light-Induced Subpicosecond Lattice Symmetry Switch in MoTe_{2}
title_full Light-Induced Subpicosecond Lattice Symmetry Switch in MoTe_{2}
title_fullStr Light-Induced Subpicosecond Lattice Symmetry Switch in MoTe_{2}
title_full_unstemmed Light-Induced Subpicosecond Lattice Symmetry Switch in MoTe_{2}
title_sort light-induced subpicosecond lattice symmetry switch in mote_{2}
publisher American Physical Society
publishDate 2019
url https://doaj.org/article/f0bfc4ab9c5b44fabfea6a374b4f5897
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