Dynamic evolution and reversibility of single-atom Ni(II) active site in 1T-MoS2 electrocatalysts for hydrogen evolution

While single atom catalysis combines heterogeneous materials with molecular understanding, the role of the single atoms remains vague. Here, authors examine single Ni on MoS2 via in situ X-ray absorption spectroscopy to reveal the intermediate and catalytically active species.

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Autores principales: Brian Pattengale, Yichao Huang, Xingxu Yan, Sizhuo Yang, Sabrina Younan, Wenhui Hu, Zhida Li, Sungsik Lee, Xiaoqing Pan, Jing Gu, Jier Huang
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Publicado: Nature Portfolio 2020
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Acceso en línea:https://doaj.org/article/f40f39b587c94aad95314bbf8a6ea22d
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spelling oai:doaj.org-article:f40f39b587c94aad95314bbf8a6ea22d2021-12-02T15:10:47ZDynamic evolution and reversibility of single-atom Ni(II) active site in 1T-MoS2 electrocatalysts for hydrogen evolution10.1038/s41467-020-17904-z2041-1723https://doaj.org/article/f40f39b587c94aad95314bbf8a6ea22d2020-08-01T00:00:00Zhttps://doi.org/10.1038/s41467-020-17904-zhttps://doaj.org/toc/2041-1723While single atom catalysis combines heterogeneous materials with molecular understanding, the role of the single atoms remains vague. Here, authors examine single Ni on MoS2 via in situ X-ray absorption spectroscopy to reveal the intermediate and catalytically active species.Brian PattengaleYichao HuangXingxu YanSizhuo YangSabrina YounanWenhui HuZhida LiSungsik LeeXiaoqing PanJing GuJier HuangNature PortfolioarticleScienceQENNature Communications, Vol 11, Iss 1, Pp 1-9 (2020)
institution DOAJ
collection DOAJ
language EN
topic Science
Q
spellingShingle Science
Q
Brian Pattengale
Yichao Huang
Xingxu Yan
Sizhuo Yang
Sabrina Younan
Wenhui Hu
Zhida Li
Sungsik Lee
Xiaoqing Pan
Jing Gu
Jier Huang
Dynamic evolution and reversibility of single-atom Ni(II) active site in 1T-MoS2 electrocatalysts for hydrogen evolution
description While single atom catalysis combines heterogeneous materials with molecular understanding, the role of the single atoms remains vague. Here, authors examine single Ni on MoS2 via in situ X-ray absorption spectroscopy to reveal the intermediate and catalytically active species.
format article
author Brian Pattengale
Yichao Huang
Xingxu Yan
Sizhuo Yang
Sabrina Younan
Wenhui Hu
Zhida Li
Sungsik Lee
Xiaoqing Pan
Jing Gu
Jier Huang
author_facet Brian Pattengale
Yichao Huang
Xingxu Yan
Sizhuo Yang
Sabrina Younan
Wenhui Hu
Zhida Li
Sungsik Lee
Xiaoqing Pan
Jing Gu
Jier Huang
author_sort Brian Pattengale
title Dynamic evolution and reversibility of single-atom Ni(II) active site in 1T-MoS2 electrocatalysts for hydrogen evolution
title_short Dynamic evolution and reversibility of single-atom Ni(II) active site in 1T-MoS2 electrocatalysts for hydrogen evolution
title_full Dynamic evolution and reversibility of single-atom Ni(II) active site in 1T-MoS2 electrocatalysts for hydrogen evolution
title_fullStr Dynamic evolution and reversibility of single-atom Ni(II) active site in 1T-MoS2 electrocatalysts for hydrogen evolution
title_full_unstemmed Dynamic evolution and reversibility of single-atom Ni(II) active site in 1T-MoS2 electrocatalysts for hydrogen evolution
title_sort dynamic evolution and reversibility of single-atom ni(ii) active site in 1t-mos2 electrocatalysts for hydrogen evolution
publisher Nature Portfolio
publishDate 2020
url https://doaj.org/article/f40f39b587c94aad95314bbf8a6ea22d
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