Structural Regulation of Pd‐Based Nanoalloys for Advanced Electrocatalysis

Palladium (Pd)‐based materials have attracted increasing attentions as a kind of novel candidate catalysts for many electrocatalytic reactions to replace classic platinum (Pt) catalysts, especially in the fuel cell‐related electrocatalysis. However, the requirement of high activity and stability tow...

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Autores principales:	Menggang Li, Zhonghong Xia, Mingchuan Luo, Lin He, Lu Tao, Weiwei Yang, Yongsheng Yu, Shaojun Guo
Formato:	article
Lenguaje:	EN
Publicado:	Wiley-VCH 2021
Materias:	dimensionality of Pd‐based nanoalloys electrocatalysis fuel cells palladium Materials of engineering and construction. Mechanics of materials TA401-492
Acceso en línea:	https://doaj.org/article/f50ad52421e948899dc411bba5ec0c64
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id	oai:doaj.org-article:f50ad52421e948899dc411bba5ec0c64
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spelling	oai:doaj.org-article:f50ad52421e948899dc411bba5ec0c642021-11-16T03:55:57ZStructural Regulation of Pd‐Based Nanoalloys for Advanced Electrocatalysis2688-404610.1002/smsc.202100061https://doaj.org/article/f50ad52421e948899dc411bba5ec0c642021-11-01T00:00:00Zhttps://doi.org/10.1002/smsc.202100061https://doaj.org/toc/2688-4046Palladium (Pd)‐based materials have attracted increasing attentions as a kind of novel candidate catalysts for many electrocatalytic reactions to replace classic platinum (Pt) catalysts, especially in the fuel cell‐related electrocatalysis. However, the requirement of high activity and stability toward further practical applications makes the development of Pd‐based catalysts cease to advance. Combining alloying and structure‐controlled strategies has well addressed this challenge by optimizing the adsorption/desorption behaviors toward reaction intermediates. Herein, the recent advances of rational structural designs in terms of tuning the dimensionalities of Pd‐based nanoalloys are overviewed. To further enhance the intrinsic electrocatalytic activity, several advanced strategies, including intermetallics, doping, defects, surface, and interface engineering, are presented to engineer the electronic and/or physical properties of Pd‐based electrocatalysts. Using typical electrocatalytic reactions as probes, the significance of structural regulation of Pd‐based nanocrystals on the enhanced electrocatalysis is demonstrated. Finally, several possible trends and challenges for future advanced research directions are presented. It is anticipated that the rational structural regulation can make promising Pd‐based catalysts touch the ceiling of electrocatalytic activity and stability.Menggang LiZhonghong XiaMingchuan LuoLin HeLu TaoWeiwei YangYongsheng YuShaojun GuoWiley-VCHarticledimensionality of Pd‐based nanoalloyselectrocatalysisfuel cellspalladiumMaterials of engineering and construction. Mechanics of materialsTA401-492ENSmall Science, Vol 1, Iss 11, Pp n/a-n/a (2021)
institution	DOAJ
collection	DOAJ
language	EN
topic	dimensionality of Pd‐based nanoalloys electrocatalysis fuel cells palladium Materials of engineering and construction. Mechanics of materials TA401-492
spellingShingle	dimensionality of Pd‐based nanoalloys electrocatalysis fuel cells palladium Materials of engineering and construction. Mechanics of materials TA401-492 Menggang Li Zhonghong Xia Mingchuan Luo Lin He Lu Tao Weiwei Yang Yongsheng Yu Shaojun Guo Structural Regulation of Pd‐Based Nanoalloys for Advanced Electrocatalysis
description	Palladium (Pd)‐based materials have attracted increasing attentions as a kind of novel candidate catalysts for many electrocatalytic reactions to replace classic platinum (Pt) catalysts, especially in the fuel cell‐related electrocatalysis. However, the requirement of high activity and stability toward further practical applications makes the development of Pd‐based catalysts cease to advance. Combining alloying and structure‐controlled strategies has well addressed this challenge by optimizing the adsorption/desorption behaviors toward reaction intermediates. Herein, the recent advances of rational structural designs in terms of tuning the dimensionalities of Pd‐based nanoalloys are overviewed. To further enhance the intrinsic electrocatalytic activity, several advanced strategies, including intermetallics, doping, defects, surface, and interface engineering, are presented to engineer the electronic and/or physical properties of Pd‐based electrocatalysts. Using typical electrocatalytic reactions as probes, the significance of structural regulation of Pd‐based nanocrystals on the enhanced electrocatalysis is demonstrated. Finally, several possible trends and challenges for future advanced research directions are presented. It is anticipated that the rational structural regulation can make promising Pd‐based catalysts touch the ceiling of electrocatalytic activity and stability.
format	article
author	Menggang Li Zhonghong Xia Mingchuan Luo Lin He Lu Tao Weiwei Yang Yongsheng Yu Shaojun Guo
author_facet	Menggang Li Zhonghong Xia Mingchuan Luo Lin He Lu Tao Weiwei Yang Yongsheng Yu Shaojun Guo
author_sort	Menggang Li
title	Structural Regulation of Pd‐Based Nanoalloys for Advanced Electrocatalysis
title_short	Structural Regulation of Pd‐Based Nanoalloys for Advanced Electrocatalysis
title_full	Structural Regulation of Pd‐Based Nanoalloys for Advanced Electrocatalysis
title_fullStr	Structural Regulation of Pd‐Based Nanoalloys for Advanced Electrocatalysis
title_full_unstemmed	Structural Regulation of Pd‐Based Nanoalloys for Advanced Electrocatalysis
title_sort	structural regulation of pd‐based nanoalloys for advanced electrocatalysis
publisher	Wiley-VCH
publishDate	2021
url	https://doaj.org/article/f50ad52421e948899dc411bba5ec0c64
work_keys_str_mv	AT menggangli structuralregulationofpdbasednanoalloysforadvancedelectrocatalysis AT zhonghongxia structuralregulationofpdbasednanoalloysforadvancedelectrocatalysis AT mingchuanluo structuralregulationofpdbasednanoalloysforadvancedelectrocatalysis AT linhe structuralregulationofpdbasednanoalloysforadvancedelectrocatalysis AT lutao structuralregulationofpdbasednanoalloysforadvancedelectrocatalysis AT weiweiyang structuralregulationofpdbasednanoalloysforadvancedelectrocatalysis AT yongshengyu structuralregulationofpdbasednanoalloysforadvancedelectrocatalysis AT shaojunguo structuralregulationofpdbasednanoalloysforadvancedelectrocatalysis
_version_	1718426820812996608

Structural Regulation of Pd‐Based Nanoalloys for Advanced Electrocatalysis

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